Sensitive and Selective Detection of Low-Frequency Vibrational Modes Through a Phase-Shifting Fourier Transform Spectroscopy
We introduce a sensitive technique for the measurement of impulsively excited vibrational Raman modes. A linear sweep in the instantaneous frequency of the probe pulse isolates Raman sidebands from noise, enhancing sensitivity. The temporal interference between two stretched, time-delayed pump pulse...
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Veröffentlicht in: | IEEE journal of quantum electronics 2009-07, Vol.45 (7), p.777-782 |
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container_title | IEEE journal of quantum electronics |
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creator | Schlup, P. Wilson, J.W. Bartels, R.A. |
description | We introduce a sensitive technique for the measurement of impulsively excited vibrational Raman modes. A linear sweep in the instantaneous frequency of the probe pulse isolates Raman sidebands from noise, enhancing sensitivity. The temporal interference between two stretched, time-delayed pump pulses allows us to selectively excite specific modes. The method is shown to be applicable to different phases of the samples. |
doi_str_mv | 10.1109/JQE.2009.2013121 |
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A linear sweep in the instantaneous frequency of the probe pulse isolates Raman sidebands from noise, enhancing sensitivity. The temporal interference between two stretched, time-delayed pump pulses allows us to selectively excite specific modes. The method is shown to be applicable to different phases of the samples.</description><identifier>ISSN: 0018-9197</identifier><identifier>EISSN: 1558-1713</identifier><identifier>DOI: 10.1109/JQE.2009.2013121</identifier><identifier>CODEN: IEJQA7</identifier><language>eng</language><publisher>New York, NY: IEEE</publisher><subject>Exact sciences and technology ; Excitation ; Fourier transforms ; Fundamental areas of phenomenology (including applications) ; Noise ; Nonlinear optics ; Optical interferometry ; Optical pulses ; Optical scattering ; Optics ; Phase detection ; Phases ; Physics ; Probes ; Pumps ; Quantum electronics ; Raman scattering ; Raman spectroscopy ; Spectroscopy ; Temporal logic ; Ultrafast optics ; Ultrafast processes; optical pulse generation and pulse compression ; Vibration measurement</subject><ispartof>IEEE journal of quantum electronics, 2009-07, Vol.45 (7), p.777-782</ispartof><rights>2009 INIST-CNRS</rights><rights>Copyright The Institute of Electrical and Electronics Engineers, Inc. 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A linear sweep in the instantaneous frequency of the probe pulse isolates Raman sidebands from noise, enhancing sensitivity. The temporal interference between two stretched, time-delayed pump pulses allows us to selectively excite specific modes. The method is shown to be applicable to different phases of the samples.</description><subject>Exact sciences and technology</subject><subject>Excitation</subject><subject>Fourier transforms</subject><subject>Fundamental areas of phenomenology (including applications)</subject><subject>Noise</subject><subject>Nonlinear optics</subject><subject>Optical interferometry</subject><subject>Optical pulses</subject><subject>Optical scattering</subject><subject>Optics</subject><subject>Phase detection</subject><subject>Phases</subject><subject>Physics</subject><subject>Probes</subject><subject>Pumps</subject><subject>Quantum electronics</subject><subject>Raman scattering</subject><subject>Raman spectroscopy</subject><subject>Spectroscopy</subject><subject>Temporal logic</subject><subject>Ultrafast optics</subject><subject>Ultrafast processes; optical pulse generation and pulse compression</subject><subject>Vibration measurement</subject><issn>0018-9197</issn><issn>1558-1713</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2009</creationdate><recordtype>article</recordtype><sourceid>RIE</sourceid><recordid>eNp9kUFvEzEQhS0EEqHljsTFQgJOWzzr3bV9RKUBqlSAEriuvJNx42qzDvYGFKk_Hi-JeuDAxfZovnnym8fYCxAXAMK8u_52dVEKYfIBEkp4xGZQ17oABfIxmwkBujBg1FP2LKW7XFaVFjN2v6Qh-dH_Im6HNV9ST_i3-kDj9AoDD44vwu9iHunnngY88B--i3Zq2Z7fhDUlvtrEsL_dcMu_bmyiYrnxbvTDLZ-HffQU-SraIbkQt3y5y7IxJAy7wzl74myf6PnpPmPf51ery0_F4svHz5fvFwVWUoxFo0hr1J2tO3CmQ0SJ0--RKrDoOtPBWqBpyKBUlbOu7JpO1ShJy7rUSp6xt0fdXQzZQxrbrU9IfW8HCvvU6sboGkqpM_nmv6SsGq1NU2Xw1T_gXbaaN5LVatVUotQyQ-IIYTacIrl2F_3WxkMLop1Sa3Nq7ZRae0otj7w-6dqEtnd5b-jTw1wJWkijTOZeHjlPRA_tWkhlTCn_AA2Uodw</recordid><startdate>20090701</startdate><enddate>20090701</enddate><creator>Schlup, P.</creator><creator>Wilson, J.W.</creator><creator>Bartels, R.A.</creator><general>IEEE</general><general>Institute of Electrical and Electronics Engineers</general><general>The Institute of Electrical and Electronics Engineers, Inc. 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A linear sweep in the instantaneous frequency of the probe pulse isolates Raman sidebands from noise, enhancing sensitivity. The temporal interference between two stretched, time-delayed pump pulses allows us to selectively excite specific modes. The method is shown to be applicable to different phases of the samples.</abstract><cop>New York, NY</cop><pub>IEEE</pub><doi>10.1109/JQE.2009.2013121</doi><tpages>6</tpages></addata></record> |
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source | IEEE Electronic Library (IEL) |
subjects | Exact sciences and technology Excitation Fourier transforms Fundamental areas of phenomenology (including applications) Noise Nonlinear optics Optical interferometry Optical pulses Optical scattering Optics Phase detection Phases Physics Probes Pumps Quantum electronics Raman scattering Raman spectroscopy Spectroscopy Temporal logic Ultrafast optics Ultrafast processes optical pulse generation and pulse compression Vibration measurement |
title | Sensitive and Selective Detection of Low-Frequency Vibrational Modes Through a Phase-Shifting Fourier Transform Spectroscopy |
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