Strain-Controlled Epitaxial Stabilization in Ultrathin LaNiO3 Films Grown by Pulsed Laser Deposition
We report on the epitaxial stabilization effect of strain on the growth of ultrathin heterostructures of a correlated metal LaNiO3 (10 unit cells, ∼3.84 nm; u.c. hereafter) grown on a series of perovskite oxide substrates with both tensile and compressive strain. An unusual polynomial dependence of...
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Veröffentlicht in: | Crystal growth & design 2013-06, Vol.13 (6), p.2256-2259 |
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creator | Moon, E. J Gray, B. A Pimpinelli, A Kareev, M Meyers, D Chakhalian, J |
description | We report on the epitaxial stabilization effect of strain on the growth of ultrathin heterostructures of a correlated metal LaNiO3 (10 unit cells, ∼3.84 nm; u.c. hereafter) grown on a series of perovskite oxide substrates with both tensile and compressive strain. An unusual polynomial dependence of the activation energy for surface relaxation processes in terms of the lattice misfit was observed. Our experimental investigations further demonstrate the influence of strain relaxation on the self-ordering of complex oxide compounds in the perovskite structure during high supersaturation monolayer (interrupted layer-by-layer) deposition. |
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J ; Gray, B. A ; Pimpinelli, A ; Kareev, M ; Meyers, D ; Chakhalian, J</creator><creatorcontrib>Moon, E. J ; Gray, B. A ; Pimpinelli, A ; Kareev, M ; Meyers, D ; Chakhalian, J</creatorcontrib><description>We report on the epitaxial stabilization effect of strain on the growth of ultrathin heterostructures of a correlated metal LaNiO3 (10 unit cells, ∼3.84 nm; u.c. hereafter) grown on a series of perovskite oxide substrates with both tensile and compressive strain. An unusual polynomial dependence of the activation energy for surface relaxation processes in terms of the lattice misfit was observed. Our experimental investigations further demonstrate the influence of strain relaxation on the self-ordering of complex oxide compounds in the perovskite structure during high supersaturation monolayer (interrupted layer-by-layer) deposition.</description><identifier>ISSN: 1528-7483</identifier><identifier>EISSN: 1528-7505</identifier><identifier>DOI: 10.1021/cg300958z</identifier><language>eng</language><publisher>Washington,DC: American Chemical Society</publisher><subject>Condensed matter: structure, mechanical and thermal properties ; Cross-disciplinary physics: materials science; rheology ; Equations of state, phase equilibria, and phase transitions ; Exact sciences and technology ; General studies of phase transitions ; Laser deposition ; Materials science ; Methods of crystal growth; physics of crystal growth ; Methods of deposition of films and coatings; film growth and epitaxy ; Order-disorder and statistical mechanics of model systems ; Physics ; Theory and models of crystal growth; physics of crystal growth, crystal morphology and orientation</subject><ispartof>Crystal growth & design, 2013-06, Vol.13 (6), p.2256-2259</ispartof><rights>Copyright © 2013 American Chemical Society</rights><rights>2014 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/cg300958z$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/cg300958z$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,780,784,27076,27924,27925,56738,56788</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=27449013$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>Moon, E. 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Our experimental investigations further demonstrate the influence of strain relaxation on the self-ordering of complex oxide compounds in the perovskite structure during high supersaturation monolayer (interrupted layer-by-layer) deposition.</description><subject>Condensed matter: structure, mechanical and thermal properties</subject><subject>Cross-disciplinary physics: materials science; rheology</subject><subject>Equations of state, phase equilibria, and phase transitions</subject><subject>Exact sciences and technology</subject><subject>General studies of phase transitions</subject><subject>Laser deposition</subject><subject>Materials science</subject><subject>Methods of crystal growth; physics of crystal growth</subject><subject>Methods of deposition of films and coatings; film growth and epitaxy</subject><subject>Order-disorder and statistical mechanics of model systems</subject><subject>Physics</subject><subject>Theory and models of crystal growth; physics of crystal growth, crystal morphology and orientation</subject><issn>1528-7483</issn><issn>1528-7505</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2013</creationdate><recordtype>article</recordtype><recordid>eNpFUEtLw0AYXETBWj34D_biMfrtK9kcJbZVCFaoPYcvL92y3YTdFG1_vSm-TjMwD4Yh5JrBLQPO7qo3AZAqfTghE6a4jhIF6vSXSy3OyUUIGwBIYiEmpF4NHo2Lss4NvrO2qemsNwN-GrR0NWBprDngYDpHjaNrO7qH95Hl-GyWgs6N3Qa68N2Ho-WevuxsGBtyDI2nD03fBXOMXpKzFkfl6genZD2fvWaPUb5cPGX3eYScqSFqayWQt5LHTalBibpVPJVtWjYVoEql1KhB6IozLLVMJFNMJUeMGaSxQDElN9-9PYYKbevRVSYUvTdb9PuCJ1KmwMS_D6tQbLqdd-OqgkFxvLD4u1B8AR8BYuY</recordid><startdate>20130605</startdate><enddate>20130605</enddate><creator>Moon, E. 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J</creatorcontrib><creatorcontrib>Gray, B. A</creatorcontrib><creatorcontrib>Pimpinelli, A</creatorcontrib><creatorcontrib>Kareev, M</creatorcontrib><creatorcontrib>Meyers, D</creatorcontrib><creatorcontrib>Chakhalian, J</creatorcontrib><collection>Pascal-Francis</collection><jtitle>Crystal growth & design</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Moon, E. J</au><au>Gray, B. A</au><au>Pimpinelli, A</au><au>Kareev, M</au><au>Meyers, D</au><au>Chakhalian, J</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Strain-Controlled Epitaxial Stabilization in Ultrathin LaNiO3 Films Grown by Pulsed Laser Deposition</atitle><jtitle>Crystal growth & design</jtitle><addtitle>Cryst. Growth Des</addtitle><date>2013-06-05</date><risdate>2013</risdate><volume>13</volume><issue>6</issue><spage>2256</spage><epage>2259</epage><pages>2256-2259</pages><issn>1528-7483</issn><eissn>1528-7505</eissn><abstract>We report on the epitaxial stabilization effect of strain on the growth of ultrathin heterostructures of a correlated metal LaNiO3 (10 unit cells, ∼3.84 nm; u.c. hereafter) grown on a series of perovskite oxide substrates with both tensile and compressive strain. An unusual polynomial dependence of the activation energy for surface relaxation processes in terms of the lattice misfit was observed. Our experimental investigations further demonstrate the influence of strain relaxation on the self-ordering of complex oxide compounds in the perovskite structure during high supersaturation monolayer (interrupted layer-by-layer) deposition.</abstract><cop>Washington,DC</cop><pub>American Chemical Society</pub><doi>10.1021/cg300958z</doi><tpages>4</tpages></addata></record> |
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subjects | Condensed matter: structure, mechanical and thermal properties Cross-disciplinary physics: materials science rheology Equations of state, phase equilibria, and phase transitions Exact sciences and technology General studies of phase transitions Laser deposition Materials science Methods of crystal growth physics of crystal growth Methods of deposition of films and coatings film growth and epitaxy Order-disorder and statistical mechanics of model systems Physics Theory and models of crystal growth physics of crystal growth, crystal morphology and orientation |
title | Strain-Controlled Epitaxial Stabilization in Ultrathin LaNiO3 Films Grown by Pulsed Laser Deposition |
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