Multidimensional Coherent Spectroscopy of Molecular Polaritons: Langevin Approach

We present a microscopic theory for nonlinear optical spectroscopy of N molecules in an optical cavity. Using the Heisenberg-Langevin equation, an analytical expression is derived for the time- and frequency-resolved signals accounting for arbitrary numbers of vibrational excitations. We identify cl...

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Veröffentlicht in:	Physical review letters 2023-03, Vol.130 (10), p.103001-103001, Article 103001
Hauptverfasser:	Zhang, Zhedong, Nie, Xiaoyu, Lei, Dangyuan, Mukamel, Shaul
Format:	Artikel
Sprache:	eng
Schlagworte:	ATOMIC AND MOLECULAR PHYSICS Atoms, ions, & molecules in cavities Chemical physics & physical chemistry light-matter interaction Molecules Organic microcavities Physics Polaritons
Online-Zugang:	Volltext
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