An Autoradiographical Method Using an Imaging Plate for the Analyses of Plutonium Contamination in a Plutonium Handling Facility
An autoradiographical method using an imaging plate (IP) was developed to analyze plutonium contamination in a plutonium handling facility. The IPs were exposed to ten specimens having a single plutonium particle. Photostimulated luminescence (PSL) images of the specimens were taken using a laser sc...
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Veröffentlicht in: | Journal of nuclear science and technology 2011-06, Vol.48 (6), p.911-918 |
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creator | TAKASAKI, Koji SAGAWA, Naoki KUROSAWA, Shigeyuki MIZUNIWA, Harumi |
description | An autoradiographical method using an imaging plate (IP) was developed to analyze plutonium contamination in a plutonium handling facility. The IPs were exposed to ten specimens having a single plutonium particle. Photostimulated luminescence (PSL) images of the specimens were taken using a laser scanning machine. One relatively large spot induced by α-radioactivity from plutonium was observed in each PSL image. The plutonium-induced spots were discriminated by a threshold derived from background and the size of the spot. A good relationship between the PSL intensities of the spots and α- radioactivities measured using a radiation counter was obtained by least-square fitting, taking the fading effect into consideration. This method was applied to workplace monitoring in an actual uraniumplutonium mixed oxide (MOX) fuel fabrication facility. Plutonium contaminations were analyzed in ten other specimens having more than two plutonium spots. The α-radioactivities of plutonium contamination were derived from the PSL images and their relative errors were evaluated from exposure time. |
doi_str_mv | 10.1080/18811248.2011.9711777 |
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The IPs were exposed to ten specimens having a single plutonium particle. Photostimulated luminescence (PSL) images of the specimens were taken using a laser scanning machine. One relatively large spot induced by α-radioactivity from plutonium was observed in each PSL image. The plutonium-induced spots were discriminated by a threshold derived from background and the size of the spot. A good relationship between the PSL intensities of the spots and α- radioactivities measured using a radiation counter was obtained by least-square fitting, taking the fading effect into consideration. This method was applied to workplace monitoring in an actual uraniumplutonium mixed oxide (MOX) fuel fabrication facility. Plutonium contaminations were analyzed in ten other specimens having more than two plutonium spots. The α-radioactivities of plutonium contamination were derived from the PSL images and their relative errors were evaluated from exposure time.</description><identifier>ISSN: 0022-3131</identifier><identifier>EISSN: 1881-1248</identifier><identifier>DOI: 10.1080/18811248.2011.9711777</identifier><identifier>CODEN: JNSTAX</identifier><language>eng</language><publisher>Tokyo: Taylor & Francis Group</publisher><subject>alpha radioactivity ; Applied sciences ; autoradiography ; contamination ; Energy ; Energy. 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The IPs were exposed to ten specimens having a single plutonium particle. Photostimulated luminescence (PSL) images of the specimens were taken using a laser scanning machine. One relatively large spot induced by α-radioactivity from plutonium was observed in each PSL image. The plutonium-induced spots were discriminated by a threshold derived from background and the size of the spot. A good relationship between the PSL intensities of the spots and α- radioactivities measured using a radiation counter was obtained by least-square fitting, taking the fading effect into consideration. This method was applied to workplace monitoring in an actual uraniumplutonium mixed oxide (MOX) fuel fabrication facility. Plutonium contaminations were analyzed in ten other specimens having more than two plutonium spots. The α-radioactivities of plutonium contamination were derived from the PSL images and their relative errors were evaluated from exposure time.