Fabrication of In2O3/TiO2 nanotube arrays hybrids with homogeneously developed nanostructure for photocatalytic degradation of Rhodamine B
[Display omitted] •A new class of plate-like In2O3/TNAs photocatalyst is successfully fabricated.•The obtained In2O3/TNAs hybrid presents a well-aligned nanotubular structure.•In2O3 particles are dispersed homogeneously on TNAs without blocking the nozzles.•In2O3/TNAs hybrid shows a much enhanced Rh...
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Veröffentlicht in: | Materials research bulletin 2018-10, Vol.106, p.197-203 |
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creator | Xiao, Changren Tan, Zijun Wang, Cong Yang, Xiaoqing Zhang, Guoqing Pan, Huageng |
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•A new class of plate-like In2O3/TNAs photocatalyst is successfully fabricated.•The obtained In2O3/TNAs hybrid presents a well-aligned nanotubular structure.•In2O3 particles are dispersed homogeneously on TNAs without blocking the nozzles.•In2O3/TNAs hybrid shows a much enhanced Rhodamine B degradation efficiency.•In2O3/TNAs hybrid demonstrates an excellent recycling capability.
To enhance the photocatalytic recycling capability of the TiO2-based photocatalysts, a new kind of plate-like In2O3/TiO2 nanotube array (TNA) hybrids is fabricated herein by constructing TNAs via an anodization method followed by doping In2O3 via a solvothermal method. The obtained In2O3/TNA hybrid demonstrates a well-aligned nanotubular structure with homogeneous dispersion of In2O3 nanoparticles. It shows a much higher degradation rate of 77% after 2 h compared to TNA (37%). In addition, the plate-like feature endows the photocatalysts with an excellent recycling capability. These superior photocatalytic degradation performances can be ascribed to the following factors: (1) the enhanced light absorption ability and efficient separation of photoexcited electron-hole pairs derived from the formation of the heterostructure between the interface of TiO2 and In2O3; (2) the efficient transport of reactant molecules provided by the well-defined TNAs and the homogeneous distribution of the In2O3 nanoparticles without blocking the nanotubes. |
doi_str_mv | 10.1016/j.materresbull.2018.05.022 |
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•A new class of plate-like In2O3/TNAs photocatalyst is successfully fabricated.•The obtained In2O3/TNAs hybrid presents a well-aligned nanotubular structure.•In2O3 particles are dispersed homogeneously on TNAs without blocking the nozzles.•In2O3/TNAs hybrid shows a much enhanced Rhodamine B degradation efficiency.•In2O3/TNAs hybrid demonstrates an excellent recycling capability.
To enhance the photocatalytic recycling capability of the TiO2-based photocatalysts, a new kind of plate-like In2O3/TiO2 nanotube array (TNA) hybrids is fabricated herein by constructing TNAs via an anodization method followed by doping In2O3 via a solvothermal method. The obtained In2O3/TNA hybrid demonstrates a well-aligned nanotubular structure with homogeneous dispersion of In2O3 nanoparticles. It shows a much higher degradation rate of 77% after 2 h compared to TNA (37%). In addition, the plate-like feature endows the photocatalysts with an excellent recycling capability. These superior photocatalytic degradation performances can be ascribed to the following factors: (1) the enhanced light absorption ability and efficient separation of photoexcited electron-hole pairs derived from the formation of the heterostructure between the interface of TiO2 and In2O3; (2) the efficient transport of reactant molecules provided by the well-defined TNAs and the homogeneous distribution of the In2O3 nanoparticles without blocking the nanotubes.</description><identifier>ISSN: 0025-5408</identifier><identifier>EISSN: 1873-4227</identifier><identifier>DOI: 10.1016/j.materresbull.2018.05.022</identifier><language>eng</language><publisher>United States: Elsevier Ltd</publisher><subject>ABSORPTION ; ANODIZATION ; ELECTRON-HOLE COUPLING ; FABRICATION ; Heterostructure ; In2O3 ; INDIUM OXIDES ; NANOPARTICLES ; NANOSCIENCE AND NANOTECHNOLOGY ; NANOTUBES ; PHOTOCATALYSIS ; Photocatalyst ; RECYCLING ; Rhodamine B ; RHODAMINES ; TiO2 nanotube arrays ; TITANIUM OXIDES ; VISIBLE RADIATION</subject><ispartof>Materials research bulletin, 2018-10, Vol.106, p.197-203</ispartof><rights>2018 Elsevier Ltd</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.materresbull.2018.05.022$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>230,314,780,784,885,3548,27923,27924,45994</link.rule.ids><backlink>$$Uhttps://www.osti.gov/biblio/22805212$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Xiao, Changren</creatorcontrib><creatorcontrib>Tan, Zijun</creatorcontrib><creatorcontrib>Wang, Cong</creatorcontrib><creatorcontrib>Yang, Xiaoqing</creatorcontrib><creatorcontrib>Zhang, Guoqing</creatorcontrib><creatorcontrib>Pan, Huageng</creatorcontrib><title>Fabrication of In2O3/TiO2 nanotube arrays hybrids with homogeneously developed nanostructure for photocatalytic degradation of Rhodamine B</title><title>Materials research bulletin</title><description>[Display omitted]
•A new class of plate-like In2O3/TNAs photocatalyst is successfully fabricated.•The obtained In2O3/TNAs hybrid presents a well-aligned nanotubular structure.•In2O3 particles are dispersed homogeneously on TNAs without blocking the nozzles.•In2O3/TNAs hybrid shows a much enhanced Rhodamine B degradation efficiency.•In2O3/TNAs hybrid demonstrates an excellent recycling capability.
