Mechanisms of impedance rise in high-power, lithium-ion cells
Cells were life-cycled cells using profiles with a 3, 6, or 9% change in state of charge (ΔSOC) at 40, 50, 60, and 70 °C. From the voltage response of the cells to the life-cycle profile at each temperature, we separated the overall impedance rise into two simpler terms, R o (ohmic) and R p (polariz...
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| Veröffentlicht in: | Journal of power sources 2002-09, Vol.111 (1), p.152-159 |
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| container_issue | 1 |
| container_start_page | 152 |
| container_title | Journal of power sources |
| container_volume | 111 |
| creator | Bloom, Ira Jones, Scott A. Polzin, Edward G. Battaglia, Vincent S. Henriksen, Gary L. Motloch, Chester G. Wright, Randy B. Jungst, Rudolph G. Case, Herbert L. Doughty, Daniel H. |
| description | Cells were life-cycled cells using profiles with a 3, 6, or 9% change in state of charge (ΔSOC) at 40, 50, 60, and 70
°C. From the voltage response of the cells to the life-cycle profile at each temperature, we separated the overall impedance rise into two simpler terms,
R
o (ohmic) and
R
p (polarization), using an equivalent circuit model. The
R
o data tend to follow the expected trends (40>50>60>70
°C). Although the
R
p data trends show that
R
p can either decrease or increase asymptotically with time, the overall temperature-dependent behavior is similar to that of
R
o. We illustrate the types of processes that can occur in one lithium-ion cell chemistry. Based on the initial rates, the processes are complex. The
R
o term dominates the observable cell impedance, but
R
p adds a non-trivial contribution. |
| doi_str_mv | 10.1016/S0378-7753(02)00302-6 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_osti_</sourceid><recordid>TN_cdi_osti_scitechconnect_949694</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><els_id>S0378775302003026</els_id><sourcerecordid>27215043</sourcerecordid><originalsourceid>FETCH-LOGICAL-c394t-4c59f284e4811828c62ac2c6d698618bd3d72898347612b0ae45ad4be8a6b1b73</originalsourceid><addsrcrecordid>eNqFkE1v1DAURS0EEsPAT0BKF1RUquH5I7azqBCq2oLUqgtgbTnOS8coiVM7A-LfN5lU7ZLV25z77tUh5D2DTwyY-vwDhDZU61J8BH4CIIBT9YJsmNGCcl2WL8nmCXlN3uT8GwAY07AhZzfod24Iuc9FbIvQj9i4wWORQsYiDMUu3O3oGP9iOi26MO3CvqchDoXHrstvyavWdRnfPd4t-XV58fP8G72-vfp-_vWaelHJiUpfVi03EqVhzHDjFXeee9Woyihm6kY0mpvKCKkV4zU4lKVrZI3GqZrVWmzJ0fo35inY7MM0r_ZxGNBPtpKVquTMHK_MmOL9HvNk-5CXlW7AuM-Wa85KkGIGyxX0KeacsLVjCr1L_ywDuwi1B6F2sWWB24NQq-bch8cCl73r2jR7Cvk5LBWAEXzmvqwczkb-BEzLYJydNiEte5sY_tP0AJR8iAk</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>27215043</pqid></control><display><type>article</type><title>Mechanisms of impedance rise in high-power, lithium-ion cells</title><source>ScienceDirect Journals (5 years ago - present)</source><creator>Bloom, Ira ; Jones, Scott A. ; Polzin, Edward G. ; Battaglia, Vincent S. ; Henriksen, Gary L. ; Motloch, Chester G. ; Wright, Randy B. ; Jungst, Rudolph G. ; Case, Herbert L. ; Doughty, Daniel H.</creator><creatorcontrib>Bloom, Ira ; Jones, Scott A. ; Polzin, Edward G. ; Battaglia, Vincent S. ; Henriksen, Gary L. ; Motloch, Chester G. ; Wright, Randy B. ; Jungst, Rudolph G. ; Case, Herbert L. ; Doughty, Daniel H. ; Argonne National Lab. (ANL), Argonne, IL (United States)</creatorcontrib><description>Cells were life-cycled cells using profiles with a 3, 6, or 9% change in state of charge (ΔSOC) at 40, 50, 60, and 70
°C. From the voltage response of the cells to the life-cycle profile at each temperature, we separated the overall impedance rise into two simpler terms,
R
o (ohmic) and
R
p (polarization), using an equivalent circuit model. The
R
o data tend to follow the expected trends (40>50>60>70
°C). Although the
R
p data trends show that
R
p can either decrease or increase asymptotically with time, the overall temperature-dependent behavior is similar to that of
R
o. We illustrate the types of processes that can occur in one lithium-ion cell chemistry. Based on the initial rates, the processes are complex. The
R
o term dominates the observable cell impedance, but
R
