Investigation of the Reaction of Partial Oxidation of Methane over Ni/La2O3 Catalyst

The reaction of the partial oxidation of methane was investigated over Ni/La2O3 catalysts prepared by impregnation. Two different reactors were used, a perfectly jet-stirred reactor and a fixed-bed reactor. The influences of nickel content, calcination temperature, reaction temperature, residence ti...

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Veröffentlicht in:	Energy & fuels 2006-11, Vol.20 (6), p.2321-2329
Hauptverfasser:	Fleys, Matthieu, Simon, Yves, Swierczynski, Dariusz, Kiennemann, Alain, Marquaire, Paul-Marie
Format:	Artikel
Sprache:	eng
Schlagworte:	Applied sciences Energy Exact sciences and technology Fuel processing. Carbochemistry and petrochemistry Fuels Gas processing
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creator	Fleys, Matthieu Simon, Yves Swierczynski, Dariusz Kiennemann, Alain Marquaire, Paul-Marie
description	The reaction of the partial oxidation of methane was investigated over Ni/La2O3 catalysts prepared by impregnation. Two different reactors were used, a perfectly jet-stirred reactor and a fixed-bed reactor. The influences of nickel content, calcination temperature, reaction temperature, residence time, and contact time were investigated. Mechanistic information was derived from the comparison of the results obtained in both reactors. Characterization techniques such as X-ray diffraction, temperature-programmed oxidation, temperature-programmed reduction, and transmission electron microscopy were used to assess the state of the catalyst prior to and after the reaction.
doi_str_mv	10.1021/ef0602729
format	Article
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title	Investigation of the Reaction of Partial Oxidation of Methane over Ni/La2O3 Catalyst
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