Effects of water vapor on oxidation behavior of ferritic stainless steels under solid oxide fuel cell interconnect exposure conditions
The oxidation of ferritic stainless steels has been studied under solid oxide fuel cell (SOFC) interconnect “dual” exposure conditions, i.e., simultaneous exposure to air on one side of the sample, and fuel (hydrogen) on the other. It was found that, under the dual exposures, the oxidation behavior...
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| Veröffentlicht in: | Solid state ionics 2005-05, Vol.176 (17), p.1495-1503 |
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| creator | Yang, Zhenguo Xia, Guanguang Singh, Prabhakar Stevenson, Jeffry W. |
| description | The oxidation of ferritic stainless steels has been studied under solid oxide fuel cell (SOFC) interconnect “dual” exposure conditions, i.e., simultaneous exposure to air on one side of the sample, and fuel (hydrogen) on the other. It was found that, under the dual exposures, the oxidation behavior of the stainless steels at the airside differed significantly from that observed during exposure to air at both sides. Increased water vapor partial pressure in the air at the airside further accelerated the anomalous oxidation, resulting in nucleation and growth of hematite in the scale that led to a localized attack. The accelerated oxidation and growth of the hematite nodules was a result of combined effects of hydrogen transport from the fuel side to the airside and the presence of increased water vapor. |
| doi_str_mv | 10.1016/j.ssi.2005.03.019 |
| format | Article |
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(PNNL), Richland, WA (United States)</creatorcontrib><description>The oxidation of ferritic stainless steels has been studied under solid oxide fuel cell (SOFC) interconnect “dual” exposure conditions, i.e., simultaneous exposure to air on one side of the sample, and fuel (hydrogen) on the other. It was found that, under the dual exposures, the oxidation behavior of the stainless steels at the airside differed significantly from that observed during exposure to air at both sides. Increased water vapor partial pressure in the air at the airside further accelerated the anomalous oxidation, resulting in nucleation and growth of hematite in the scale that led to a localized attack. The accelerated oxidation and growth of the hematite nodules was a result of combined effects of hydrogen transport from the fuel side to the airside and the presence of increased water vapor.</description><identifier>ISSN: 0167-2738</identifier><identifier>EISSN: 1872-7689</identifier><identifier>DOI: 10.1016/j.ssi.2005.03.019</identifier><language>eng</language><publisher>United States: Elsevier B.V</publisher><subject>08 HYDROGEN ; 30 DIRECT ENERGY CONVERSION ; AIR ; Ferritic ; Fuel Cell ; HEMATITE ; HYDROGEN ; Interconnect ; MATERIALS SCIENCE ; NUCLEATION ; OXIDATION ; PARTIAL PRESSURE ; SOFC ; Solid oxide fuel cell (SOFC) ; SOLID OXIDE FUEL CELLS ; Stainless Steel ; STAINLESS STEELS ; TRANSPORT ; WATER VAPOR</subject><ispartof>Solid state ionics, 2005-05, Vol.176 (17), p.1495-1503</ispartof><rights>2005 Elsevier B.V.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c420t-383b7718d3d8be556afff056a5f8f4f5df87e76a8a2a319e23b03c024ea3ce483</citedby></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0167273805000937$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>230,314,776,780,881,3537,27901,27902,65306</link.rule.ids><backlink>$$Uhttps://www.osti.gov/biblio/859958$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Yang, Zhenguo</creatorcontrib><creatorcontrib>Xia, Guanguang</creatorcontrib><creatorcontrib>Singh, Prabhakar</creatorcontrib><creatorcontrib>Stevenson, Jeffry W.</creatorcontrib><creatorcontrib>Pacific Northwest National Lab. (PNNL), Richland, WA (United States)</creatorcontrib><title>Effects of water vapor on oxidation behavior of ferritic stainless steels under solid oxide fuel cell interconnect exposure conditions</title><title>Solid state ionics</title><description>The oxidation of ferritic stainless steels has been studied under solid oxide fuel cell (SOFC) interconnect “dual” exposure conditions, i.e., simultaneous exposure to air on one side of the sample, and fuel (hydrogen) on the other. It was found that, under the dual exposures, the oxidation behavior of the stainless steels at the airside differed significantly from that observed during exposure to air at both sides. Increased water vapor partial pressure in the air at the airside further accelerated the anomalous oxidation, resulting in nucleation and growth of hematite in the scale that led to a localized attack. The accelerated oxidation and growth of the hematite nodules was a result of combined effects of hydrogen transport from the fuel side to the airside and the presence of increased water vapor.