The ReactorAFM: non-contact atomic force microscope operating under high-pressure and high-temperature catalytic conditions
An Atomic Force Microscope (AFM) has been integrated in a miniature high-pressure flow reactor for in-situ observations of heterogeneous catalytic reactions under conditions similar to those of industrial processes. The AFM can image model catalysts such as those consisting of metal nanoparticles on...
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| Veröffentlicht in: | Review of scientific instruments 2015-03, Vol.86 (3), p.033706-033706 |
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| container_title | Review of scientific instruments |
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| creator | Roobol, S B Cañas-Ventura, M E Bergman, M van Spronsen, M A Onderwaater, W G van der Tuijn, P C Koehler, R Ofitserov, A van Baarle, G J C Frenken, J W M |
| description | An Atomic Force Microscope (AFM) has been integrated in a miniature high-pressure flow reactor for in-situ observations of heterogeneous catalytic reactions under conditions similar to those of industrial processes. The AFM can image model catalysts such as those consisting of metal nanoparticles on flat oxide supports in a gas atmosphere up to 6 bar and at a temperature up to 600 K, while the catalytic activity can be measured using mass spectrometry. The high-pressure reactor is placed inside an Ultrahigh Vacuum (UHV) system to supplement it with standard UHV sample preparation and characterization techniques. To demonstrate that this instrument successfully bridges both the pressure gap and the materials gap, images have been recorded of supported palladium nanoparticles catalyzing the oxidation of carbon monoxide under high-pressure, high-temperature conditions. |
| doi_str_mv | 10.1063/1.4916194 |
| format | Article |
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The AFM can image model catalysts such as those consisting of metal nanoparticles on flat oxide supports in a gas atmosphere up to 6 bar and at a temperature up to 600 K, while the catalytic activity can be measured using mass spectrometry. The high-pressure reactor is placed inside an Ultrahigh Vacuum (UHV) system to supplement it with standard UHV sample preparation and characterization techniques. To demonstrate that this instrument successfully bridges both the pressure gap and the materials gap, images have been recorded of supported palladium nanoparticles catalyzing the oxidation of carbon monoxide under high-pressure, high-temperature conditions.</description><identifier>ISSN: 0034-6748</identifier><identifier>EISSN: 1089-7623</identifier><identifier>DOI: 10.1063/1.4916194</identifier><identifier>PMID: 25832237</identifier><language>eng</language><publisher>United States: American Institute of Physics</publisher><subject>ATMOSPHERES ; Atomic force microscopes ; ATOMIC FORCE MICROSCOPY ; CARBON MONOXIDE ; Catalysis ; CATALYSTS ; Catalytic activity ; Contact pressure ; INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY ; INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY ; Mass spectrometry ; MASS SPECTROSCOPY ; Microscopes ; NANOPARTICLES ; Nuclear reactors ; OXIDATION ; PALLADIUM ; SAMPLE PREPARATION ; Scientific apparatus & instruments ; TEMPERATURE RANGE 0400-1000 K ; Ultrahigh vacuum</subject><ispartof>Review of scientific instruments, 2015-03, Vol.86 (3), p.033706-033706</ispartof><rights>2015 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c479t-2feb68cce0e84a1ccac9bf82583cc4e41f7504cec8f7424ce4cbdd807b21920d3</citedby><cites>FETCH-LOGICAL-c479t-2feb68cce0e84a1ccac9bf82583cc4e41f7504cec8f7424ce4cbdd807b21920d3</cites><orcidid>0000-0001-9307-9851</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,776,780,881,27901,27902</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/25832237$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/biblio/22392415$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Roobol, S