Barium isotopes in individual presolar silicon carbide grains from the Murchison meteorite

Barium isotopic compositions of single 2.3–5.3 μm presolar SiC grains from the Murchison meteorite were measured by resonant ionization mass spectrometry. Mainstream SiC grains are enriched in s-process barium and show a spread in isotopic composition from solar to dominantly s-process. In the relat...

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Veröffentlicht in:Geochimica et cosmochimica acta 2003-09, Vol.67 (17), p.3201-3214
Hauptverfasser: Savina, Michael R., Davis, Andrew M., Tripa, C.Emil, Pellin, Michael J., Clayton, Robert N., Lewis, Roy S., Amari, Sachiko, Gallino, Roberto, Lugaro, Maria
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container_end_page 3214
container_issue 17
container_start_page 3201
container_title Geochimica et cosmochimica acta
container_volume 67
creator Savina, Michael R.
Davis, Andrew M.
Tripa, C.Emil
Pellin, Michael J.
Clayton, Robert N.
Lewis, Roy S.
Amari, Sachiko
Gallino, Roberto
Lugaro, Maria
description Barium isotopic compositions of single 2.3–5.3 μm presolar SiC grains from the Murchison meteorite were measured by resonant ionization mass spectrometry. Mainstream SiC grains are enriched in s-process barium and show a spread in isotopic composition from solar to dominantly s-process. In the relatively coarse grain size fraction analyzed, there are large grain-to-grain variations of barium isotopic composition. Comparison of single grain data with models of nucleosynthesis in asymptotic giant branch (AGB) stars indicates that the grains most likely come from low mass carbon-rich AGB stars (1.5 to 3 solar masses) of about solar metallicity and with approximately solar initial proportions of r- and s-process isotopes. Measurements of single grains imply a wide variety of neutron-to-seed ratios, in agreement with previous measurements of strontium, zirconium and molybdenum isotopic compositions of single presolar SiC grains.
doi_str_mv 10.1016/S0016-7037(03)00083-8
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subjects BARIUM
BARIUM ISOTOPES
CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS
GRAIN SIZE
IONIZATION
MASS SPECTROSCOPY
METEORITES
MOLYBDENUM
NUCLEOSYNTHESIS
S PROCESS
SILICON CARBIDES
STARS
STRONTIUM
ZIRCONIUM
title Barium isotopes in individual presolar silicon carbide grains from the Murchison meteorite
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