Radiolytic evaluation of a new technetium redox control reagent for advanced used nuclear fuel separations

Technetium is a problematic radioisotope for used nuclear fuel (UNF) and subsequent waste management owing to its high environmental mobility and coextraction in reprocessing technologies as the pertechnetate anion (TcO 4 − ). Consequently, several strategies are under development to control the tra...

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Veröffentlicht in:	Physical chemistry chemical physics : PCCP 2024-01, Vol.26 (5), p.439-446
Hauptverfasser:	Dang, Anh N, Rogalski, Maya H, Pilgrim, Corey D, Wilbanks, Joseph R, Peterman, Dean R, Carrie, Jesse D, Zalupski, Peter R, Mezyk, Stephen P, Horne, Gregory P
Format:	Artikel
Sprache:	eng
Schlagworte:	Degradation Dodecane Gamma irradiation Hydrogen atoms Nitrates Nitric acid Nitrous acid Nuclear fuels Oxidation Radiation Radiation chemistry Radicals Radioisotopes Radiolysis Reaction kinetics Reagents Reducing agents Reprocessing Solvents Spent nuclear fuels Steady state Technetium Waste management
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