High Coke-Resistance Pt/Mg1-xNixO Catalyst for Dry Reforming of Methane
A highly active and stable nano structured Pt/Mg1-xNixO catalysts was developed by a simple co-precipitation method. The obtained Pt/Mg1-xNixO catalyst exhibited cubic structure nanocatalyst with a size of 50-80 nm and realized CH4 and CO2 conversions as high as 98% at 900°C with excellent stability...
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| Veröffentlicht in: | PloS one 2016, Vol.11 (1), p.e0145862-e0145862 |
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| creator | Al-Doghachi, Faris A J Islam, Aminul Zainal, Zulkarnain Saiman, Mohd Izham Embong, Zaidi Taufiq-Yap, Yun Hin |
| description | A highly active and stable nano structured Pt/Mg1-xNixO catalysts was developed by a simple co-precipitation method. The obtained Pt/Mg1-xNixO catalyst exhibited cubic structure nanocatalyst with a size of 50-80 nm and realized CH4 and CO2 conversions as high as 98% at 900°C with excellent stability in the dry reforming of methane. The characterization of catalyst was performed using various kinds of analytical techniques including XRD, BET, XRF, TPR-H2, TGA, TEM, FESEM, FT-IR, and XPS analyses. Characterization of spent catalyst further confirms that Pt/Mg1-xNixO catalyst has high coke-resistance for dry reforming. Thus, the catalyst demonstrated in this study, offers a promising catalyst for resolving the dilemma between dispersion and reducibility of supported metal, as well as activity and stability during high temperature reactions. |
| doi_str_mv | 10.1371/journal.pone.0145862 |
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The obtained Pt/Mg1-xNixO catalyst exhibited cubic structure nanocatalyst with a size of 50-80 nm and realized CH4 and CO2 conversions as high as 98% at 900°C with excellent stability in the dry reforming of methane. The characterization of catalyst was performed using various kinds of analytical techniques including XRD, BET, XRF, TPR-H2, TGA, TEM, FESEM, FT-IR, and XPS analyses. Characterization of spent catalyst further confirms that Pt/Mg1-xNixO catalyst has high coke-resistance for dry reforming. Thus, the catalyst demonstrated in this study, offers a promising catalyst for resolving the dilemma between dispersion and reducibility of supported metal, as well as activity and stability during high temperature reactions.</description><identifier>ISSN: 1932-6203</identifier><identifier>EISSN: 1932-6203</identifier><identifier>DOI: 10.1371/journal.pone.0145862</identifier><identifier>PMID: 26745623</identifier><language>eng</language><publisher>United States: Public Library of Science</publisher><subject>Alternative energy sources ; Biogas ; Carbon dioxide ; Carbon Dioxide - chemistry ; Catalysis ; Catalysts ; Chemistry ; Coke ; Fluidized bed reactors ; Gases ; High temperature ; Hydrogen ; Magnesium - chemistry ; Metal Nanoparticles - chemistry ; Metal Nanoparticles - ultrastructure ; Metals ; Methane ; Methane - chemistry ; Nickel ; Nickel - chemistry ; Particle Size ; Platinum ; Platinum - chemistry ; Reforming ; Science ; Solid solutions ; Spectroscopy, Fourier Transform Infrared ; Stability ; Sulfur ; Synthesis gas ; Thermogravimetry ; X ray photoelectron spectroscopy</subject><ispartof>PloS one, 2016, Vol.11 (1), p.e0145862-e0145862</ispartof><rights>2016 Al-Doghachi et al. This is an open access article distributed under the terms of the Creative Commons Attribution License: http://creativecommons.org/licenses/by/4.0/ (the “License”), which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited. Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><rights>2016 Al-Doghachi et al 2016 Al-Doghachi et al</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c526t-2d6127254324f76eb330ea3954257d226a7f39d0eac5aa142b7ba274676a72d53</citedby><cites>FETCH-LOGICAL-c526t-2d6127254324f76eb330ea3954257d226a7f39d0eac5aa142b7ba274676a72d53</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC4706417/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC4706417/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,315,728,781,785,865,886,2103,2929,4025,23868,27925,27926,27927,53793,53795</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/26745623$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><contributor>Yang, Gang</contributor><creatorcontrib>Al-Doghachi, Faris A J</creatorcontrib><creatorcontrib>Islam, Aminul</creatorcontrib><creatorcontrib>Zainal, Zulkarnain</creatorcontrib><creatorcontrib>Saiman, Mohd Izham</creatorcontrib><creatorcontrib>Embong, Zaidi</creatorcontrib><creatorcontrib>Taufiq-Yap, Yun Hin</creatorcontrib><title>High Coke-Resistance Pt/Mg1-xNixO Catalyst for Dry Reforming of Methane</title><title>PloS one</title><addtitle>PLoS One</addtitle><description>A highly active and stable nano structured Pt/Mg1-xNixO catalysts was developed by a simple co-precipitation method. The obtained Pt/Mg1-xNixO catalyst exhibited cubic structure nanocatalyst with a size of 50-80 nm and realized CH4 and CO2 conversions as high as 98% at 900°C with excellent stability in the dry reforming of methane. The characterization of catalyst was performed using various kinds of analytical techniques including XRD, BET, XRF, TPR-H2, TGA, TEM, FESEM, FT-IR, and XPS analyses. Characterization of spent catalyst further confirms that Pt/Mg1-xNixO catalyst has high coke-resistance for dry reforming. 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Academic</collection><collection>PubMed Central (Full Participant titles)</collection><collection>DOAJ Directory of Open Access Journals</collection><jtitle>PloS one</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Al-Doghachi, Faris A J</au><au>Islam, Aminul</au><au>Zainal, Zulkarnain</au><au>Saiman, Mohd Izham</au><au>Embong, Zaidi</au><au>Taufiq-Yap, Yun Hin</au><au>Yang, Gang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>High Coke-Resistance Pt/Mg1-xNixO Catalyst for Dry Reforming of Methane</atitle><jtitle>PloS one</jtitle><addtitle>PLoS One</addtitle><date>2016</date><risdate>2016</risdate><volume>11</volume><issue>1</issue><spage>e0145862</spage><epage>e0145862</epage><pages>e0145862-e0145862</pages><issn>1932-6203</issn><eissn>1932-6203</eissn><abstract>A highly active and stable nano structured Pt/Mg1-xNixO catalysts was developed by a simple co-precipitation method. The obtained Pt/Mg1-xNixO catalyst exhibited cubic structure nanocatalyst with a size of 50-80 nm and realized CH4 and CO2 conversions as high as 98% at 900°C with excellent stability in the dry reforming of methane. The characterization of catalyst was performed using various kinds of analytical techniques including XRD, BET, XRF, TPR-H2, TGA, TEM, FESEM, FT-IR, and XPS analyses. Characterization of spent catalyst further confirms that Pt/Mg1-xNixO catalyst has high coke-resistance for dry reforming. Thus, the catalyst demonstrated in this study, offers a promising catalyst for resolving the dilemma between dispersion and reducibility of supported metal, as well as activity and stability during high temperature reactions.</abstract><cop>United States</cop><pub>Public Library of Science</pub><pmid>26745623</pmid><doi>10.1371/journal.pone.0145862</doi><oa>free_for_read</oa></addata></record> |
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| subjects | Alternative energy sources Biogas Carbon dioxide Carbon Dioxide - chemistry Catalysis Catalysts Chemistry Coke Fluidized bed reactors Gases High temperature Hydrogen Magnesium - chemistry Metal Nanoparticles - chemistry Metal Nanoparticles - ultrastructure Metals Methane Methane - chemistry Nickel Nickel - chemistry Particle Size Platinum Platinum - chemistry Reforming Science Solid solutions Spectroscopy, Fourier Transform Infrared Stability Sulfur Synthesis gas Thermogravimetry X ray photoelectron spectroscopy |
| title | High Coke-Resistance Pt/Mg1-xNixO Catalyst for Dry Reforming of Methane |
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