To enhance the photocatalytic recycling capability of the TiO2-based photocatalysts, a new kind of plate-like In2O3/TiO2 nanotube array (TNA) hybrids is fabricated herein by constructing TNAs via an anodization method followed by doping In2O3 via a solvothermal method. The obtained In2O3/TNA hybrid demonstrates a well-aligned nanotubular structure with homogeneous dispersion of In2O3 nanoparticles. It shows a much higher degradation rate of 77% after 2 h compared to TNA (37%). In addition, the plate-like feature endows the photocatalysts with an excellent recycling capability. These superior photocatalytic degradation performances can be ascribed to the following factors: (1) the enhanced light absorption ability and efficient separation of photoexcited electron-hole pairs derived from the formation of the heterostructure between the interface of TiO2 and In2O3; (2) the efficient transport of reactant molecules provided by the well-defined TNAs and the homogeneous distribution of the In2O3 nanoparticles without blocking the nanotubes.</description><subject>ABSORPTION</subject><subject>ANODIZATION</subject><subject>ELECTRON-HOLE COUPLING</subject><subject>FABRICATION</subject><subject>Heterostructure</subject><subject>In2O3</subject><subject>INDIUM OXIDES</subject><subject>NANOPARTICLES</subject><subject>NANOSCIENCE AND NANOTECHNOLOGY</subject><subject>NANOTUBES</subject><subject>PHOTOCATALYSIS</subject><subject>Photocatalyst</subject><subject>RECYCLING</subject><subject>Rhodamine B</subject><subject>RHODAMINES</subject><subject>TiO2 nanotube arrays</subject><subject>TITANIUM OXIDES</subject><subject>VISIBLE RADIATION</subject><issn>0025-5408</issn><issn>1873-4227</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNpNkctOwzAQRS0EEuXxDxask47tunGXvApISJVQWVuOMyGuUhvZDqi_wFeTAkKsZnNm7h0dQi4YlAzYfLoptyZjjJjqoe9LDkyVIEvg_IBMmKpEMeO8OiQTAC4LOQN1TE5S2gDATFXVhHwuTR2dNdkFT0NLHz1fienarTj1xoc81EhNjGaXaLcbySbRD5c72oVteEWPYUj9jjb4jn14w-Z7KeU42DxEpG2I9K0LOYwBpt9lZ0f0NZrmL--5C43ZOo_0-owctaZPeP47T8nL8m5981A8re4fb66eCuSK5WJhzKKVCioEJmpVtYrjQlQLA_O5tU1rDWNSyErMlWA18PFzJpWUYI2wAlpxSi5_7o5FnU7WZbSdDd6jzZpzBZIzPlK3PxSOVd4dxj2J3mLj4h5sgtMM9N6C3uj_FvTeggapRwviCwC8gs8</recordid><startdate>20181001</startdate><enddate>20181001</enddate><creator>Xiao, Changren</creator><creator>Tan, Zijun</creator><creator>Wang, Cong</creator><creator>Yang, Xiaoqing</creator><creator>Zhang, Guoqing</creator><creator>Pan, Huageng</creator><general>Elsevier Ltd</general><scope>OTOTI</scope></search><sort><creationdate>20181001</creationdate><title>Fabrication of In2O3/TiO2 nanotube arrays hybrids with homogeneously developed nanostructure for photocatalytic degradation of Rhodamine B</title><author>Xiao, Changren ; Tan, Zijun ; Wang, Cong ; Yang, Xiaoqing ; Zhang, Guoqing ; Pan, Huageng</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-e281t-9aa9f5807e013b87f82e9379a066ccdfca11535736831b02002158550ca3c30f3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>ABSORPTION</topic><topic>ANODIZATION</topic><topic>ELECTRON-HOLE COUPLING</topic><topic>FABRICATION</topic><topic>Heterostructure</topic><topic>In2O3</topic><topic>INDIUM OXIDES</topic><topic>NANOPARTICLES</topic><topic>NANOSCIENCE AND NANOTECHNOLOGY</topic><topic>NANOTUBES</topic><topic>PHOTOCATALYSIS</topic><topic>Photocatalyst</topic><topic>RECYCLING</topic><topic>Rhodamine