Volatilization of 137Cs and 106Ru from Borosilicate Glass Containing Actual High-Level Waste

Volatility of 137 Cs and 106Ru from borosilicate glass containing actual high‐level waste was measured in an almost closed stainless‐steel canister. The temperature dependence of the volatility of 137Cs was close to that obtained in our previous study using 134Cs. The volatility of 106Ru was about o...

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Veröffentlicht in:Journal of the American Ceramic Society 1989-08, Vol.72 (8), p.1438-1441
Hauptverfasser: Kamizono, Hiroshi, Kikkawa, Shizuo, Togashi, Yoshihiro, Tashiro, Shingo
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container_issue 8
container_start_page 1438
container_title Journal of the American Ceramic Society
container_volume 72
creator Kamizono, Hiroshi
Kikkawa, Shizuo
Togashi, Yoshihiro
Tashiro, Shingo
description Volatility of 137 Cs and 106Ru from borosilicate glass containing actual high‐level waste was measured in an almost closed stainless‐steel canister. The temperature dependence of the volatility of 137Cs was close to that obtained in our previous study using 134Cs. The volatility of 106Ru was about one‐fifth that of 137Cs at 600° and 800°C. The air contamination by 137Cs and 106Ru in the canister at 400°C was estimated at 1.8 × 102 and 2 × 10 Bq/cm3, respectively, when it was assumed that the glass contained a realistic amount of 137Cs and 106Ru expected in commercial waste glass. These results are useful for predicting safety in a storage facility under operation.
doi_str_mv 10.1111/j.1151-2916.1989.tb07669.x
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The temperature dependence of the volatility of 137Cs was close to that obtained in our previous study using 134Cs. The volatility of 106Ru was about one‐fifth that of 137Cs at 600° and 800°C. The air contamination by 137Cs and 106Ru in the canister at 400°C was estimated at 1.8 × 102 and 2 × 10 Bq/cm3, respectively, when it was assumed that the glass contained a realistic amount of 137Cs and 106Ru expected in commercial waste glass. These results are useful for predicting safety in a storage facility under operation.</description><identifier>ISSN: 0002-7820</identifier><identifier>EISSN: 1551-2916</identifier><identifier>DOI: 10.1111/j.1151-2916.1989.tb07669.x</identifier><identifier>CODEN: JACTAW</identifier><language>eng</language><publisher>Oxford, UK: Blackwell Publishing Ltd</publisher><subject>Applied sciences ; borosilicates ; Building materials. Ceramics. 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The temperature dependence of the volatility of 137Cs was close to that obtained in our previous study using 134Cs. The volatility of 106Ru was about one‐fifth that of 137Cs at 600° and 800°C. The air contamination by 137Cs and 106Ru in the canister at 400°C was estimated at 1.8 × 102 and 2 × 10 Bq/cm3, respectively, when it was assumed that the glass contained a realistic amount of 137Cs and 106Ru expected in commercial waste glass. These results are useful for predicting safety in a storage facility under operation.</description><subject>Applied sciences</subject><subject>borosilicates</subject><subject>Building materials. Ceramics. Glasses</subject><subject>cesium</subject><subject>Chemical industry and chemicals</subject><subject>Exact sciences and technology</subject><subject>glass</subject><subject>Glasses</subject><subject>nuclear waste</subject><subject>ruthenium</subject><subject>Structure, analysis, properties</subject><issn>0002-7820</issn><issn>1551-2916</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>1989</creationdate><recordtype>article</recordtype><recordid>eNo9kNFPwjAQxhujiYj-D43xddhb1619ExcEDWBCiLyYNGVrsTg2sg4F_3q7QLiHu1zuy_flfgjdA-mBr8e1HwyCUEDcA8FFr1mSJI5Fb3-BOsBOp0vUIYSEQcJDco1unFv71cujDvr8qArV2ML--V6VuDIYaJI6rMocA4lnO2zqaoOfq7pyXpapRuNhoZzDaVU2ypa2XOF-1uxUgUd29RWM9Y8u8EK5Rt-iK6MKp-9Os4vmL4N5OgrG78PXtD8OViENeRAzIWAJEc81CQUjnHMGueDUwDKOM53nyrDcLIkKBc3BhAaiKEqEYYmmwGkXPRxtt8plqjC1KjPr5La2G1UfZJwAi0TkZU9H2a8t9OF8BiJblHItW5Sy5SVblPKEUu7lWz8dQETbpOBoYf13-7OFqr99Ck2YXEyHkkxnyYRPJhLoP1mceKM</recordid><startdate>198908</startdate><enddate>198908</enddate><creator>Kamizono, Hiroshi</creator><creator>Kikkawa, Shizuo</creator><creator>Togashi, Yoshihiro</creator><creator>Tashiro, Shingo</creator><general>Blackwell Publishing Ltd</general><general>Blackwell</general><scope>BSCLL</scope><scope>IQODW</scope></search><sort><creationdate>198908</creationdate><title>Volatilization of 137Cs and 106Ru from Borosilicate Glass Containing Actual High-Level Waste</title><author>Kamizono, Hiroshi ; Kikkawa, Shizuo ; Togashi, Yoshihiro ; Tashiro, Shingo</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-g2328-65991b148de0295088851d983f1b66ceddaf5dfb0a293d1f2f144479f57e3183</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>1989</creationdate><topic>Applied sciences</topic><topic>borosilicates</topic><topic>Building materials. 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The temperature dependence of the volatility of 137Cs was close to that obtained in our previous study using 134Cs. The volatility of 106Ru was about one‐fifth that of 137Cs at 600° and 800°C. The air contamination by 137Cs and 106Ru in the canister at 400°C was estimated at 1.8 × 102 and 2 × 10 Bq/cm3, respectively, when it was assumed that the glass contained a realistic amount of 137Cs and 106Ru expected in commercial waste glass. These results are useful for predicting safety in a storage facility under operation.</abstract><cop>Oxford, UK</cop><pub>Blackwell Publishing Ltd</pub><doi>10.1111/j.1151-2916.1989.tb07669.x</doi><tpages>4</tpages></addata></record>
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subjects Applied sciences
borosilicates
Building materials. Ceramics. Glasses
cesium
Chemical industry and chemicals
Exact sciences and technology
glass
Glasses
nuclear waste
ruthenium
Structure, analysis, properties
title Volatilization of 137Cs and 106Ru from Borosilicate Glass Containing Actual High-Level Waste
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