Nonlinear delayed symmetry breaking in a solid excited by hard x-ray free electron laser pulses
We have studied the ultrafast changes of electronic states in bulk ZnO upon intense hard x-ray excitation from a free electron laser. By monitoring the transient anisotropy induced in an optical probe beam, we observe a delayed breaking of the initial c-plane symmetry of the crystal that lasts for s...
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| Veröffentlicht in: | Applied physics letters 2015-04, Vol.106 (15) |
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| container_title | Applied physics letters |
| container_volume | 106 |
| creator | Ferrer, A. Johnson, J. A. Huber, T. Mariager, S. O. Trant, M. Grübel, S. Zhu, D. Chollet, M. Robinson, J. Lemke, H. T. Ingold, G. Milne, C. Staub, U. Beaud, P. Johnson, S. L. |
| description | We have studied the ultrafast changes of electronic states in bulk ZnO upon intense hard x-ray excitation from a free electron laser. By monitoring the transient anisotropy induced in an optical probe beam, we observe a delayed breaking of the initial c-plane symmetry of the crystal that lasts for several picoseconds. Interaction with the intense x-ray pulses modifies the electronic state filling in a manner inconsistent with a simple increase in electronic temperature. These results may indicate a way to use intense ultrashort x-ray pulses to investigate high-energy carrier dynamics and to control certain properties of solid-state materials. |
| doi_str_mv | 10.1063/1.4917506 |
| format | Article |
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A. ; Huber, T. ; Mariager, S. O. ; Trant, M. ; Grübel, S. ; Zhu, D. ; Chollet, M. ; Robinson, J. ; Lemke, H. T. ; Ingold, G. ; Milne, C. ; Staub, U. ; Beaud, P. ; Johnson, S. L.</creator><creatorcontrib>Ferrer, A. ; Johnson, J. A. ; Huber, T. ; Mariager, S. O. ; Trant, M. ; Grübel, S. ; Zhu, D. ; Chollet, M. ; Robinson, J. ; Lemke, H. T. ; Ingold, G. ; Milne, C. ; Staub, U. ; Beaud, P. ; Johnson, S. L.</creatorcontrib><description>We have studied the ultrafast changes of electronic states in bulk ZnO upon intense hard x-ray excitation from a free electron laser. By monitoring the transient anisotropy induced in an optical probe beam, we observe a delayed breaking of the initial c-plane symmetry of the crystal that lasts for several picoseconds. Interaction with the intense x-ray pulses modifies the electronic state filling in a manner inconsistent with a simple increase in electronic temperature. These results may indicate a way to use intense ultrashort x-ray pulses to investigate high-energy carrier dynamics and to control certain properties of solid-state materials.</description><identifier>ISSN: 0003-6951</identifier><identifier>EISSN: 1077-3118</identifier><identifier>DOI: 10.1063/1.4917506</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>ANISOTROPY ; Applied physics ; Broken symmetry ; CHARGE CARRIERS ; CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY ; CRYSTALS ; Electron states ; ELECTRONIC STRUCTURE ; EXCITATION ; FREE ELECTRON LASERS ; HARD X RADIATION ; Laser beams ; MONITORING ; NONLINEAR PROBLEMS ; PHYSICAL RADIATION EFFECTS ; PROBES ; SOLIDS ; SYMMETRY BREAKING ; TRANSIENTS ; Zinc oxide ; ZINC OXIDES</subject><ispartof>Applied physics letters, 2015-04, Vol.106 (15)</ispartof><rights>2015 AIP Publishing LLC.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c320t-a5cc3ef87fcc27e31b34189bfcd9f0e5c8228c99cc0bd63e230fd7449992075e3</citedby><cites>FETCH-LOGICAL-c320t-a5cc3ef87fcc27e31b34189bfcd9f0e5c8228c99cc0bd63e230fd7449992075e3</cites><orcidid>0000-0003-4714-9139</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,776,780,881,27901,27902</link.rule.ids><backlink>$$Uhttps://www.osti.gov/biblio/22398913$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Ferrer, A.</creatorcontrib><creatorcontrib>Johnson, J. A.</creatorcontrib><creatorcontrib>Huber, T.</creatorcontrib><creatorcontrib>Mariager, S. O.</creatorcontrib><creatorcontrib>Trant, M.</creatorcontrib><creatorcontrib>Grübel, S.</creatorcontrib><creatorcontrib>Zhu, D.