Lightning NOx influence on large-scale NOy and O3 plumes observed over the northern mid-latitudes
This paper describes the NO y plumes originating from lightning emissions based on 4 yr (2001-2005) of MOZAIC measurements in the upper troposphere of the northern mid-latitudes, together with ground- and space-based observations of lightning flashes and clouds. This analysis is primarily for the No...
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| Veröffentlicht in: | Tellus B: Chemical and Physical Meteorology 2014, Vol.66 (1), p.25544-17 |
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| creator | Gressent, Alicia Sauvage, Bastien Defer, Eric Pätz, Hans Werner Thomas, Karin Holle, Ronald Cammas, Jean-Pierre Nédélec, Philippe Boulanger, Damien Thouret, Valérie Volz-Thomas, Andreas |
| description | This paper describes the NO
y
plumes originating from lightning emissions based on 4 yr (2001-2005) of MOZAIC measurements in the upper troposphere of the northern mid-latitudes, together with ground- and space-based observations of lightning flashes and clouds. This analysis is primarily for the North Atlantic region where the MOZAIC flights are the most frequent and for which the measurements are well representative in space and time. The study investigates the influence of lightning NO
x
(LNO
x
) emissions on large-scale (300-2000 km) plumes (LSPs) of NO
y
. One hundred and twenty seven LSPs (6% of the total MOZAIC NO
y
dataset) have been attributed to LNO
x
emissions. Most of these LSPs were recorded over North America and the Atlantic mainly in spring and summer during the maximum lightning activity occurrence. The majority of the LSPs (74%) is related to warm conveyor belts and extra-tropical cyclones originating from North America and entering the intercontinental transport pathway between North America and Europe, leading to a negative (positive) west to east NO
y
(O
3
) zonal gradient with −0.4 (+18) ppbv difference during spring and −0.6 (+14) ppbv difference in summer. The NO
y
zonal gradient can correspond to the mixing of the plume with the background air. On the other hand, the O
3
gradient is associated with both mixing of background air and with photochemical production during transport. Such transatlantic LSPs may have a potential impact on the European pollution. The remaining sampled LSPs are related to mesoscale convection over Western Europe and the Mediterranean Sea (18%) and to tropical convection (8%). |
| doi_str_mv | 10.3402/tellusb.v66.25544 |
| format | Article |
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y
plumes originating from lightning emissions based on 4 yr (2001-2005) of MOZAIC measurements in the upper troposphere of the northern mid-latitudes, together with ground- and space-based observations of lightning flashes and clouds. This analysis is primarily for the North Atlantic region where the MOZAIC flights are the most frequent and for which the measurements are well representative in space and time. The study investigates the influence of lightning NO
x
(LNO
x
) emissions on large-scale (300-2000 km) plumes (LSPs) of NO
y
. One hundred and twenty seven LSPs (6% of the total MOZAIC NO
y
dataset) have been attributed to LNO
x
emissions. Most of these LSPs were recorded over North America and the Atlantic mainly in spring and summer during the maximum lightning activity occurrence. The majority of the LSPs (74%) is related to warm conveyor belts and extra-tropical cyclones originating from North America and entering the intercontinental transport pathway between North America and Europe, leading to a negative (positive) west to east NO
y
(O
3
) zonal gradient with −0.4 (+18) ppbv difference during spring and −0.6 (+14) ppbv difference in summer. The NO
y
zonal gradient can correspond to the mixing of the plume with the background air. On the other hand, the O
3