p adds a non-trivial contribution.</description><identifier>ISSN: 0378-7753</identifier><identifier>EISSN: 1873-2755</identifier><identifier>DOI: 10.1016/S0378-7753(02)00302-6</identifier><identifier>CODEN: JPSODZ</identifier><language>eng</language><publisher>Lausanne: Elsevier B.V</publisher><subject>Applied sciences ; CHEMISTRY ; Direct energy conversion and energy accumulation ; Electrical engineering. Electrical power engineering ; Electrical power engineering ; Electrochemical conversion: primary and secondary batteries, fuel cells ; ENERGY STORAGE ; EQUIVALENT CIRCUITS ; Exact sciences and technology ; High-power ; IMPEDANCE ; LIFE CYCLE ; Lithium-ion ; POLARIZATION</subject><ispartof>Journal of power sources, 2002-09, Vol.111 (1), p.152-159</ispartof><rights>2002 Elsevier Science B.V.</rights><rights>2003 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c394t-4c59f284e4811828c62ac2c6d698618bd3d72898347612b0ae45ad4be8a6b1b73</citedby><cites>FETCH-LOGICAL-c394t-4c59f284e4811828c62ac2c6d698618bd3d72898347612b0ae45ad4be8a6b1b73</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0378775302003026$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>230,314,776,780,881,3537,27901,27902,65534</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=14600832$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/biblio/949694$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Bloom, Ira</creatorcontrib><creatorcontrib>Jones, Scott A.</creatorcontrib><creatorcontrib>Polzin, Edward G.</creatorcontrib><creatorcontrib>Battaglia, Vincent S.</creatorcontrib><creatorcontrib>Henriksen, Gary L.</creatorcontrib><creatorcontrib>Motloch, Chester G.</creatorcontrib><creatorcontrib>Wright, Randy B.</creatorcontrib><creatorcontrib>Jungst, Rudolph G.</creatorcontrib><creatorcontrib>Case, Herbert L.</creatorcontrib><creatorcontrib>Doughty, Daniel H.</creatorcontrib><creatorcontrib>Argonne National Lab. (ANL), Argonne, IL (United States)</creatorcontrib><title>Mechanisms of impedance rise in high-power, lithium-ion cells</title><title>Journal of power sources</title><description>Cells were life-cycled cells using profiles with a 3, 6, or 9% change in state of charge (ΔSOC) at 40, 50, 60, and 70
°C. From the voltage response of the cells to the life-cycle profile at each temperature, we separated the overall impedance rise into two simpler terms,
R
o (ohmic) and
R
p (polarization), using an equivalent circuit model. The
R
o data tend to follow the expected trends (40>50>60>70
°C). Although the
R
p data trends show that
R
p can either decrease or increase asymptotically with time, the overall temperature-dependent behavior is similar to that of
R
o. We illustrate the types of processes that can occur in one lithium-ion cell chemistry. Based on the initial rates, the processes are complex. The
R
o term dominates the observable cell impedance, but
R
p adds a non-trivial contribution.</description><subject>Applied sciences</subject><subject>CHEMISTRY</subject><subject>Direct energy conversion and energy accumulation</subject><subject>Electrical engineering. Electrical power engineering</subject><subject>Electrical power engineering</subject><subject>Electrochemical conversion: primary and secondary batteries, fuel cells</subject><subject>ENERGY STORAGE</subject><subject>EQUIVALENT CIRCUITS</subject><subject>Exact sciences and technology</subject><subject>High-power</subject><subject>IMPEDANCE</subject><subject>LIFE CYCLE</subject><subject>Lithium-ion</subject><subject>POLARIZATION</subject><issn>0378-7753</issn><issn>1873-2755</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2002</creationdate><recordtype>article</recordtype><recordid>eNqFkE1v1DAURS0EEsPAT0BKF1RUquH5I7azqBCq2oLUqgtgbTnOS8coiVM7A-LfN5lU7ZLV25z77tUh5D2DTwyY-vwDhDZU61J8BH4CIIBT9YJsmNGCcl2WL8nmCXlN3uT8GwAY07AhZzfod24Iuc9FbIvQj9i4wWORQsYiDMUu3O3oGP9iOi26MO3CvqchDoXHrstvyavWdRnfPd4t-XV58fP8G72-vfp-_vWaelHJiUpfVi03EqVhzHDjFXeee9Woyihm6kY0mpvKCKkV4zU4lKVrZI3GqZrVWmzJ0fo35inY7MM0r_ZxGNBPtpKVquTMHK_MmOL9HvNk-5CXlW7AuM-Wa85KkGIGyxX0KeacsLVjCr1L_ywDuwi1B6F2sWWB24NQq-bch8cCl73r2jR7Cvk5LBWAEXzmvqwczkb-BEzLYJydNiEte5sY_tP0AJR8iAk</recordid><startdate>20020918</startdate><enddate>20020918</enddate><creator>Bloom, Ira</creator><creator>Jones, Scott A.</creator><creator>Polzin, Edward G.</creator><creator>Battaglia, Vincent S.</creator><creator>Henriksen, Gary L.</creator><creator>Motloch, Chester G.</creator><creator>Wright, Randy B.</creator><creator>Jungst, Rudolph G.</creator><creator>Case, Herbert L.</creator><creator>Doughty, Daniel H.