Atomically Local Electric Field Induced Interface Water Reorientation for Alkaline Hydrogen Evolution Reaction

The slow water dissociation process in alkaline electrolyte severely limits the kinetics of HER. The orientation of H2O is well known to affect the dissociation process, but H2O orientation is hard to control because of its random distribution. Herein, an atomically asymmetric local electric field w...

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Veröffentlicht in:	Angewandte Chemie International Edition 2023-06, Vol.62 (26), p.e202300873-n/a
Hauptverfasser:	Cai, Chao, Liu, Kang, Zhang, Long, Li, Fangbiao, Tan, Yao, Li, Pengcheng, Wang, Yanqiu, Wang, Maoyu, Feng, Zhenxing, Motta Meira, Debora, Qu, Wenqiang, Stefancu, Andrei, Li, Wenzhang, Li, Hongmei, Fu, Junwei, Wang, Hui, Zhang, Dengsong, Cortés, Emiliano, Liu, Min
Format:	Artikel
Sprache:	eng
Schlagworte:	Adsorption Alkaline HER Atomic Charge Distribution Electric fields Hydrogen bonds Hydrogen evolution reactions INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY Interfacial Water Orientation Molecular dynamics Orientation Raman spectroscopy Single-Atom Site Water Dissociation
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