Catalytic performance of sheet-like Fe/ZSM-5 zeolites for the selective oxidation of benzene with nitrous oxide

Nanostructuring of Fe/ZSM-5 results in significantly higher phenol productivity during benzene oxidation with nitrous oxide. Optimal performance is obtained at low iron content. [Display omitted] ► Nanometer-thin ZSM-5 nanosheets functionalized by iron. ► High hydrothermal stability of the Fe/ZSM-5...

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Veröffentlicht in:	Journal of catalysis 2013-03, Vol.299, p.81-89
Hauptverfasser:	Koekkoek, A.J.J., Kim, W., Degirmenci, V., Xin, H., Ryoo, R., Hensen, E.J.M.
Format:	Artikel
Sprache:	eng
Schlagworte:	Benzene Catalysis Catalysts catalytic activity Catalytic oxidation Chemical compounds Chemical reactions Chemistry Exact sciences and technology Fe/ZSM-5 General and physical chemistry Hierarchical zeolite Ion-exchange iron micropores nanosheets Nanostructured materials nitrous oxide oxidants Oxidation Phenol probability silicon spectroscopy Surface physical chemistry surfactants Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry transmission electron microscopy X-ray diffraction zeolites Zeolites: preparations and properties
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