Volatilization of 137Cs and 106Ru from Borosilicate Glass Containing Actual High-Level Waste
Volatility of 137 Cs and 106Ru from borosilicate glass containing actual high‐level waste was measured in an almost closed stainless‐steel canister. The temperature dependence of the volatility of 137Cs was close to that obtained in our previous study using 134Cs. The volatility of 106Ru was about o...
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Veröffentlicht in: | Journal of the American Ceramic Society 1989-08, Vol.72 (8), p.1438-1441 |
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container_title | Journal of the American Ceramic Society |
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creator | Kamizono, Hiroshi Kikkawa, Shizuo Togashi, Yoshihiro Tashiro, Shingo |
description | Volatility of 137 Cs and 106Ru from borosilicate glass containing actual high‐level waste was measured in an almost closed stainless‐steel canister. The temperature dependence of the volatility of 137Cs was close to that obtained in our previous study using 134Cs. The volatility of 106Ru was about one‐fifth that of 137Cs at 600° and 800°C. The air contamination by 137Cs and 106Ru in the canister at 400°C was estimated at 1.8 × 102 and 2 × 10 Bq/cm3, respectively, when it was assumed that the glass contained a realistic amount of 137Cs and 106Ru expected in commercial waste glass. These results are useful for predicting safety in a storage facility under operation. |
doi_str_mv | 10.1111/j.1151-2916.1989.tb07669.x |
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The temperature dependence of the volatility of 137Cs was close to that obtained in our previous study using 134Cs. The volatility of 106Ru was about one‐fifth that of 137Cs at 600° and 800°C. The air contamination by 137Cs and 106Ru in the canister at 400°C was estimated at 1.8 × 102 and 2 × 10 Bq/cm3, respectively, when it was assumed that the glass contained a realistic amount of 137Cs and 106Ru expected in commercial waste glass. These results are useful for predicting safety in a storage facility under operation.</description><identifier>ISSN: 0002-7820</identifier><identifier>EISSN: 1551-2916</identifier><identifier>DOI: 10.1111/j.1151-2916.1989.tb07669.x</identifier><identifier>CODEN: JACTAW</identifier><language>eng</language><publisher>Oxford, UK: Blackwell Publishing Ltd</publisher><subject>Applied sciences ; borosilicates ; Building materials. Ceramics. 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The temperature dependence of the volatility of 137Cs was close to that obtained in our previous study using 134Cs. The volatility of 106Ru was about one‐fifth that of 137Cs at 600° and 800°C. The air contamination by 137Cs and 106Ru in the canister at 400°C was estimated at 1.8 × 102 and 2 × 10 Bq/cm3, respectively, when it was assumed that the glass contained a realistic amount of 137Cs and 106Ru expected in commercial waste glass. These results are useful for predicting safety in a storage facility under operation.</description><subject>Applied sciences</subject><subject>borosilicates</subject><subject>Building materials. Ceramics. Glasses</subject><subject>cesium</subject><subject>Chemical industry and chemicals</subject><subject>Exact sciences and technology</subject><subject>glass</subject><subject>Glasses</subject><subject>nuclear waste</subject><subject>ruthenium</subject><subject>Structure, analysis, properties</subject><issn>0002-7820</issn><issn>1551-2916</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>1989</creationdate><recordtype>article</recordtype><recordid>eNo9kNFPwjAQxhujiYj-D43xddhb1619ExcEDWBCiLyYNGVrsTg2sg4F_3q7QLiHu1zuy_flfgjdA-mBr8e1HwyCUEDcA8FFr1mSJI5Fb3-BOsBOp0vUIYSEQcJDco1unFv71cujDvr8qArV2ML--V6VuDIYaJI6rMocA4lnO2zqaoOfq7pyXpapRuNhoZzDaVU2ypa2XOF-1uxUgUd29RWM9Y8u8EK5Rt-iK6MKp-9Os4vmL4N5OgrG78PXtD8OViENeRAzIWAJEc81CQUjnHMGueDUwDKOM53nyrDcLIkKBc3BhAaiKEqEYYmmwGkXPRxtt8plqjC1KjPr5La2G1UfZJwAi0TkZU9H2a8t9OF8BiJblHItW5Sy5SVblPKEUu7lWz8dQETbpOBoYf13-7OFqr99Ck2YXEyHkkxnyYRPJhLoP1mceKM</recordid><startdate>198908</startdate><enddate>198908</enddate><creator>Kamizono, Hiroshi</creator><creator>Kikkawa, Shizuo</creator><creator>Togashi, Yoshihiro</creator><creator>Tashiro, Shingo</creator><general>Blackwell Publishing Ltd</general><general>Blackwell</general><scope>BSCLL</scope><scope>IQODW</scope></search><sort><creationdate>198908</creationdate><title>Volatilization of 137Cs and 106Ru from Borosilicate Glass Containing Actual High-Level Waste</title><author>Kamizono, Hiroshi ; Kikkawa, Shizuo ; Togashi, Yoshihiro ; Tashiro, Shingo</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-g2328-65991b148de0295088851d983f1b66ceddaf5dfb0a293d1f2f144479f57e3183</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>1989</creationdate><topic>Applied sciences</topic><topic>borosilicates</topic><topic>Building materials. Ceramics. Glasses</topic><topic>cesium</topic><topic>Chemical industry and chemicals</topic><topic>Exact sciences and technology</topic><topic>glass</topic><topic>Glasses</topic><topic>nuclear waste</topic><topic>ruthenium</topic><topic>Structure, analysis, properties</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Kamizono, Hiroshi</creatorcontrib><creatorcontrib>Kikkawa, Shizuo</creatorcontrib><creatorcontrib>Togashi, Yoshihiro</creatorcontrib><creatorcontrib>Tashiro, Shingo</creatorcontrib><collection>Istex</collection><collection>Pascal-Francis</collection><jtitle>Journal of the American Ceramic Society</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Kamizono, Hiroshi</au><au>Kikkawa, Shizuo</au><au>Togashi, Yoshihiro</au><au>Tashiro, Shingo</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Volatilization of 137Cs and 106Ru from Borosilicate Glass Containing Actual High-Level Waste</atitle><jtitle>Journal of the American Ceramic Society</jtitle><date>1989-08</date><risdate>1989</risdate><volume>72</volume><issue>8</issue><spage>1438</spage><epage>1441</epage><pages>1438-1441</pages><issn>0002-7820</issn><eissn>1551-2916</eissn><coden>JACTAW</coden><abstract>Volatility of 137 Cs and 106Ru from borosilicate glass containing actual high‐level waste was measured in an almost closed stainless‐steel canister. The temperature dependence of the volatility of 137Cs was close to that obtained in our previous study using 134Cs. The volatility of 106Ru was about one‐fifth that of 137Cs at 600° and 800°C. The air contamination by 137Cs and 106Ru in the canister at 400°C was estimated at 1.8 × 102 and 2 × 10 Bq/cm3, respectively, when it was assumed that the glass contained a realistic amount of 137Cs and 106Ru expected in commercial waste glass. These results are useful for predicting safety in a storage facility under operation.</abstract><cop>Oxford, UK</cop><pub>Blackwell Publishing Ltd</pub><doi>10.1111/j.1151-2916.1989.tb07669.x</doi><tpages>4</tpages></addata></record> |
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subjects | Applied sciences borosilicates Building materials. Ceramics. Glasses cesium Chemical industry and chemicals Exact sciences and technology glass Glasses nuclear waste ruthenium Structure, analysis, properties |
title | Volatilization of 137Cs and 106Ru from Borosilicate Glass Containing Actual High-Level Waste |
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