Cork stoppers as an effective sorbent for water treatment: the removal of mercury at environmentally relevant concentrations and conditions
The technical feasibility of using stopper-derived cork as an effective biosorbent towards bivalent mercury at environmentally relevant concentrations and conditions was evaluated in this study. Only 25 mg/L of cork powder was able to achieve 94 % of mercury removal for an initial mercury concentrat...
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| Veröffentlicht in: | Environmental science and pollution research international 2014-02, Vol.21 (3), p.2108-2121 |
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| creator | Lopes, Cláudia B Oliveira, Joana R Rocha, Luciana S Tavares, Daniela S Silva, Carlos M Silva, Susana P Hartog, Niels Duarte, Armando C Pereira, E |
| description | The technical feasibility of using stopper-derived cork as an effective biosorbent towards bivalent mercury at environmentally relevant concentrations and conditions was evaluated in this study. Only 25 mg/L of cork powder was able to achieve 94 % of mercury removal for an initial mercury concentration of 500 μg/L. It was found that under the conditions tested, the efficiency of mercury removal expressed as equilibrium removal percentage does not depend on the amount of cork or its particle size, but is very sensitive to initial metal concentration, with higher removal efficiencies at higher initial concentrations. Ion exchange was identified as one of the mechanisms involved in the sorption of Hg onto cork in the absence of ionic competition. Under ionic competition, stopper-derived cork showed to be extremely effective and selective for mercury in binary mixtures, while in complex matrices like seawater, moderate inhibition of the sorption process was observed, attributed to a change in mercury speciation. The loadings achieved are similar to the majority of literature values found for other biosorbents and for other metals, suggesting that cork stoppers can be recycled as an effective biosorbent for water treatment. However, the most interesting result is that equilibrium data show a very rare behaviour, with the isotherm presenting an almost square convex shape to the concentration axis, with an infinite slope for an Hg concentration in solution around 25 μg/L. |
| doi_str_mv | 10.1007/s11356-013-2104-0 |
| format | Article |
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Only 25 mg/L of cork powder was able to achieve 94 % of mercury removal for an initial mercury concentration of 500 μg/L. It was found that under the conditions tested, the efficiency of mercury removal expressed as equilibrium removal percentage does not depend on the amount of cork or its particle size, but is very sensitive to initial metal concentration, with higher removal efficiencies at higher initial concentrations. Ion exchange was identified as one of the mechanisms involved in the sorption of Hg onto cork in the absence of ionic competition. Under ionic competition, stopper-derived cork showed to be extremely effective and selective for mercury in binary mixtures, while in complex matrices like seawater, moderate inhibition of the sorption process was observed, attributed to a change in mercury speciation. The loadings achieved are similar to the majority of literature values found for other biosorbents and for other metals, suggesting that cork stoppers can be recycled as an effective biosorbent for water treatment. However, the most interesting result is that equilibrium data show a very rare behaviour, with the isotherm presenting an almost square convex shape to the concentration axis, with an infinite slope for an Hg concentration in solution around 25 μg/L.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-013-2104-0</identifier><identifier>PMID: 24026204</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer-Verlag</publisher><subject>Adsorption ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Bioremediation ; cork ; cork stoppers ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Feasibility studies ; Heavy metal content ; Heavy metals ; Hydrogen-Ion Concentration ; Industrial wastes ; Ion Exchange ; Mercury ; Mercury - analysis ; Mercury - chemistry ; Metal concentrations ; Metals ; Particle size ; Quercus ; Recycling ; Research Article ; Seawater ; Sorption ; Speciation ; Studies ; Waste Disposal, Fluid - methods ; Waste Water Technology ; Water Management ; Water Pollutants, Chemical - analysis ; Water Pollutants, Chemical - chemistry ; Water Pollution Control ; Water Purification - methods ; Water treatment ; Wood products</subject><ispartof>Environmental science and pollution research international, 2014-02, Vol.21 (3), p.2108-2121</ispartof><rights>Springer-Verlag Berlin Heidelberg 2013</rights><rights>Springer-Verlag Berlin Heidelberg 2014</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c459t-d29ca8345fcc7031c035f5527bc11f943c7da41bf447f0f21f9518d101b9baf03</citedby><cites>FETCH-LOGICAL-c459t-d29ca8345fcc7031c035f5527bc11f943c7da41bf447f0f21f9518d101b9baf03</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-013-2104-0$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-013-2104-0$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/24026204$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Lopes, Cláudia B</creatorcontrib><creatorcontrib>Oliveira, Joana R</creatorcontrib><creatorcontrib>Rocha, Luciana S</creatorcontrib><creatorcontrib>Tavares, Daniela S</creatorcontrib><creatorcontrib>Silva, Carlos M</creatorcontrib><creatorcontrib>Silva, Susana P</creatorcontrib><creatorcontrib>Hartog, Niels</creatorcontrib><creatorcontrib>Duarte, Armando C</creatorcontrib><creatorcontrib>Pereira, E</creatorcontrib><title>Cork stoppers as an effective sorbent for water treatment: the removal of mercury at environmentally relevant concentrations and conditions</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>The technical feasibility of using stopper-derived cork as an effective biosorbent towards bivalent mercury at environmentally relevant concentrations and conditions was evaluated in this study. Only 25 mg/L of cork powder was able to achieve 94 % of mercury removal for an initial mercury concentration of 500 μg/L. It was found that under the conditions tested, the efficiency of mercury removal expressed as equilibrium removal percentage does not depend on the amount