Graphene nanosheets decorated with heterostructured ruthenium sulfide as catalyst for enhanced hydrogen evolution reaction
In present findings, a simple pyrolysis technique was applied to decorate S and N doped graphene with RuS2-CoO nanoparticles synthesizing a heterostructured nanocomposite RuS2-CoO@SNG. XPS results demonstrate the elemental composition of these nanomaterials with the hint of metal-metal charge transf...
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| creator | Naseeb, Warisha Khosa, Muhammad Kaleem Noor, Awal Qayyum, Sadaf Chen, Shaowei |
| description | In present findings, a simple pyrolysis technique was applied to decorate S and N doped graphene with RuS2-CoO nanoparticles synthesizing a heterostructured nanocomposite RuS2-CoO@SNG. XPS results demonstrate the elemental composition of these nanomaterials with the hint of metal-metal charge transfer phenomenon likely due to heterostructure composition. These modifications led to a significant active surface area resulting in elevated electrocatalytic performance. In comparison to benchmark Pt/C at -60 mV in 1 M KOH, hydrogen evolution reaction (HER) reached at current density around 10 mA cm-2 at -90 mV overpotential. The stability test displayed excellent results with a decrease of 2 mV in overpotential at current density of 10 mA cm-2. Results indicate that such heterostructured nanocomposites can be used as an effective catalyst for HER. |
| doi_str_mv | 10.1371/journal.pone.0311885 |
| format | Article |
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| subjects | Analysis Carbon Catalysis Catalysts Charge transfer Chemical composition Chemical synthesis Composition Current density Electrodes Electrolytes Electrons Energy consumption Engineering and Technology Evolution Fossil fuels Graphene Graphite - chemistry Greenhouse gases Heterostructures Hydrogen Hydrogen - chemistry Hydrogen evolution reactions Hydrogenation Methods Nanocomposites Nanocomposites - chemistry Nanomaterials Nanoparticles Nanostructures - chemistry Nanotechnology Physical Sciences Properties Pyrolysis Quantum dots Research and Analysis Methods Ruthenium Ruthenium - chemistry Spectrum analysis Stability tests Sulfides - chemistry |
| title | Graphene nanosheets decorated with heterostructured ruthenium sulfide as catalyst for enhanced hydrogen evolution reaction |
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