X-ray induced grain boundary formation and grain rotation in Bi2Se3

Optimizing grain boundary characteristics in polycrystalline materials can improve their properties. Many processing methods have been developed for grain boundary manipulation, including the use of intense radiation in certain applications. In this work, we used X-ray free electron laser pulses to...

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Veröffentlicht in:Scripta materialia 2025-02, Vol.256 (C), p.116416, Article 116416
Hauptverfasser: Katagiri, Kento, Kozioziemski, Bernard, Folsom, Eric, Göde, Sebastian, Wang, Yifan, Appel, Karen, Chalise, Darshan, Cook, Philip K., Eggert, Jon, Howard, Marylesa, Kim, Sungwon, Konôpková, Zuzana, Makita, Mikako, Nakatsutsumi, Motoaki, Nielsen, Martin M., Pelka, Alexander, Poulsen, Henning F., Preston, Thomas R., Reddy, Tharun, Schwinkendorf, Jan-Patrick, Seiboth, Frank, Simons, Hugh, Wang, Bihan, Yang, Wenge, Zastrau, Ulf, Kim, Hyunjung, Dresselhaus-Marais, Leora E.
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container_issue C
container_start_page 116416
container_title Scripta materialia
container_volume 256
creator Katagiri, Kento
Kozioziemski, Bernard
Folsom, Eric
Göde, Sebastian
Wang, Yifan
Appel, Karen
Chalise, Darshan
Cook, Philip K.
Eggert, Jon
Howard, Marylesa
Kim, Sungwon
Konôpková, Zuzana
Makita, Mikako
Nakatsutsumi, Motoaki
Nielsen, Martin M.
Pelka, Alexander
Poulsen, Henning F.
Preston, Thomas R.
Reddy, Tharun
Schwinkendorf, Jan-Patrick
Seiboth, Frank
Simons, Hugh
Wang, Bihan
Yang, Wenge
Zastrau, Ulf
Kim, Hyunjung
Dresselhaus-Marais, Leora E.
description Optimizing grain boundary characteristics in polycrystalline materials can improve their properties. Many processing methods have been developed for grain boundary manipulation, including the use of intense radiation in certain applications. In this work, we used X-ray free electron laser pulses to irradiate single-crystalline bismuth selenide (Bi2Se3) and observed grain boundary formation and subsequent grain rotation in response to the X-ray radiation. Our observations with simultaneous transmission X-ray microscopy and X-ray diffraction demonstrate how intense X-ray radiation can rapidly change size and texture of grains. [Display omitted]
doi_str_mv 10.1016/j.scriptamat.2024.116416
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subjects Bismuth selenide (Bi2Se3)
Dislocation dynamics
Grain boundary engineering
Thermoelectric materials
title X-ray induced grain boundary formation and grain rotation in Bi2Se3
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