gradient is associated with both mixing of background air and with photochemical production during transport. Such transatlantic LSPs may have a potential impact on the European pollution. The remaining sampled LSPs are related to mesoscale convection over Western Europe and the Mediterranean Sea (18%) and to tropical convection (8%).</description><identifier>ISSN: 0280-6509</identifier><identifier>EISSN: 1600-0889</identifier><identifier>DOI: 10.3402/tellusb.v66.25544</identifier><language>eng</language><publisher>Stockholm: Taylor & Francis</publisher><subject>Air pollution ; Altitude ; Americas ; Convection ; Emissions ; Full text ; Influence ; Latitude ; Lightning ; lightning NO ; lightning NOx emissions ; Meteorology ; nitrogen species ; ozone ; Photochemicals ; Plumes ; Sciences of the Universe ; Spring ; Springs ; Stratosphere ; Summer ; the MOZAIC programme ; Transport ; Tropical cyclones ; Troposphere</subject><ispartof>Tellus B: Chemical and Physical Meteorology, 2014, Vol.66 (1), p.25544-17</ispartof><rights>2014 A. Gressent et al. 2014</rights><rights>Copyright Co-Action Publishing 2014</rights><rights>Attribution</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c407t-25ddfcaff78d6eab7d698be7450ac2eefc0f38b9b51cb8263fd84e0a6ee25aac3</citedby><cites>FETCH-LOGICAL-c407t-25ddfcaff78d6eab7d698be7450ac2eefc0f38b9b51cb8263fd84e0a6ee25aac3</cites><orcidid>0000-0002-9548-2078 ; 0000-0003-3478-1899</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.tandfonline.com/doi/pdf/10.3402/tellusb.v66.25544$$EPDF$$P50$$Ginformaworld$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.tandfonline.com/doi/full/10.3402/tellusb.v66.25544$$EHTML$$P50$$Ginformaworld$$Hfree_for_read</linktohtml><link.rule.ids>230,314,780,784,864,885,2102,4024,4139,27502,27923,27924,27925,59143,59144</link.rule.ids><backlink>$$Uhttps://hal.science/hal-04118176$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Gressent, Alicia</creatorcontrib><creatorcontrib>Sauvage, Bastien</creatorcontrib><creatorcontrib>Defer, Eric</creatorcontrib><creatorcontrib>Pätz, Hans Werner</creatorcontrib><creatorcontrib>Thomas, Karin</creatorcontrib><creatorcontrib>Holle, Ronald</creatorcontrib><creatorcontrib>Cammas, Jean-Pierre</creatorcontrib><creatorcontrib>Nédélec, Philippe</creatorcontrib><creatorcontrib>Boulanger, Damien</creatorcontrib><creatorcontrib>Thouret, Valérie</creatorcontrib><creatorcontrib>Volz-Thomas, Andreas</creatorcontrib><title>Lightning NOx influence on large-scale NOy and O3 plumes observed over the northern mid-latitudes</title><title>Tellus B: Chemical and Physical Meteorology</title><description>This paper describes the NO
y
plumes originating from lightning emissions based on 4 yr (2001-2005) of MOZAIC measurements in the upper troposphere of the northern mid-latitudes, together with ground- and space-based observations of lightning flashes and clouds. This analysis is primarily for the North Atlantic region where the MOZAIC flights are the most frequent and for which the measurements are well representative in space and time. The study investigates the influence of lightning NO
x
(LNO
x
) emissions on large-scale (300-2000 km) plumes (LSPs) of NO
y
. One hundred and twenty seven LSPs (6% of the total MOZAIC NO
y
dataset) have been attributed to LNO
x
emissions. Most of these LSPs were recorded over North America and the Atlantic mainly in spring and summer during the maximum lightning activity occurrence. The majority of the LSPs (74%) is related to warm conveyor belts and extra-tropical cyclones originating from North America and entering the intercontinental transport pathway between North America and Europe, leading to a negative (positive) west to east NO
y
(O
3
) zonal gradient with −0.4 (+18) ppbv difference during spring and −0.6 (+14) ppbv difference in summer. The NO
y
zonal gradient can correspond to the mixing of the plume with the background air. On the other hand, the O
3
