{sup 75}As NMR and XRD Study of Structural and Electronic Inhomogeneities in Ba(Fe{sub 1−x}Ni{sub x}){sub 2}As{sub 2}

We have used {sup 75}As NMR and x-ray diffraction analysis to study the structural and electronic inhomogeneities in Ba(Fe{sub 1−x}Ni{sub x}){sub 2}As{sub 2} crystals with x near the border of the antiferromagnetic domain. Unequal nickel population of the equivalent Fe planes and rather homogeneous...

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Veröffentlicht in:Journal of superconductivity and novel magnetism 2018-10, Vol.31 (10)
Hauptverfasser: Nikolaev, E. G., Lugansky, L. B., Vlasenko, V. A., Pervakov, K. S., Martovitsky, V. P., Eltsev, Yu. F., Bud’ko, S. L., Canfield, P. C.
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container_issue 10
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container_title Journal of superconductivity and novel magnetism
container_volume 31
creator Nikolaev, E. G.
Lugansky, L. B.
Vlasenko, V. A.
Pervakov, K. S.
Martovitsky, V. P.
Eltsev, Yu. F.
Bud’ko, S. L.
Canfield, P. C.
description We have used {sup 75}As NMR and x-ray diffraction analysis to study the structural and electronic inhomogeneities in Ba(Fe{sub 1−x}Ni{sub x}){sub 2}As{sub 2} crystals with x near the border of the antiferromagnetic domain. Unequal nickel population of the equivalent Fe planes and rather homogeneous distribution of Ni inside the planes have been found in the well-ordered single crystal with x = 0.036. Below 40 K a signal wipeout of {sup 75}As NMR spectra is observed for the crystals with x = 0.036 and 0.037. This fact together with spin-lattice relaxation peculiarities is treated a result of the system glassy behavior in this region of the phase diagram. The {sup 75}As NMR data also indicate on partial suppression of antiferromagnetic spin fluctuations around the Ni impurity in these crystals at low temperatures.
doi_str_mv 10.1007/S10948-018-4587-X
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subjects ANTIFERROMAGNETISM
ARSENIC 75
ARSENIDES
BARIUM COMPLEXES
CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
IMPURITIES
IRON
MONOCRYSTALS
NICKEL
NUCLEAR MAGNETIC RESONANCE
PHASE DIAGRAMS
SPIN-LATTICE RELAXATION
TEMPERATURE RANGE 0065-0273 K
X-RAY DIFFRACTION
title {sup 75}As NMR and XRD Study of Structural and Electronic Inhomogeneities in Ba(Fe{sub 1−x}Ni{sub x}){sub 2}As{sub 2}
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