Multielectron inner-shell photoexcitation in absorption spectra of Kr : theory and experiment
The probability of Kr 1[ital s] photoionization alone and accompanied by 4[ital p], 3[ital d], 3[ital p], 2[ital s], and 2[ital s]4[ital p] excitations has been calculated as a function of photon energy in the vicinity of the respective thresholds; pertinent energies have been computed including rel...
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| Veröffentlicht in: | Physical review. A, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 1993-03, Vol.47 (3), p.1953-1966 |
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| container_end_page | 1966 |
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| container_issue | 3 |
| container_start_page | 1953 |
| container_title | Physical review. A, Atomic, molecular, and optical physics |
| container_volume | 47 |
| creator | SCHAPHORST, S. J KODRE, A. F RUSCHEINSKI, J CRASEMANN, B ÅBERG, T TULKKI, J MAU HSIUNG CHEN AZUMA, Y BROWN, G. S |
| description | The probability of Kr 1[ital s] photoionization alone and accompanied by 4[ital p], 3[ital d], 3[ital p], 2[ital s], and 2[ital s]4[ital p] excitations has been calculated as a function of photon energy in the vicinity of the respective thresholds; pertinent energies have been computed including relativistic, quantum-electrodynamic, and relaxation effects. Sharp features from two-electron excitations are expected in absorption spectra only if at least one of the electrons undergoes a transition to a bound state; this becomes less probable in inner shells. An absorption-spectrometry experiment on Kr has been performed with synchrotron radiation; results generally confirm the predictions but also point toward refinements that are required in the theory and the need for improvements in techniques and synchrotron-radiation sources. |
| doi_str_mv | 10.1103/physreva.47.1953 |
| format | Article |
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J ; KODRE, A. F ; RUSCHEINSKI, J ; CRASEMANN, B ; ÅBERG, T ; TULKKI, J ; MAU HSIUNG CHEN ; AZUMA, Y ; BROWN, G. S</creator><creatorcontrib>SCHAPHORST, S. J ; KODRE, A. F ; RUSCHEINSKI, J ; CRASEMANN, B ; ÅBERG, T ; TULKKI, J ; MAU HSIUNG CHEN ; AZUMA, Y ; BROWN, G. S</creatorcontrib><description>The probability of Kr 1[ital s] photoionization alone and accompanied by 4[ital p], 3[ital d], 3[ital p], 2[ital s], and 2[ital s]4[ital p] excitations has been calculated as a function of photon energy in the vicinity of the respective thresholds; pertinent energies have been computed including relativistic, quantum-electrodynamic, and relaxation effects. Sharp features from two-electron excitations are expected in absorption spectra only if at least one of the electrons undergoes a transition to a bound state; this becomes less probable in inner shells. An absorption-spectrometry experiment on Kr has been performed with synchrotron radiation; results generally confirm the predictions but also point toward refinements that are required in the theory and the need for improvements in techniques and synchrotron-radiation sources.</description><identifier>ISSN: 1050-2947</identifier><identifier>EISSN: 1094-1622</identifier><identifier>DOI: 10.1103/physreva.47.1953</identifier><identifier>PMID: 9909149</identifier><identifier>CODEN: PLRAAN</identifier><language>eng</language><publisher>College Park, MD: American Physical Society</publisher><subject>664200 - Spectra of Atoms & Molecules & their Interactions with Photons- (1992-) ; ABSORPTION SPECTRA ; ATOMIC AND MOLECULAR PHYSICS ; Atomic properties and interactions with photons ; BOUND STATE ; BREMSSTRAHLUNG ; CROSS SECTIONS ; DATA ; ELECTRODYNAMICS ; ELECTROMAGNETIC RADIATION ; ELEMENTS ; ENERGY ; ENERGY RANGE ; ENERGY-LEVEL TRANSITIONS ; Exact sciences and technology ; EXCITATION ; EXPERIMENTAL DATA ; FIELD THEORIES ; FLUIDS ; GASES ; INFORMATION ; INNER-SHELL IONIZATION ; IONIZATION ; KRYPTON ; MANY-BODY PROBLEM ; NONMETALS ; NUMERICAL DATA ; PHOTOIONIZATION ; Photoionization of atoms and ions ; Photon interactions with atoms ; Physics ; PROBABILITY ; QUANTUM ELECTRODYNAMICS ; QUANTUM FIELD THEORY ; RADIATIONS ; RARE GASES ; RELATIVISTIC RANGE ; RELAXATION ; SPECTRA ; SYNCHROTRON RADIATION ; THEORETICAL DATA ; THRESHOLD ENERGY ; TOTAL CROSS SECTIONS ; TWO-BODY PROBLEM</subject><ispartof>Physical review. 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Sharp features from two-electron excitations are expected in absorption spectra only if at least one of the electrons undergoes a transition to a bound state; this becomes less probable in inner shells. An absorption-spectrometry experiment on Kr has been performed with synchrotron radiation; results generally confirm the predictions but also point toward refinements that are required in the theory and the need for improvements in techniques and synchrotron-radiation sources.