stratospheric trace gas concentrations in the Arctic polar night derived by FTIR-spectroscopy with the Moon as IR light source

In winter 1992/93 we have performed ground‐based FTIR measurements in the Arctic (79°N, 12°E) to derive column densities of stratospheric trace gases within the polar vortex. Due to the polar night the moon had to serve as infrared light source instead of the sun. It was possible to perform FTIR‐mea...

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Veröffentlicht in:Geophysical research letters 1993-10, Vol.20 (19), p.2059-2062
Hauptverfasser: Notholt, J., Neuber, R., Schrems, O., Clarmann, T. V.
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container_title Geophysical research letters
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creator Notholt, J.
Neuber, R.
Schrems, O.
Clarmann, T. V.
description In winter 1992/93 we have performed ground‐based FTIR measurements in the Arctic (79°N, 12°E) to derive column densities of stratospheric trace gases within the polar vortex. Due to the polar night the moon had to serve as infrared light source instead of the sun. It was possible to perform FTIR‐measurements for about a week around full moon. Column densities of N2O, CH4, HF, HCl, O3, NO2, HNO3 and ClONO2 have been obtained. The spectra were recorded at 0.01 cm−1 or 0.02 cm−1 resolution using MCT or InSb detectors. Measurements with an aerosol lidar performed at the same site show that polar stratospheric clouds (PSCs) appeared several times during the polar night. It seems that the concentrations of the stratospheric trace gases are strongly influenced by the occurrence of PSCs.
doi_str_mv 10.1029/93GL01971
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V.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>stratospheric trace gas concentrations in the Arctic polar night derived by FTIR-spectroscopy with the Moon as IR light source</atitle><jtitle>Geophysical research letters</jtitle><addtitle>Geophys. Res. Lett</addtitle><date>1993-10-08</date><risdate>1993</risdate><volume>20</volume><issue>19</issue><spage>2059</spage><epage>2062</epage><pages>2059-2062</pages><issn>0094-8276</issn><eissn>1944-8007</eissn><coden>GPRLAJ</coden><abstract>In winter 1992/93 we have performed ground‐based FTIR measurements in the Arctic (79°N, 12°E) to derive column densities of stratospheric trace gases within the polar vortex. Due to the polar night the moon had to serve as infrared light source instead of the sun. It was possible to perform FTIR‐measurements for about a week around full moon. Column densities of N2O, CH4, HF, HCl, O3, NO2, HNO3 and ClONO2 have been obtained. The spectra were recorded at 0.01 cm−1 or 0.02 cm−1 resolution using MCT or InSb detectors. Measurements with an aerosol lidar performed at the same site show that polar stratospheric clouds (PSCs) appeared several times during the polar night. It seems that the concentrations of the stratospheric trace gases are strongly influenced by the occurrence of PSCs.</abstract><cop>Washington, DC</cop><pub>Blackwell Publishing Ltd</pub><doi>10.1029/93GL01971</doi><tpages>4</tpages></addata></record>
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identifier ISSN: 0094-8276
ispartof Geophysical research letters, 1993-10, Vol.20 (19), p.2059-2062
issn 0094-8276
1944-8007
language eng
recordid cdi_osti_scitechconnect_5370218
source Wiley Online Library Journals Frontfile Complete
subjects ALKANES
Atmospheric composition. Chemical and photochemical reactions
CHALCOGENIDES
CHLORINE COMPOUNDS
CLOUDS
Density
EARTH ATMOSPHERE
Earth, ocean, space
ECOLOGICAL CONCENTRATION
ENVIRONMENTAL SCIENCES
Exact sciences and technology
External geophysics
FLUORINE COMPOUNDS
HALOGEN COMPOUNDS
HYDROCARBONS
HYDROCHLORIC ACID
HYDROFLUORIC ACID
HYDROGEN COMPOUNDS
Indium antimonides
INORGANIC ACIDS
Light sources
METHANE
Moon
Night
NITRIC ACID
NITROGEN COMPOUNDS
NITROGEN OXIDES
Nitrous oxides
ORGANIC COMPOUNDS
OXIDES
OXYGEN COMPOUNDS 540120 -- Environment, Atmospheric-- Chemicals Monitoring & Transport-- (1990-)
OZONE
Physics of the high neutral atmosphere
STRATOSPHERE
Trace gases
title stratospheric trace gas concentrations in the Arctic polar night derived by FTIR-spectroscopy with the Moon as IR light source
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