</creator><general>Elsevier B.V</general><general>Elsevier Sequoia</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>8FD</scope><scope>L7M</scope><scope>OTOTI</scope></search><sort><creationdate>20020918</creationdate><title>Mechanisms of impedance rise in high-power, lithium-ion cells</title><author>Bloom, Ira ; Jones, Scott A. ; Polzin, Edward G. ; Battaglia, Vincent S. ; Henriksen, Gary L. ; Motloch, Chester G. ; Wright, Randy B. ; Jungst, Rudolph G. ; Case, Herbert L. ; Doughty, Daniel H.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c394t-4c59f284e4811828c62ac2c6d698618bd3d72898347612b0ae45ad4be8a6b1b73</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2002</creationdate><topic>Applied sciences</topic><topic>CHEMISTRY</topic><topic>Direct energy conversion and energy accumulation</topic><topic>Electrical engineering. Electrical power engineering</topic><topic>Electrical power engineering</topic><topic>Electrochemical conversion: primary and secondary batteries, fuel cells</topic><topic>ENERGY STORAGE</topic><topic>EQUIVALENT CIRCUITS</topic><topic>Exact sciences and technology</topic><topic>High-power</topic><topic>IMPEDANCE</topic><topic>LIFE CYCLE</topic><topic>Lithium-ion</topic><topic>POLARIZATION</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Bloom, Ira</creatorcontrib><creatorcontrib>Jones, Scott A.</creatorcontrib><creatorcontrib>Polzin, Edward G.</creatorcontrib><creatorcontrib>Battaglia, Vincent S.</creatorcontrib><creatorcontrib>Henriksen, Gary L.</creatorcontrib><creatorcontrib>Motloch, Chester G.</creatorcontrib><creatorcontrib>Wright, Randy B.</creatorcontrib><creatorcontrib>Jungst, Rudolph G.</creatorcontrib><creatorcontrib>Case, Herbert L.</creatorcontrib><creatorcontrib>Doughty, Daniel H.</creatorcontrib><creatorcontrib>Argonne National Lab. (ANL), Argonne, IL (United States)</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Technology Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>OSTI.GOV</collection><jtitle>Journal of power sources</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Bloom, Ira</au><au>Jones, Scott A.</au><au>Polzin, Edward G.</au><au>Battaglia, Vincent S.</au><au>Henriksen, Gary L.</au><au>Motloch, Chester G.</au><au>Wright, Randy B.</au><au>Jungst, Rudolph G.</au><au>Case, Herbert L.</au><au>Doughty, Daniel H.</au><aucorp>Argonne National Lab. (ANL), Argonne, IL (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Mechanisms of impedance rise in high-power, lithium-ion cells</atitle><jtitle>Journal of power sources</jtitle><date>2002-09-18</date><risdate>2002</risdate><volume>111</volume><issue>1</issue><spage>152</spage><epage>159</epage><pages>152-159</pages><issn>0378-7753</issn><eissn>1873-2755</eissn><coden>JPSODZ</coden><abstract>Cells were life-cycled cells using profiles with a 3, 6, or 9% change in state of charge (ΔSOC) at 40, 50, 60, and 70
°C. From the voltage response of the cells to the life-cycle profile at each temperature, we separated the overall impedance rise into two simpler terms,
R
o (ohmic) and
R
p (polarization), using an equivalent circuit model. The
R
o data tend to follow the expected trends (40>50>60>70
°C). Although the
R
p data trends show that
R
p can either decrease or increase asymptotically with time, the overall temperature-dependent behavior is similar to that of
R
o. We illustrate the types of processes that can occur in one lithium-ion cell chemistry. Based on the initial rates, the processes are complex. The
R
o term dominates the observable cell impedance, but
R
p adds a non-trivial contribution.</abstract><cop>Lausanne</cop><pub>Elsevier B.V</pub><doi>10.1016/S0378-7753(02)00302-6</doi><tpages>8</tpages></addata></record> |
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| ispartof | Journal of power sources, 2002-09, Vol.111 (1), p.152-159 |
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| recordid | cdi_osti_scitechconnect_949694 |
| source | ScienceDirect Journals (5 years ago - present) |
| subjects | Applied sciences CHEMISTRY Direct energy conversion and energy accumulation Electrical engineering. Electrical power engineering Electrical power engineering Electrochemical conversion: primary and secondary batteries, fuel cells ENERGY STORAGE EQUIVALENT CIRCUITS Exact sciences and technology High-power IMPEDANCE LIFE CYCLE Lithium-ion POLARIZATION |
| title | Mechanisms of impedance rise in high-power, lithium-ion cells |
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