</description><subject>664200 - Spectra of Atoms & Molecules & their Interactions with Photons- (1992-)</subject><subject>ABSORPTION SPECTRA</subject><subject>ATOMIC AND MOLECULAR PHYSICS</subject><subject>Atomic properties and interactions with photons</subject><subject>BOUND STATE</subject><subject>BREMSSTRAHLUNG</subject><subject>CROSS SECTIONS</subject><subject>DATA</subject><subject>ELECTRODYNAMICS</subject><subject>ELECTROMAGNETIC RADIATION</subject><subject>ELEMENTS</subject><subject>ENERGY</subject><subject>ENERGY RANGE</subject><subject>ENERGY-LEVEL TRANSITIONS</subject><subject>Exact sciences and technology</subject><subject>EXCITATION</subject><subject>EXPERIMENTAL DATA</subject><subject>FIELD THEORIES</subject><subject>FLUIDS</subject><subject>GASES</subject><subject>INFORMATION</subject><subject>INNER-SHELL IONIZATION</subject><subject>IONIZATION</subject><subject>KRYPTON</subject><subject>MANY-BODY PROBLEM</subject><subject>NONMETALS</subject><subject>NUMERICAL DATA</subject><subject>PHOTOIONIZATION</subject><subject>Photoionization of atoms and ions</subject><subject>Photon interactions with atoms</subject><subject>Physics</subject><subject>PROBABILITY</subject><subject>QUANTUM ELECTRODYNAMICS</subject><subject>QUANTUM FIELD THEORY</subject><subject>RADIATIONS</subject><subject>RARE GASES</subject><subject>RELATIVISTIC RANGE</subject><subject>RELAXATION</subject><subject>SPECTRA</subject><subject>SYNCHROTRON RADIATION</subject><subject>THEORETICAL DATA</subject><subject>THRESHOLD ENERGY</subject><subject>TOTAL CROSS SECTIONS</subject><subject>TWO-BODY PROBLEM</subject><issn>1050-2947</issn><issn>1094-1622</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>1993</creationdate><recordtype>article</recordtype><recordid>eNo9kEtLxDAUhYMovvduhCAu3HRMmqRp3In4QkURXUpI01ta6TQ1yYjz702dwWyScM653PMhdETJjFLCzsd2GTx8mxmXM6oE20C7lCie0SLPN6e3IFmuuNxBeyF8knR4qbbRtlJEUa520cfToo8d9GCjdwPuhgF8Flroezy2Ljr4sV00sfvTsKmC8-PfL4xTxGDX4AePL3BswfklNkON4WcE381hiAdoqzF9gMP1vY_eb67fru6yx-fb-6vLx8zyQsQsBymLsqIgKZRQMyNqaFReqyqXUBCQ3NqmKkVNStUwWQirLGs4yLzmnJGS7aOT1VwXYqdDWhlsa10qY6MuFKeiUMl0tjKN3n0tIEQ974JNTc0AbhE0LYWiZeIyWcnKar0LCXCjx1TI-KWmRE_g9UsC_wrfl5pLPYFPkeP19EU1h_o_sCad9NO1boI1fePNYLvwb-NECCkZ-wXlxI5F</recordid><startdate>19930301</startdate><enddate>19930301</enddate><creator>SCHAPHORST, S. 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S</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Multielectron inner-shell photoexcitation in absorption spectra of Kr : theory and experiment</atitle><jtitle>Physical review. A, Atomic, molecular, and optical physics</jtitle><addtitle>Phys Rev A</addtitle><date>1993-03-01</date><risdate>1993</risdate><volume>47</volume><issue>3</issue><spage>1953</spage><epage>1966</epage><pages>1953-1966</pages><issn>1050-2947</issn><eissn>1094-1622</eissn><coden>PLRAAN</coden><abstract>The probability of Kr 1[ital s] photoionization alone and accompanied by 4[ital p], 3[ital d], 3[ital p], 2[ital s], and 2[ital s]4[ital p] excitations has been calculated as a function of photon energy in the vicinity of the respective thresholds; pertinent energies have been computed including relativistic, quantum-electrodynamic, and relaxation effects. Sharp features from two-electron excitations are expected in absorption spectra only if at least one of the electrons undergoes a transition to a bound state; this becomes less probable in inner shells. An absorption-spectrometry experiment on Kr has been performed with synchrotron radiation; results generally confirm the predictions but also point toward refinements that are required in the theory and the need for improvements in techniques and synchrotron-radiation sources.</abstract><cop>College Park, MD</cop><pub>American Physical Society</pub><pmid>9909149</pmid><doi>10.1103/physreva.47.1953</doi><tpages>14</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1050-2947 |
| ispartof | Physical review. A, Atomic, molecular, and optical physics, 1993-03, Vol.47 (3), p.1953-1966 |
| issn | 1050-2947 1094-1622 |
| language | eng |
| recordid | cdi_osti_scitechconnect_6941569 |
| source | American Physical Society Journals |
| subjects | 664200 - Spectra of Atoms & Molecules & their Interactions with Photons- (1992-) ABSORPTION SPECTRA ATOMIC AND MOLECULAR PHYSICS Atomic properties and interactions with photons BOUND STATE BREMSSTRAHLUNG CROSS SECTIONS DATA ELECTRODYNAMICS ELECTROMAGNETIC RADIATION ELEMENTS ENERGY ENERGY RANGE ENERGY-LEVEL TRANSITIONS Exact sciences and technology EXCITATION EXPERIMENTAL DATA FIELD THEORIES FLUIDS GASES INFORMATION INNER-SHELL IONIZATION IONIZATION KRYPTON MANY-BODY PROBLEM NONMETALS NUMERICAL DATA PHOTOIONIZATION Photoionization of atoms and ions Photon interactions with atoms Physics PROBABILITY QUANTUM ELECTRODYNAMICS QUANTUM FIELD THEORY RADIATIONS RARE GASES RELATIVISTIC RANGE RELAXATION SPECTRA SYNCHROTRON RADIATION THEORETICAL DATA THRESHOLD ENERGY TOTAL CROSS SECTIONS TWO-BODY PROBLEM |
| title | Multielectron inner-shell photoexcitation in absorption spectra of Kr : theory and experiment |
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