Distribution of Radiocesium in Gunma Prefecture Released by the Fukushima Daiichi Nuclear Power Plant Accident

We investigated the distribution of radiocesium in soils of Gunma Prefecture released by the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident. The arithmetic mean of the Cs-134/Cs-137 radioactivity ratio of soil samples (n = 253) from Gunma Pref. is 0.996±0.0014 (decay corrected to March 11, 2...

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Veröffentlicht in:BUNSEKI KAGAKU 2017/04/05, Vol.66(4), pp.281-297
Hauptverfasser: AIZAWA, Shoichi, TSUNODA, Kin-ichi
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description We investigated the distribution of radiocesium in soils of Gunma Prefecture released by the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident. The arithmetic mean of the Cs-134/Cs-137 radioactivity ratio of soil samples (n = 253) from Gunma Pref. is 0.996±0.0014 (decay corrected to March 11, 2011), which may indicate that the radiocesium precipitated in Gunma Pref. is mainly derived from the Reactors 2 and 3 in the FDNPP. The geometric mean of the concentrations (decay corrected to March 25, 2011) of radiocesium (Cs-134 + Cs-137) in soil samples (n = 267) collected from Gunma Pref. is about 1 kBq kg−1. However, the geometric mean (1.4 kBq kg−1, n = 171) of mountainous soil samples of Gunma Pref. is two or three-times higher than that (0.54 kBq kg−1, n = 96) of plain soil ones of the same pref. The profiles of vertical distribution of radiocesium in soil samples collected from 3 different environmental situations are quite similar despite the difference in the kinds and amount ratios of clay minerals included. Moreover, more than 95 % of radiocesium is retained within the upper part (0-4 cm), even though 5 years after elapsed. The relationship between the spatial radiation dose rate of sampling points (1 m height) and the concentrations of radiocesium in soil samples is positive but weak (r = 0.65), probably because the concentration of radiocesium in soil samples changes widely even in a small area. The distribution of radiocesium deposition obtained in this work is substantially consistent with that by the MEXT (Ministry of Education, Culture, Sports, Science and Technology) airborne radiation monitoring, except the area (≤10 kBq m−2) of the plain region of Gunma Pref.
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The arithmetic mean of the Cs-134/Cs-137 radioactivity ratio of soil samples (n = 253) from Gunma Pref. is 0.996±0.0014 (decay corrected to March 11, 2011), which may indicate that the radiocesium precipitated in Gunma Pref. is mainly derived from the Reactors 2 and 3 in the FDNPP. The geometric mean of the concentrations (decay corrected to March 25, 2011) of radiocesium (Cs-134 + Cs-137) in soil samples (n = 267) collected from Gunma Pref. is about 1 kBq kg−1. However, the geometric mean (1.4 kBq kg−1, n = 171) of mountainous soil samples of Gunma Pref. is two or three-times higher than that (0.54 kBq kg−1, n = 96) of plain soil ones of the same pref. The profiles of vertical distribution of radiocesium in soil samples collected from 3 different environmental situations are quite similar despite the difference in the kinds and amount ratios of clay minerals included. Moreover, more than 95 % of radiocesium is retained within the upper part (0-4 cm), even though 5 years after elapsed. The relationship between the spatial radiation dose rate of sampling points (1 m height) and the concentrations of radiocesium in soil samples is positive but weak (r = 0.65), probably because the concentration of radiocesium in soil samples changes widely even in a small area. 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The arithmetic mean of the Cs-134/Cs-137 radioactivity ratio of soil samples (n = 253) from Gunma Pref. is 0.996±0.0014 (decay corrected to March 11, 2011), which may indicate that the radiocesium precipitated in Gunma Pref. is mainly derived from the Reactors 2 and 3 in the FDNPP. The geometric mean of the concentrations (decay corrected to March 25, 2011) of radiocesium (Cs-134 + Cs-137) in soil samples (n = 267) collected from Gunma Pref. is about 1 kBq kg−1. However, the geometric mean (1.4 kBq kg−1, n = 171) of mountainous soil samples of Gunma Pref. is two or three-times higher than that (0.54 kBq kg−1, n = 96) of plain soil ones of the same pref. The profiles of vertical distribution of radiocesium in soil samples collected from 3 different environmental situations are quite similar despite the difference in the kinds and amount ratios of clay minerals included. Moreover, more than 95 % of radiocesium is retained within the upper part (0-4 cm), even though 5 years after elapsed. The relationship between the spatial radiation dose rate of sampling points (1 m height) and the concentrations of radiocesium in soil samples is positive but weak (r = 0.65), probably because the concentration of radiocesium in soil samples changes widely even in a small area. 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The arithmetic mean of the Cs-134/Cs-137 radioactivity ratio of soil samples (n = 253) from Gunma Pref. is 0.996±0.0014 (decay corrected to March 11, 2011), which may indicate that the radiocesium precipitated in Gunma Pref. is mainly derived from the Reactors 2 and 3 in the FDNPP. The geometric mean of the concentrations (decay corrected to March 25, 2011) of radiocesium (Cs-134 + Cs-137) in soil samples (n = 267) collected from Gunma Pref. is about 1 kBq kg−1. However, the geometric mean (1.4 kBq kg−1, n = 171) of mountainous soil samples of Gunma Pref. is two or three-times higher than that (0.54 kBq kg−1, n = 96) of plain soil ones of the same pref. The profiles of vertical distribution of radiocesium in soil samples collected from 3 different environmental situations are quite similar despite the difference in the kinds and amount ratios of clay minerals included. Moreover, more than 95 % of radiocesium is retained within the upper part (0-4 cm), even though 5 years after elapsed. The relationship between the spatial radiation dose rate of sampling points (1 m height) and the concentrations of radiocesium in soil samples is positive but weak (r = 0.65), probably because the concentration of radiocesium in soil samples changes widely even in a small area. The distribution of radiocesium deposition obtained in this work is substantially consistent with that by the MEXT (Ministry of Education, Culture, Sports, Science and Technology) airborne radiation monitoring, except the area (≤10 kBq m−2) of the plain region of Gunma Pref.</abstract><cop>Tokyo</cop><pub>The Japan Society for Analytical Chemistry</pub><doi>10.2116/bunsekikagaku.66.281</doi><tpages>17</tpages><oa>free_for_read</oa></addata></record>
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subjects Arithmetic
Clay minerals
Decay
Deposition
Education
Electric power plants
Environmental monitoring
Gunma Prefecture
Nuclear accidents
Nuclear electric power generation
Nuclear power
Nuclear power plants
Nuclear reactors
Radiation dosage
Radiation measurement
Radioactivity
radiocesium
soil
Soil investigations
Soil testing
Vertical distribution
γ-ray spectrometry
title Distribution of Radiocesium in Gunma Prefecture Released by the Fukushima Daiichi Nuclear Power Plant Accident
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