Ultrafast nuclear dynamics in double-core-ionized water molecules
Double-core-hole (DCH) states in isolated-water and heavy-water molecules, resulting from the sequential absorption of two x-ray photons, have been investigated. A comparison of the subsequent Auger emission spectra from the two isotopes provides direct evidence of ultrafast nuclear motion during th...
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| Veröffentlicht in: | Physical review. A 2024-07, Vol.110 (1), Article 013108 |
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| creator | Ismail, Iyas Inhester, Ludger Marchenko, Tatiana Trinter, Florian Verma, Abhishek De Fanis, Alberto Ferté, Anthony Rivas, Daniel E. Peng, Dawei Koulentianos, Dimitris Kukk, Edwin Penent, Francis Doumy, Gilles Sansone, Giuseppe Bozek, John D. Li, Kai Young, Linda Ilchen, Markus Piancastelli, Maria Novella Meyer, Michael Velasquez, Nicolas Travnikova, Oksana Boll, Rebecca Guillemin, Renaud Dörner, Reinhard Taïeb, Richard Dold, Simon Carniato, Stéphane Baumann, Thomas M. Mazza, Tommaso Ovcharenko, Yevheniy Püttner, Ralph Simon, Marc |
| description | Double-core-hole (DCH) states in isolated-water and heavy-water molecules, resulting from the sequential absorption of two x-ray photons, have been investigated. A comparison of the subsequent Auger emission spectra from the two isotopes provides direct evidence of ultrafast nuclear motion during the 1.5-fs lifetime of these DCH states. Our numerical results align well with the experimental data, providing for various DCH states an in-depth study of the dynamics responsible of the observed isotope effect. |
| doi_str_mv | 10.1103/PhysRevA.110.013108 |
| format | Article |
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| subjects | ATOMIC AND MOLECULAR PHYSICS Chemical Sciences Physics |
| title | Ultrafast nuclear dynamics in double-core-ionized water molecules |
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