gradient is associated with both mixing of background air and with photochemical production during transport. Such transatlantic LSPs may have a potential impact on the European pollution. The remaining sampled LSPs are related to mesoscale convection over Western Europe and the Mediterranean Sea (18%) and to tropical convection (8%).</description><subject>Air pollution</subject><subject>Altitude</subject><subject>Americas</subject><subject>Convection</subject><subject>Emissions</subject><subject>Full text</subject><subject>Influence</subject><subject>Latitude</subject><subject>Lightning</subject><subject>lightning NO</subject><subject>lightning NOx emissions</subject><subject>Meteorology</subject><subject>nitrogen species</subject><subject>ozone</subject><subject>Photochemicals</subject><subject>Plumes</subject><subject>Sciences of the Universe</subject><subject>Spring</subject><subject>Springs</subject><subject>Stratosphere</subject><subject>Summer</subject><subject>the MOZAIC programme</subject><subject>Transport</subject><subject>Tropical cyclones</subject><subject>Troposphere</subject><issn>0280-6509</issn><issn>1600-0889</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><sourceid>0YH</sourceid><sourceid>8G5</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><sourceid>GUQSH</sourceid><sourceid>M2O</sourceid><sourceid>DOA</sourceid><recordid>eNqNkkGLFDEQhRtRcF39Ad4CXvTQYyWdpNPgZVnUXRici55DdVKZ6SXTWZPu0fn39uwsgoLgqaDqe4-i6lXVaw6rRoJ4P1GMc-lXB61XQikpn1QXXAPUYEz3tLoAYaDWCrrn1YtS7gBAqk5fVLgetrtpHMYt-7L5yYYxxJlGRyyNLGLeUl0cRlqGR4ajZ5uG3cd5T4WlvlA-kGfpQJlNO2JjykvJI9sPvo44DdPsqbysngWMhV491svq26ePX69v6vXm8-311bp2EtqpFsr74DCE1nhN2Lded6anVipAJ4iCg9CYvusVd70RugneSALUREIhuuayuj37-oR39j4Pe8xHm3CwD42UtxbzNLhINqg2eGmUQkOyFU0fFG-gcU40ILE5eb07e-0w_mF1c7W2px5Izg1v9YEv7Nsze5_T95nKZPdDccs7cKQ0F8u14lIZAfAfqBSat9CqBX3zF3qX5jwuB1wo0UkNbdstFD9TLqdSMoXfy3Kwp1zYx1zYJRf2IReL5sNZs_w65T3-SDl6O-Exphwyjm4otvm3_BcOS8H9</recordid><startdate>2014</startdate><enddate>2014</enddate><creator>Gressent, Alicia</creator><creator>Sauvage, Bastien</creator><creator>Defer, Eric</creator><creator>Pätz, Hans Werner</creator><creator>Thomas, Karin</creator><creator>Holle, Ronald</creator><creator>Cammas, Jean-Pierre</creator><creator>Nédélec, Philippe</creator><creator>Boulanger, Damien</creator><creator>Thouret, Valérie</creator><creator>Volz-Thomas, Andreas</creator><general>Taylor & Francis</general><general>Ubiquity Press</general><general>Stockholm University 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NOx influence on large-scale NOy and O3 plumes observed over the northern mid-latitudes</title><author>Gressent, Alicia ; Sauvage, Bastien ; Defer, Eric ; Pätz, Hans Werner ; Thomas, Karin ; Holle, Ronald ; Cammas, Jean-Pierre ; Nédélec, Philippe ; Boulanger, Damien ; Thouret, Valérie ; Volz-Thomas, Andreas</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c407t-25ddfcaff78d6eab7d698be7450ac2eefc0f38b9b51cb8263fd84e0a6ee25aac3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>Air pollution</topic><topic>Altitude</topic><topic>Americas</topic><topic>Convection</topic><topic>Emissions</topic><topic>Full text</topic><topic>Influence</topic><topic>Latitude</topic><topic>Lightning</topic><topic>lightning NO</topic><topic>lightning NOx emissions</topic><topic>Meteorology</topic><topic>nitrogen species</topic><topic>ozone</topic><topic>Photochemicals</topic><topic>Plumes</topic><topic>Sciences of the Universe</topic><topic>Spring</topic><topic>Springs</topic><topic>Stratosphere</topic><topic>Summer</topic><topic>the MOZAIC programme</topic><topic>Transport</topic><topic>Tropical cyclones</topic><topic>Troposphere</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Gressent, Alicia</creatorcontrib><creatorcontrib>Sauvage, Bastien</creatorcontrib><creatorcontrib>Defer, Eric</creatorcontrib><creatorcontrib>Pätz, Hans Werner</creatorcontrib><creatorcontrib>Thomas, Karin</creatorcontrib><creatorcontrib>Holle, Ronald</creatorcontrib><creatorcontrib>Cammas, Jean-Pierre</creatorcontrib><creatorcontrib>Nédélec, Philippe</creatorcontrib><creatorcontrib>Boulanger, Damien</creatorcontrib><creatorcontrib>Thouret, Valérie</creatorcontrib><creatorcontrib>Volz-Thomas, Andreas</creatorcontrib><collection>Access