Charge order, dynamics, and magnetostructural transition in multiferroic LuFe2O4

We investigated the series of temperature and field-driven transitions in LuFe2O4 by optical and Mössbauer spectroscopies, magnetization, and x-ray scattering in order to understand the interplay between charge, structure, and magnetism in this multiferroic material. We demonstrate that charge fluct...

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Veröffentlicht in:Physical review letters 2008-11, Vol.101 (22), p.227602-227602
Hauptverfasser: Xu, X S, Angst, M, Brinzari, T V, Hermann, R P, Musfeldt, J L, Christianson, A D, Mandrus, D, Sales, B C, McGill, S, Kim, J-W, Islam, Z
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container_end_page 227602
container_issue 22
container_start_page 227602
container_title Physical review letters
container_volume 101
creator Xu, X S
Angst, M
Brinzari, T V
Hermann, R P
Musfeldt, J L
Christianson, A D
Mandrus, D
Sales, B C
McGill, S
Kim, J-W
Islam, Z
description We investigated the series of temperature and field-driven transitions in LuFe2O4 by optical and Mössbauer spectroscopies, magnetization, and x-ray scattering in order to understand the interplay between charge, structure, and magnetism in this multiferroic material. We demonstrate that charge fluctuation has an onset well below the charge ordering transition, supporting the "order by fluctuation" mechanism for the development of charge order superstructure. Bragg splitting and large magneto-optical contrast suggest a low-temperature monoclinic distortion that can be driven by both temperature and magnetic field.
doi_str_mv 10.1103/PhysRevLett.101.227602
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1079-7114
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source American Physical Society Journals
subjects CHARGE CARRIERS
IRON OXIDES
LUTETIUM OXIDES
MAGNETIC FIELDS
MAGNETIZATION
MATERIALS SCIENCE
PHASE TRANSFORMATIONS
Physical, chemical, mathematical & earth Sciences
Physics
Physique
Physique, chimie, mathématiques & sciences de la terre
PRECURSOR
TEMPERATURE DEPENDENCE
title Charge order, dynamics, and magnetostructural transition in multiferroic LuFe2O4
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