The origin of 2.7 eV blue luminescence band in zirconium oxide
The luminescence spectra of non-stoichiometric zirconium oxide film series with different oxygen vacancies' concentrations show the blue photoluminescence band centered near a 2.7 eV peak. There is a broad band at 5.2 eV in the luminescence excitation spectrum for blue emission. The ab-initio q...
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| Veröffentlicht in: | Journal of applied physics 2014-12, Vol.116 (24) |
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| container_title | Journal of applied physics |
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| creator | Perevalov, T. V. Gulyaev, D. V. Aliev, V. S. Zhuravlev, K. S. Gritsenko, V. A. Yelisseyev, A. P. |
| description | The luminescence spectra of non-stoichiometric zirconium oxide film series with different oxygen vacancies' concentrations show the blue photoluminescence band centered near a 2.7 eV peak. There is a broad band at 5.2 eV in the luminescence excitation spectrum for blue emission. The ab-initio quantum-chemical calculation gives a peak in the optical absorption at 5.1 eV for the oxygen vacancy in cubic ZrO2. It was concluded that the 2.7 eV blue luminescence excited near 5.2 eV in a zirconium oxide film is associated with the oxygen vacancy. |
| doi_str_mv | 10.1063/1.4905105 |
| format | Article |
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V. ; Gulyaev, D. V. ; Aliev, V. S. ; Zhuravlev, K. S. ; Gritsenko, V. A. ; Yelisseyev, A. P.</creator><creatorcontrib>Perevalov, T. V. ; Gulyaev, D. V. ; Aliev, V. S. ; Zhuravlev, K. S. ; Gritsenko, V. A. ; Yelisseyev, A. P.</creatorcontrib><description>The luminescence spectra of non-stoichiometric zirconium oxide film series with different oxygen vacancies' concentrations show the blue photoluminescence band centered near a 2.7 eV peak. There is a broad band at 5.2 eV in the luminescence excitation spectrum for blue emission. The ab-initio quantum-chemical calculation gives a peak in the optical absorption at 5.1 eV for the oxygen vacancy in cubic ZrO2. It was concluded that the 2.7 eV blue luminescence excited near 5.2 eV in a zirconium oxide film is associated with the oxygen vacancy.</description><identifier>ISSN: 0021-8979</identifier><identifier>EISSN: 1089-7550</identifier><identifier>DOI: 10.1063/1.4905105</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>ABSORPTION SPECTRA ; Applied physics ; CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS ; CONCENTRATION RATIO ; CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY ; CUBIC LATTICES ; EMISSION SPECTRA ; EV RANGE ; EXCITATION ; Excitation spectra ; Luminescence ; Organic chemistry ; Oxide coatings ; OXYGEN ; PHOTOLUMINESCENCE ; Quantum chemistry ; THIN FILMS ; VACANCIES ; Zirconium ; Zirconium dioxide ; ZIRCONIUM OXIDES</subject><ispartof>Journal of applied physics, 2014-12, Vol.116 (24)</ispartof><rights>2014 AIP Publishing LLC.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c285t-1b632829ccbb2c9b5a60393a8d93a95811784afbc71c82dd3593725c84770ce43</citedby><cites>FETCH-LOGICAL-c285t-1b632829ccbb2c9b5a60393a8d93a95811784afbc71c82dd3593725c84770ce43</cites><orcidid>0000-0002-3171-5098 ; 0000-0002-4266-971X</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,780,784,885,27924,27925</link.rule.ids><backlink>$$Uhttps://www.osti.gov/biblio/22399167$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Perevalov, T. 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P.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>The origin of 2.7 eV blue luminescence band in zirconium oxide</atitle><jtitle>Journal of applied physics</jtitle><date>2014-12-28</date><risdate>2014</risdate><volume>116</volume><issue>24</issue><issn>0021-8979</issn><eissn>1089-7550</eissn><abstract>The luminescence spectra of non-stoichiometric zirconium oxide film series with different oxygen vacancies' concentrations show the blue photoluminescence band centered near a 2.7 eV peak. There is a broad band at 5.2 eV in the luminescence excitation spectrum for blue emission. The ab-initio quantum-chemical calculation gives a peak in the optical absorption at 5.1 eV for the oxygen vacancy in cubic ZrO2. 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| ispartof | Journal of applied physics, 2014-12, Vol.116 (24) |
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| language | eng |
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| source | AIP Journals Complete; Alma/SFX Local Collection |
| subjects | ABSORPTION SPECTRA Applied physics CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS CONCENTRATION RATIO CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY CUBIC LATTICES EMISSION SPECTRA EV RANGE EXCITATION Excitation spectra Luminescence Organic chemistry Oxide coatings OXYGEN PHOTOLUMINESCENCE Quantum chemistry THIN FILMS VACANCIES Zirconium Zirconium dioxide ZIRCONIUM OXIDES |
| title | The origin of 2.7 eV blue luminescence band in zirconium oxide |
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