Heterogeneous Ice Nucleation by Soufriere Hills Volcanic Ash Immersed in Water Droplets
Fine particles of ash emitted during volcanic eruptions may sporadically influence cloud properties on a regional or global scale as well as influencing the dynamics of volcanic clouds and the subsequent dispersion of volcanic aerosol and gases. It has been shown that volcanic ash can trigger ice nu...
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| creator | Mangan, T P Atkinson, J D Neuberg, J W O'Sullivan, D Wilson, T W Whale, T F Neve, L Umo, N S Malkin, T L Murray, B J |
| description | Fine particles of ash emitted during volcanic eruptions may sporadically influence cloud properties on a regional or global scale as well as influencing the dynamics of volcanic clouds and the subsequent dispersion of volcanic aerosol and gases. It has been shown that volcanic ash can trigger ice nucleation, but ash from relatively few volcanoes has been studied for its ice nucleating ability. In this study we quantify the efficiency with which ash from the Soufriere Hills volcano on Montserrat nucleates ice when immersed in supercooled water droplets. Using an ash sample from the 11th February 2010 eruption, we report ice nucleating efficiencies from 246 to 265 K. This wide range of temperatures was achieved using two separate droplet freezing instruments, one employing nanolitre droplets, the other using microlitre droplets. Soufriere Hills volcanic ash was significantly more efficient than all other ash samples that have been previously examined. At present the reasons for these differences are not understood, but may be related to mineralogy, amorphous content and surface chemistry. |
| doi_str_mv | 10.1371/journal.pone.0169720 |
| format | Article |
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This is an open access article distributed under the terms of the Creative Commons Attribution License: http://creativecommons.org/licenses/by/4.0/ (the “License”), which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited. Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><rights>2017 Mangan et al 2017 Mangan et al</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a748t-636551608f04f8843aaa09516c1dd62629c981f9b93d991e9b5d45c38a476ece3</citedby><cites>FETCH-LOGICAL-a748t-636551608f04f8843aaa09516c1dd62629c981f9b93d991e9b5d45c38a476ece3</cites><orcidid>0000-0001-7053-5594</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC5215928/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC5215928/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,314,727,780,784,864,885,2102,2928,23866,27924,27925,53791,53793</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/28056077$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><contributor>Smith, Victoria C.</contributor><creatorcontrib>Mangan, T P</creatorcontrib><creatorcontrib>Atkinson, J D</creatorcontrib><creatorcontrib>Neuberg, J W</creatorcontrib><creatorcontrib>O'Sullivan, D</creatorcontrib><creatorcontrib>Wilson, T W</creatorcontrib><creatorcontrib>Whale, T F</creatorcontrib><creatorcontrib>Neve, L</creatorcontrib><creatorcontrib>Umo, N S</creatorcontrib><creatorcontrib>Malkin, T L</creatorcontrib><creatorcontrib>Murray, B J</creatorcontrib><title>Heterogeneous Ice Nucleation by Soufriere Hills Volcanic Ash Immersed in Water Droplets</title><title>PloS one</title><addtitle>PLoS One</addtitle><description>Fine particles of ash emitted during volcanic eruptions may sporadically influence cloud properties on a regional or global scale as well as influencing the dynamics of volcanic clouds and the subsequent dispersion of volcanic aerosol and gases. It has been shown that volcanic ash can trigger ice nucleation, but ash from relatively few volcanoes has been studied for its ice nucleating ability. In this study we quantify the efficiency with which ash from the Soufriere Hills volcano on Montserrat nucleates ice when immersed in supercooled water droplets. Using an ash sample from the 11th February 2010 eruption, we report ice nucleating efficiencies from 246 to 265 K. This wide range of temperatures was achieved using two separate droplet freezing instruments, one employing nanolitre droplets, the other using microlitre droplets. Soufriere Hills volcanic ash was significantly more efficient than all other ash samples that have been previously examined. At present the reasons for these differences are not understood, but may be related to mineralogy, amorphous content and surface chemistry.</description><subject>Atmospheric chemistry</subject><subject>Atmospheric nucleation</subject><subject>Biology and Life Sciences</subject><subject>Cloud properties</subject><subject>Clouds</subject><subject>Droplets</subject><subject>Earth Sciences</subject><subject>Ecology and Environmental Sciences</subject><subject>Freezing</subject><subject>Gases</subject><subject>Gases - chemistry</subject><subject>Hills</subject><subject>Ice</subject><subject>Ice accretion</subject><subject>Ice nucleation</subject><subject>Lava</subject><subject>Measurement</subject><subject>Measurement techniques</subject><subject>Mineralogy</subject><subject>Nucleation</subject><subject>Physical Sciences</subject><subject>Physics</subject><subject>Studies</subject><subject>Supercooled water</subject><subject>Surface chemistry</subject><subject>Temperature</subject><subject>Temperature range</subject><subject>Thermal properties</subject><subject>Volcanic activity</subject><subject>Volcanic aerosols</subject><subject>Volcanic ash</subject><subject>Volcanic Eruptions</subject><subject>Volcanic gases</subject><subject>Volcanoes</subject><subject>Water - 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It has been shown that volcanic ash can trigger ice nucleation, but ash from relatively few volcanoes has been studied for its ice nucleating ability. In this study we quantify the efficiency with which ash from the Soufriere Hills volcano on Montserrat nucleates ice when immersed in supercooled water droplets. Using an ash sample from the 11th February 2010 eruption, we report ice nucleating efficiencies from 246 to 265 K. This wide range of temperatures was achieved using two separate droplet freezing instruments, one employing nanolitre droplets, the other using microlitre droplets. Soufriere Hills volcanic ash was significantly more efficient than all other ash samples that have been previously examined. At present the reasons for these differences are not understood, but may be related to mineralogy, amorphous content and surface chemistry.</abstract><cop>United States</cop><pub>Public Library of Science</pub><pmid>28056077</pmid><doi>10.1371/journal.pone.0169720</doi><tpages>e0169720</tpages><orcidid>https://orcid.org/0000-0001-7053-5594</orcidid><oa>free_for_read</oa></addata></record> |
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| source | MEDLINE; DOAJ Directory of Open Access Journals; Public Library of Science (PLoS) Journals Open Access; EZB-FREE-00999 freely available EZB journals; PubMed Central; Free Full-Text Journals in Chemistry |
| subjects | Atmospheric chemistry Atmospheric nucleation Biology and Life Sciences Cloud properties Clouds Droplets Earth Sciences Ecology and Environmental Sciences Freezing Gases Gases - chemistry Hills Ice Ice accretion Ice nucleation Lava Measurement Measurement techniques Mineralogy Nucleation Physical Sciences Physics Studies Supercooled water Surface chemistry Temperature Temperature range Thermal properties Volcanic activity Volcanic aerosols Volcanic ash Volcanic Eruptions Volcanic gases Volcanoes Water - chemistry Water droplets Water drops |
| title | Heterogeneous Ice Nucleation by Soufriere Hills Volcanic Ash Immersed in Water Droplets |
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