</creatorcontrib><creatorcontrib>Chollet, M.</creatorcontrib><creatorcontrib>Robinson, J.</creatorcontrib><creatorcontrib>Lemke, H. T.</creatorcontrib><creatorcontrib>Ingold, G.</creatorcontrib><creatorcontrib>Milne, C.</creatorcontrib><creatorcontrib>Staub, U.</creatorcontrib><creatorcontrib>Beaud, P.</creatorcontrib><creatorcontrib>Johnson, S. L.</creatorcontrib><title>Nonlinear delayed symmetry breaking in a solid excited by hard x-ray free electron laser pulses</title><title>Applied physics letters</title><description>We have studied the ultrafast changes of electronic states in bulk ZnO upon intense hard x-ray excitation from a free electron laser. By monitoring the transient anisotropy induced in an optical probe beam, we observe a delayed breaking of the initial c-plane symmetry of the crystal that lasts for several picoseconds. Interaction with the intense x-ray pulses modifies the electronic state filling in a manner inconsistent with a simple increase in electronic temperature. These results may indicate a way to use intense ultrashort x-ray pulses to investigate high-energy carrier dynamics and to control certain properties of solid-state materials.</description><subject>ANISOTROPY</subject><subject>Applied physics</subject><subject>Broken symmetry</subject><subject>CHARGE CARRIERS</subject><subject>CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY</subject><subject>CRYSTALS</subject><subject>Electron states</subject><subject>ELECTRONIC STRUCTURE</subject><subject>EXCITATION</subject><subject>FREE ELECTRON LASERS</subject><subject>HARD X RADIATION</subject><subject>Laser beams</subject><subject>MONITORING</subject><subject>NONLINEAR PROBLEMS</subject><subject>PHYSICAL RADIATION EFFECTS</subject><subject>PROBES</subject><subject>SOLIDS</subject><subject>SYMMETRY BREAKING</subject><subject>TRANSIENTS</subject><subject>Zinc oxide</subject><subject>ZINC OXIDES</subject><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><recordid>eNpFkE1LAzEQhoMoWKsH_0HAk4etSWa3uzlK8QuKXvQcsrMTu3Wb1GQL3X_vlhY8zQw8vPPwMnYrxUyKOTzIWa5lWYj5GZtIUZYZSFmds4kQArK5LuQlu0ppPZ6FApgw8x5813qykTfU2YEanobNhvo48DqS_Wn9N289tzyFrm047bHtR6ge-MrGhu-zaAfuIhGnjrCPwfPOJop8u-sSpWt24ey43JzmlH09P30uXrPlx8vb4nGZISjRZ7ZABHJV6RBVSSBryGWla4eNdoIKrJSqUGtEUTdzIAXCNWWea62VKAuCKbs75obUtyYdJHGFwfvRySgFutIS_qltDL87Sr1Zh130o5hRUuXjExh7mrL7I4UxpBTJmW1sNzYORgpzaNlIc2oZ_gAxSG5M</recordid><startdate>20150413</startdate><enddate>20150413</enddate><creator>Ferrer, A.</creator><creator>Johnson, J. 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L.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Nonlinear delayed symmetry breaking in a solid excited by hard x-ray free electron laser pulses</atitle><jtitle>Applied physics letters</jtitle><date>2015-04-13</date><risdate>2015</risdate><volume>106</volume><issue>15</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><abstract>We have studied the ultrafast changes of electronic states in bulk ZnO upon intense hard x-ray excitation from a free electron laser. By monitoring the transient anisotropy induced in an optical probe beam, we observe a delayed breaking of the initial c-plane symmetry of the crystal that lasts for several picoseconds. Interaction with the intense x-ray pulses modifies the electronic state filling in a manner inconsistent with a simple increase in electronic temperature. 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| ispartof | Applied physics letters, 2015-04, Vol.106 (15) |
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| source | AIP Journals Complete; Alma/SFX Local Collection |
| subjects | ANISOTROPY Applied physics Broken symmetry CHARGE CARRIERS CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY CRYSTALS Electron states ELECTRONIC STRUCTURE EXCITATION FREE ELECTRON LASERS HARD X RADIATION Laser beams MONITORING NONLINEAR PROBLEMS PHYSICAL RADIATION EFFECTS PROBES SOLIDS SYMMETRY BREAKING TRANSIENTS Zinc oxide ZINC OXIDES |
| title | Nonlinear delayed symmetry breaking in a solid excited by hard x-ray free electron laser pulses |
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