</description><subject>alpha radioactivity</subject><subject>Applied sciences</subject><subject>autoradiography</subject><subject>contamination</subject><subject>Energy</subject><subject>Energy. Thermal use of fuels</subject><subject>Exact sciences and technology</subject><subject>fading</subject><subject>Fission nuclear power plants</subject><subject>Fuels</subject><subject>image analysis</subject><subject>imaging plate</subject><subject>Installations for energy generation and conversion: thermal and electrical energy</subject><subject>MOX</subject><subject>Nuclear fuels</subject><subject>plutonium</subject><issn>0022-3131</issn><issn>1881-1248</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2011</creationdate><recordtype>article</recordtype><recordid>eNp9kEtLAzEUhYMoWKs_QcjG5dRkknntLMXaQkUXdj3c5tFGMklJpsjs_OnO0FZcubqPc8-58CF0T8mEkpI80rKkNOXlJCWUTqqC0qIoLtBo2CeDcIlGhKRpwiij1-gmxs9-zHlejtD31OHpofUBpPHbAPudEWDxq2p3XuJ1NG6LweFlA9uhfbfQKqx9wO1O4akD20UVsde90qc4c2jwzLsWGuOgNd5h4zD8ERfgpB2S5iCMNW13i6402KjuTnWM1vPnj9kiWb29LGfTVSIYSYsEsjKrMp5vpFZKQZpLtRFVxVkueakJVIQLrSoqMikrllLOM8UkEVrrbFMJwsYoO-aK4GMMStf7YBoIXU1JPWCszxjrAWN9wtj7Ho6-PcSejA7ghIm_5pRzSlnG-7un451xPZ4Gvnywsm6hsz6cTez_Vz_r3Yjn</recordid><startdate>20110601</startdate><enddate>20110601</enddate><creator>TAKASAKI, Koji</creator><creator>SAGAWA, Naoki</creator><creator>KUROSAWA, Shigeyuki</creator><creator>MIZUNIWA, Harumi</creator><general>Taylor & Francis Group</general><general>Atomic Energy Society of Japan</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20110601</creationdate><title>An Autoradiographical Method Using an Imaging Plate for the Analyses of Plutonium Contamination in a Plutonium Handling Facility</title><author>TAKASAKI, Koji ; SAGAWA, Naoki ; KUROSAWA, Shigeyuki ; MIZUNIWA, Harumi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c3027-a5859546bdfeeea26debc99436d48f0a904cfe91c5dd9321445e3d0cfff5b9c03</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2011</creationdate><topic>alpha radioactivity</topic><topic>Applied sciences</topic><topic>autoradiography</topic><topic>contamination</topic><topic>Energy</topic><topic>Energy. Thermal use of fuels</topic><topic>Exact sciences and technology</topic><topic>fading</topic><topic>Fission nuclear power plants</topic><topic>Fuels</topic><topic>image analysis</topic><topic>imaging plate</topic><topic>Installations for energy generation and conversion: thermal and electrical energy</topic><topic>MOX</topic><topic>Nuclear fuels</topic><topic>plutonium</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>TAKASAKI, Koji</creatorcontrib><creatorcontrib>SAGAWA, Naoki</creatorcontrib><creatorcontrib>KUROSAWA, Shigeyuki</creatorcontrib><creatorcontrib>MIZUNIWA, Harumi</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><jtitle>Journal of nuclear science and technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>TAKASAKI, Koji</au><au>SAGAWA, Naoki</au><au>KUROSAWA, Shigeyuki</au><au>MIZUNIWA, Harumi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>An Autoradiographical Method Using an Imaging Plate for the Analyses of Plutonium Contamination in a Plutonium Handling Facility</atitle><jtitle>Journal of nuclear science and technology</jtitle><date>2011-06-01</date><risdate>2011</risdate><volume>48</volume><issue>6</issue><spage>911</spage><epage>918</epage><pages>911-918</pages><issn>0022-3131</issn><eissn>1881-1248</eissn><coden>JNSTAX</coden><abstract>An autoradiographical method using an imaging plate (IP) was developed to analyze plutonium contamination in a plutonium handling facility. The IPs were exposed to ten specimens having a single plutonium particle. Photostimulated luminescence (PSL) images of the specimens were taken using a laser scanning machine. One relatively large spot induced by α-radioactivity from plutonium was observed in each PSL image. The plutonium-induced spots were discriminated by a threshold derived from background and the size of the spot. A good relationship between the PSL intensities of the spots and α- radioactivities measured using a radiation counter was obtained by least-square fitting, taking the fading effect into consideration. This method was applied to workplace monitoring in an actual uraniumplutonium mixed oxide (MOX) fuel fabrication facility. Plutonium contaminations were analyzed in ten other specimens having more than two plutonium spots. The α-radioactivities of plutonium contamination were derived from the PSL images and their relative errors were evaluated from exposure time.</abstract><cop>Tokyo</cop><pub>Taylor & Francis Group</pub><doi>10.1080/18811248.2011.9711777</doi><tpages>8</tpages><oa>free_for_read</oa></addata></record> |
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source | Elektronische Zeitschriftenbibliothek - Frei zugängliche E-Journals; Alma/SFX Local Collection; Free Full-Text Journals in Chemistry |
subjects | alpha radioactivity Applied sciences autoradiography contamination Energy Energy. Thermal use of fuels Exact sciences and technology fading Fission nuclear power plants Fuels image analysis imaging plate Installations for energy generation and conversion: thermal and electrical energy MOX Nuclear fuels plutonium |
title | An Autoradiographical Method Using an Imaging Plate for the Analyses of Plutonium Contamination in a Plutonium Handling Facility |
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