of cork or its particle size, but is very sensitive to initial metal concentration, with higher removal efficiencies at higher initial concentrations. Ion exchange was identified as one of the mechanisms involved in the sorption of Hg onto cork in the absence of ionic competition. Under ionic competition, stopper-derived cork showed to be extremely effective and selective for mercury in binary mixtures, while in complex matrices like seawater, moderate inhibition of the sorption process was observed, attributed to a change in mercury speciation. The loadings achieved are similar to the majority of literature values found for other biosorbents and for other metals, suggesting that cork stoppers can be recycled as an effective biosorbent for water treatment. However, the most interesting result is that equilibrium data show a very rare behaviour, with the isotherm presenting an almost square convex shape to the concentration axis, with an infinite slope for an Hg concentration in solution around 25 μg/L.</description><subject>Adsorption</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Bioremediation</subject><subject>cork</subject><subject>cork stoppers</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Feasibility studies</subject><subject>Heavy metal content</subject><subject>Heavy metals</subject><subject>Hydrogen-Ion Concentration</subject><subject>Industrial wastes</subject><subject>Ion Exchange</subject><subject>Mercury</subject><subject>Mercury - analysis</subject><subject>Mercury - chemistry</subject><subject>Metal concentrations</subject><subject>Metals</subject><subject>Particle size</subject><subject>Quercus</subject><subject>Recycling</subject><subject>Research Article</subject><subject>Seawater</subject><subject>Sorption</subject><subject>Speciation</subject><subject>Studies</subject><subject>Waste Disposal, Fluid - methods</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollutants, Chemical - analysis</subject><subject>Water Pollutants, Chemical - chemistry</subject><subject>Water Pollution Control</subject><subject>Water Purification - methods</subject><subject>Water treatment</subject><subject>Wood 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stoppers as an effective sorbent for water treatment: the removal of mercury at environmentally relevant concentrations and conditions</title><author>Lopes, Cláudia B ; Oliveira, Joana R ; Rocha, Luciana S ; Tavares, Daniela S ; Silva, Carlos M ; Silva, Susana P ; Hartog, Niels ; Duarte, Armando C ; Pereira, E</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c459t-d29ca8345fcc7031c035f5527bc11f943c7da41bf447f0f21f9518d101b9baf03</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>Adsorption</topic><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Bioremediation</topic><topic>cork</topic><topic>cork stoppers</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Feasibility 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international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lopes, Cláudia B</au><au>Oliveira, Joana R</au><au>Rocha, Luciana S</au><au>Tavares, Daniela S</au><au>Silva, Carlos M</au><au>Silva, Susana P</au><au>Hartog, Niels</au><au>Duarte, Armando C</au><au>Pereira, E</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Cork stoppers as an effective sorbent for water treatment: the removal of mercury at environmentally relevant concentrations and conditions</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2014-02-01</date><risdate>2014</risdate><volume>21</volume><issue>3</issue><spage>2108</spage><epage>2121</epage><pages>2108-2121</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>The technical feasibility of using stopper-derived cork as an effective biosorbent towards bivalent mercury at environmentally relevant concentrations and conditions was evaluated in this study. Only 25 mg/L of cork powder was able to achieve 94 % of mercury removal for an initial mercury concentration of 500 μg/L. It was found that under the conditions tested, the efficiency of mercury removal expressed as equilibrium removal percentage does not depend on the amount of cork or its particle size, but is very sensitive to initial metal concentration, with higher removal efficiencies at higher initial concentrations. Ion exchange was identified as one of the mechanisms involved in the sorption of Hg onto cork in the absence of ionic competition. Under ionic competition, stopper-derived cork showed to be extremely effective and selective for mercury in binary mixtures, while in complex matrices like seawater, moderate inhibition of the sorption process was observed, attributed to a change in mercury speciation. The loadings achieved are similar to the majority of literature values found for other biosorbents and for other metals, suggesting that cork stoppers can be recycled as an effective biosorbent for water treatment. However, the most interesting result is that equilibrium data show a very rare behaviour, with the isotherm presenting an almost square convex shape to the concentration axis, with an infinite slope for an Hg concentration in solution around 25 μg/L.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer-Verlag</pub><pmid>24026204</pmid><doi>10.1007/s11356-013-2104-0</doi><tpages>14</tpages><oa>free_for_read</oa></addata></record> |
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| ispartof | Environmental science and pollution research international, 2014-02, Vol.21 (3), p.2108-2121 |
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| subjects | Adsorption Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Bioremediation cork cork stoppers Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Feasibility studies Heavy metal content Heavy metals Hydrogen-Ion Concentration Industrial wastes Ion Exchange Mercury Mercury - analysis Mercury - chemistry Metal concentrations Metals Particle size Quercus Recycling Research Article Seawater Sorption Speciation Studies Waste Disposal, Fluid - methods Waste Water Technology Water Management Water Pollutants, Chemical - analysis Water Pollutants, Chemical - chemistry Water Pollution Control Water Purification - methods Water treatment Wood products |
| title | Cork stoppers as an effective sorbent for water treatment: the removal of mercury at environmentally relevant concentrations and conditions |
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