B</topic><topic>RHODAMINES</topic><topic>TiO2 nanotube arrays</topic><topic>TITANIUM OXIDES</topic><topic>VISIBLE RADIATION</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Xiao, Changren</creatorcontrib><creatorcontrib>Tan, Zijun</creatorcontrib><creatorcontrib>Wang, Cong</creatorcontrib><creatorcontrib>Yang, Xiaoqing</creatorcontrib><creatorcontrib>Zhang, Guoqing</creatorcontrib><creatorcontrib>Pan, Huageng</creatorcontrib><collection>OSTI.GOV</collection><jtitle>Materials research bulletin</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Xiao, Changren</au><au>Tan, Zijun</au><au>Wang, Cong</au><au>Yang, Xiaoqing</au><au>Zhang, Guoqing</au><au>Pan, Huageng</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Fabrication of In2O3/TiO2 nanotube arrays hybrids with homogeneously developed nanostructure for photocatalytic degradation of Rhodamine B</atitle><jtitle>Materials research bulletin</jtitle><date>2018-10-01</date><risdate>2018</risdate><volume>106</volume><spage>197</spage><epage>203</epage><pages>197-203</pages><issn>0025-5408</issn><eissn>1873-4227</eissn><abstract>[Display omitted]
•A new class of plate-like In2O3/TNAs photocatalyst is successfully fabricated.•The obtained In2O3/TNAs hybrid presents a well-aligned nanotubular structure.•In2O3 particles are dispersed homogeneously on TNAs without blocking the nozzles.•In2O3/TNAs hybrid shows a much enhanced Rhodamine B degradation efficiency.•In2O3/TNAs hybrid demonstrates an excellent recycling capability.
To enhance the photocatalytic recycling capability of the TiO2-based photocatalysts, a new kind of plate-like In2O3/TiO2 nanotube array (TNA) hybrids is fabricated herein by constructing TNAs via an anodization method followed by doping In2O3 via a solvothermal method. The obtained In2O3/TNA hybrid demonstrates a well-aligned nanotubular structure with homogeneous dispersion of In2O3 nanoparticles. It shows a much higher degradation rate of 77% after 2 h compared to TNA (37%). In addition, the plate-like feature endows the photocatalysts with an excellent recycling capability. These superior photocatalytic degradation performances can be ascribed to the following factors: (1) the enhanced light absorption ability and efficient separation of photoexcited electron-hole pairs derived from the formation of the heterostructure between the interface of TiO2 and In2O3; (2) the efficient transport of reactant molecules provided by the well-defined TNAs and the homogeneous distribution of the In2O3 nanoparticles without blocking the nanotubes.</abstract><cop>United States</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.materresbull.2018.05.022</doi><tpages>7</tpages></addata></record> |
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subjects | ABSORPTION ANODIZATION ELECTRON-HOLE COUPLING FABRICATION Heterostructure In2O3 INDIUM OXIDES NANOPARTICLES NANOSCIENCE AND NANOTECHNOLOGY NANOTUBES PHOTOCATALYSIS Photocatalyst RECYCLING Rhodamine B RHODAMINES TiO2 nanotube arrays TITANIUM OXIDES VISIBLE RADIATION |
title | Fabrication of In2O3/TiO2 nanotube arrays hybrids with homogeneously developed nanostructure for photocatalytic degradation of Rhodamine B |
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