via Taylor & Francis (Open Access 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Database</collection><collection>Publicly Available Content Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central Basic</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 2: Ocean Technology, Policy & Non-Living Resources</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><collection>Hyper Article en Ligne (HAL)</collection><collection>Hyper Article en Ligne (HAL) (Open Access)</collection><collection>DOAJ Directory of Open Access Journals</collection><jtitle>Tellus B: Chemical and Physical Meteorology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Gressent, Alicia</au><au>Sauvage, Bastien</au><au>Defer, Eric</au><au>Pätz, Hans Werner</au><au>Thomas, Karin</au><au>Holle, Ronald</au><au>Cammas, Jean-Pierre</au><au>Nédélec, Philippe</au><au>Boulanger, Damien</au><au>Thouret, Valérie</au><au>Volz-Thomas, Andreas</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Lightning NOx influence on large-scale NOy and O3 plumes observed over the northern mid-latitudes</atitle><jtitle>Tellus B: Chemical and Physical Meteorology</jtitle><date>2014</date><risdate>2014</risdate><volume>66</volume><issue>1</issue><spage>25544</spage><epage>17</epage><pages>25544-17</pages><issn>0280-6509</issn><eissn>1600-0889</eissn><abstract>This paper describes the NO
y
plumes originating from lightning emissions based on 4 yr (2001-2005) of MOZAIC measurements in the upper troposphere of the northern mid-latitudes, together with ground- and space-based observations of lightning flashes and clouds. This analysis is primarily for the North Atlantic region where the MOZAIC flights are the most frequent and for which the measurements are well representative in space and time. The study investigates the influence of lightning NO
x
(LNO
x
) emissions on large-scale (300-2000 km) plumes (LSPs) of NO
y
. One hundred and twenty seven LSPs (6% of the total MOZAIC NO
y
dataset) have been attributed to LNO
x
emissions. Most of these LSPs were recorded over North America and the Atlantic mainly in spring and summer during the maximum lightning activity occurrence. The majority of the LSPs (74%) is related to warm conveyor belts and extra-tropical cyclones originating from North America and entering the intercontinental transport pathway between North America and Europe, leading to a negative (positive) west to east NO
y
(O
3
) zonal gradient with −0.4 (+18) ppbv difference during spring and −0.6 (+14) ppbv difference in summer. The NO
y
zonal gradient can correspond to the mixing of the plume with the background air. On the other hand, the O
3
gradient is associated with both mixing of background air and with photochemical production during transport. Such transatlantic LSPs may have a potential impact on the European pollution. The remaining sampled LSPs are related to mesoscale convection over Western Europe and the Mediterranean Sea (18%) and to tropical convection (8%).</abstract><cop>Stockholm</cop><pub>Taylor & Francis</pub><doi>10.3402/tellusb.v66.25544</doi><tpages>17</tpages><orcidid>https://orcid.org/0000-0002-9548-2078</orcidid><orcidid>https://orcid.org/0000-0003-3478-1899</orcidid><oa>free_for_read</oa></addata></record> |
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| source | DOAJ Directory of Open Access Journals; Co-Action Open Access Journals; Elektronische Zeitschriftenbibliothek - Frei zugängliche E-Journals; Access via Taylor & Francis (Open Access Collection); Alma/SFX Local Collection |
| subjects | Air pollution Altitude Americas Convection Emissions Full text Influence Latitude Lightning lightning NO lightning NOx emissions Meteorology nitrogen species ozone Photochemicals Plumes Sciences of the Universe Spring Springs Stratosphere Summer the MOZAIC programme Transport Tropical cyclones Troposphere |
| title | Lightning NOx influence on large-scale NOy and O3 plumes observed over the northern mid-latitudes |
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