</description><subject>08 HYDROGEN</subject><subject>30 DIRECT ENERGY CONVERSION</subject><subject>AIR</subject><subject>Ferritic</subject><subject>Fuel Cell</subject><subject>HEMATITE</subject><subject>HYDROGEN</subject><subject>Interconnect</subject><subject>MATERIALS SCIENCE</subject><subject>NUCLEATION</subject><subject>OXIDATION</subject><subject>PARTIAL PRESSURE</subject><subject>SOFC</subject><subject>Solid oxide fuel cell (SOFC)</subject><subject>SOLID OXIDE FUEL CELLS</subject><subject>Stainless Steel</subject><subject>STAINLESS STEELS</subject><subject>TRANSPORT</subject><subject>WATER VAPOR</subject><issn>0167-2738</issn><issn>1872-7689</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2005</creationdate><recordtype>article</recordtype><recordid>eNp9kctuHCEQRVHkSBk7_gDvyCa77vDoBy2vIsuPSCNlk6wRA4XMqN1MKHri_IC_2-DxOqsqlc6tunAJueKs5YwP3_YtYmgFY33LZMv49IFsuBpFMw5qOiObwoyNGKX6RM4R94yxQaphQ15uvQebkUZP_5oMiR7NISYaFxqfgzM5lG4Hj-YY6tRTDymFHCzFbMIyA2LpAGak6-KKHOMc3JsWqF9hphbmmYalrLZxWcotCs-HiGsCWgYu1Av4mXz0Zka4fK8X5Pfd7a-bh2b78_7HzfdtYzvBciOV3I0jV046tYO-H4z3npXSe-U73zuvRhgHo4wwkk8g5I5Jy0QHRlrolLwgX057I-ag0YYM9vHdl1b9NPWV-XpiDin-WQGzfgpYX2EWiCtqMYlOMllBfgJtiogJvD6k8GTSP82ZrqnovS6p6JqKZlKXVIrm-qQpPwbHAKmagMWCC6l6cDH8R_0KEQGY_Q</recordid><startdate>20050531</startdate><enddate>20050531</enddate><creator>Yang, Zhenguo</creator><creator>Xia, Guanguang</creator><creator>Singh, Prabhakar</creator><creator>Stevenson, Jeffry W.</creator><general>Elsevier B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SE</scope><scope>7U5</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>OTOTI</scope></search><sort><creationdate>20050531</creationdate><title>Effects of water vapor on oxidation behavior of ferritic stainless steels under solid oxide fuel cell interconnect exposure conditions</title><author>Yang, Zhenguo ; Xia, Guanguang ; Singh, Prabhakar ; Stevenson, Jeffry W.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c420t-383b7718d3d8be556afff056a5f8f4f5df87e76a8a2a319e23b03c024ea3ce483</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2005</creationdate><topic>08 HYDROGEN</topic><topic>30 DIRECT ENERGY CONVERSION</topic><topic>AIR</topic><topic>Ferritic</topic><topic>Fuel Cell</topic><topic>HEMATITE</topic><topic>HYDROGEN</topic><topic>Interconnect</topic><topic>MATERIALS SCIENCE</topic><topic>NUCLEATION</topic><topic>OXIDATION</topic><topic>PARTIAL PRESSURE</topic><topic>SOFC</topic><topic>Solid oxide fuel cell (SOFC)</topic><topic>SOLID OXIDE FUEL CELLS</topic><topic>Stainless Steel</topic><topic>STAINLESS STEELS</topic><topic>TRANSPORT</topic><topic>WATER VAPOR</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yang, Zhenguo</creatorcontrib><creatorcontrib>Xia, Guanguang</creatorcontrib><creatorcontrib>Singh, Prabhakar</creatorcontrib><creatorcontrib>Stevenson, Jeffry W.</creatorcontrib><creatorcontrib>Pacific Northwest National Lab. 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Increased water vapor partial pressure in the air at the airside further accelerated the anomalous oxidation, resulting in nucleation and growth of hematite in the scale that led to a localized attack. The accelerated oxidation and growth of the hematite nodules was a result of combined effects of hydrogen transport from the fuel side to the airside and the presence of increased water vapor.</abstract><cop>United States</cop><pub>Elsevier B.V</pub><doi>10.1016/j.ssi.2005.03.019</doi><tpages>9</tpages></addata></record> |
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| ispartof | Solid state ionics, 2005-05, Vol.176 (17), p.1495-1503 |
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| language | eng |
| recordid | cdi_osti_scitechconnect_859958 |
| source | Elsevier ScienceDirect Journals |
| subjects | 08 HYDROGEN 30 DIRECT ENERGY CONVERSION AIR Ferritic Fuel Cell HEMATITE HYDROGEN Interconnect MATERIALS SCIENCE NUCLEATION OXIDATION PARTIAL PRESSURE SOFC Solid oxide fuel cell (SOFC) SOLID OXIDE FUEL CELLS Stainless Steel STAINLESS STEELS TRANSPORT WATER VAPOR |
| title | Effects of water vapor on oxidation behavior of ferritic stainless steels under solid oxide fuel cell interconnect exposure conditions |
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