B</creatorcontrib><creatorcontrib>Cañas-Ventura, M E</creatorcontrib><creatorcontrib>Bergman, M</creatorcontrib><creatorcontrib>van Spronsen, M A</creatorcontrib><creatorcontrib>Onderwaater, W G</creatorcontrib><creatorcontrib>van der Tuijn, P C</creatorcontrib><creatorcontrib>Koehler, R</creatorcontrib><creatorcontrib>Ofitserov, A</creatorcontrib><creatorcontrib>van Baarle, G J C</creatorcontrib><creatorcontrib>Frenken, J W M</creatorcontrib><title>The ReactorAFM: non-contact atomic force microscope operating under high-pressure and high-temperature catalytic conditions</title><title>Review of scientific instruments</title><addtitle>Rev Sci Instrum</addtitle><description>An Atomic Force Microscope (AFM) has been integrated in a miniature high-pressure flow reactor for in-situ observations of heterogeneous catalytic reactions under conditions similar to those of industrial processes. The AFM can image model catalysts such as those consisting of metal nanoparticles on flat oxide supports in a gas atmosphere up to 6 bar and at a temperature up to 600 K, while the catalytic activity can be measured using mass spectrometry. The high-pressure reactor is placed inside an Ultrahigh Vacuum (UHV) system to supplement it with standard UHV sample preparation and characterization techniques. To demonstrate that this instrument successfully bridges both the pressure gap and the materials gap, images have been recorded of supported palladium nanoparticles catalyzing the oxidation of carbon monoxide under high-pressure, high-temperature conditions.</description><subject>ATMOSPHERES</subject><subject>Atomic force microscopes</subject><subject>ATOMIC FORCE MICROSCOPY</subject><subject>CARBON MONOXIDE</subject><subject>Catalysis</subject><subject>CATALYSTS</subject><subject>Catalytic activity</subject><subject>Contact pressure</subject><subject>INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY</subject><subject>INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY</subject><subject>Mass spectrometry</subject><subject>MASS SPECTROSCOPY</subject><subject>Microscopes</subject><subject>NANOPARTICLES</subject><subject>Nuclear reactors</subject><subject>OXIDATION</subject><subject>PALLADIUM</subject><subject>SAMPLE PREPARATION</subject><subject>Scientific apparatus & instruments</subject><subject>TEMPERATURE RANGE 0400-1000 K</subject><subject>Ultrahigh vacuum</subject><issn>0034-6748</issn><issn>1089-7623</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><recordid>eNpFkdFrFDEQxoMo9qw--A9IwBd92JrJ5nYT30pptVARpD6H7OxsL-U2OZPsQ_Gfb6531sCQ4ePHx8x8jL0HcQaia7_AmTLQgVEv2AqENk3fyfYlWwnRqqbrlT5hb3K-F_WtAV6zE7nWrZRtv2J_bzfEf5HDEtP51Y-vPMTQYAylKtyVOHvkU0xIvHYpZow74rWSKz7c8SWMlPjG322aXaKcl0TchfGgFJqfwL2IrrjtQ6lu1Xz0xceQ37JXk9tmenf8T9nvq8vbi-_Nzc9v1xfnNw2q3pRGTjR0GpEEaeUA0aEZJr3fAVGRgqlfC4WEeuqVrI3CYRy16AcJRoqxPWUfD74xF28z-kK4qWMEwmLrGYxUsK7UpwO1S_HPQrnY2Wek7dYFiku20HVGt0oY9d_wGb2PSwp1BytBKt2Bgq5Snw_U_m450WR3yc8uPVgQdp-bBXvMrbIfjo7LMNP4TP4Lqn0EaC-Thg</recordid><startdate>20150301</startdate><enddate>20150301</enddate><creator>Roobol, S B</creator><creator>Cañas-Ventura, M E</creator><creator>Bergman, M</creator><creator>van Spronsen, M A</creator><creator>Onderwaater, W G</creator><creator>van der Tuijn, P C</creator><creator>Koehler, R</creator><creator>Ofitserov, A</creator><creator>van Baarle, G J C</creator><creator>Frenken, J W M</creator><general>American Institute of Physics</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><scope>7X8</scope><scope>OTOTI</scope><orcidid>https://orcid.org/0000-0001-9307-9851</orcidid></search><sort><creationdate>20150301</creationdate><title>The ReactorAFM: non-contact atomic force microscope operating under high-pressure and high-temperature catalytic conditions</title><author>Roobol, S B ; Cañas-Ventura, M E ; Bergman, M ; van Spronsen, M A ; Onderwaater, W G ; van der Tuijn, P C ; Koehler, R ; Ofitserov, A ; van Baarle, G J C ; Frenken, J W M</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c479t-2feb68cce0e84a1ccac9bf82583cc4e41f7504cec8f7424ce4cbdd807b21920d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>ATMOSPHERES</topic><topic>Atomic force microscopes</topic><topic>ATOMIC FORCE MICROSCOPY</topic><topic>CARBON MONOXIDE</topic><topic>Catalysis</topic><topic>CATALYSTS</topic><topic>Catalytic activity</topic><topic>Contact pressure</topic><topic>INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY</topic><topic>INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY</topic><topic>Mass spectrometry</topic><topic>MASS SPECTROSCOPY</topic><topic>Microscopes</topic><topic>NANOPARTICLES</topic><topic>Nuclear reactors</topic><topic>OXIDATION</topic><topic>PALLADIUM</topic><topic>SAMPLE PREPARATION</topic><topic>Scientific apparatus & instruments</topic><topic>TEMPERATURE RANGE 0400-1000 K</topic><topic>Ultrahigh vacuum</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Roobol, S B</creatorcontrib><creatorcontrib>Cañas-Ventura, M E</creatorcontrib><creatorcontrib>Bergman, M</creatorcontrib><creatorcontrib>van Spronsen, M A</creatorcontrib><creatorcontrib>Onderwaater, W G</creatorcontrib><creatorcontrib>van der Tuijn, P C</creatorcontrib><creatorcontrib>Koehler, R</creatorcontrib><creatorcontrib>Ofitserov, A</creatorcontrib><creatorcontrib>van Baarle, G J C</creatorcontrib><creatorcontrib>Frenken, J W M</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><collection>OSTI.GOV</collection><jtitle>Review of scientific instruments</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Roobol, S B</au><au>Cañas-Ventura, M E</au><au>Bergman, M</au><au>van Spronsen, M A</au><au>Onderwaater, W G</au><au>van der Tuijn, P C</au><au>Koehler, R</au><au>Ofitserov, A</au><au>van Baarle, G J C</au><au>Frenken, J W M</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>The ReactorAFM: non-contact atomic force microscope operating under high-pressure and high-temperature catalytic conditions</atitle><jtitle>Review of scientific instruments</jtitle><addtitle>Rev Sci Instrum</addtitle><date>2015-03-01</date><risdate>2015</risdate><volume>86</volume><issue>3</issue><spage>033706</spage><epage>033706</epage><pages>033706-033706</pages><issn>0034-6748</issn><eissn>1089-7623</eissn><abstract>An Atomic Force Microscope (AFM) has been integrated in a miniature high-pressure flow reactor for in-situ observations of heterogeneous catalytic reactions under conditions similar to those of industrial processes. The AFM can image model catalysts such as those consisting of metal nanoparticles on flat oxide supports in a gas atmosphere up to 6 bar and at a temperature up to 600 K, while the catalytic activity can be measured using mass spectrometry. The high-pressure reactor is placed inside an Ultrahigh Vacuum (UHV) system to supplement it with standard UHV sample preparation and characterization techniques. To demonstrate that this instrument successfully bridges both the pressure gap and the materials gap, images have been recorded of supported palladium nanoparticles catalyzing the oxidation of carbon monoxide under high-pressure, high-temperature conditions.</abstract><cop>United States</cop><pub>American Institute of Physics</pub><pmid>25832237</pmid><doi>10.1063/1.4916194</doi><tpages>1</tpages><orcidid>https://orcid.org/0000-0001-9307-9851</orcidid><oa>free_for_read</oa></addata></record> |
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| ispartof | Review of scientific instruments, 2015-03, Vol.86 (3), p.033706-033706 |
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| source | AIP Journals; Alma/SFX Local Collection |
| subjects | ATMOSPHERES Atomic force microscopes ATOMIC FORCE MICROSCOPY CARBON MONOXIDE Catalysis CATALYSTS Catalytic activity Contact pressure INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY Mass spectrometry MASS SPECTROSCOPY Microscopes NANOPARTICLES Nuclear reactors OXIDATION PALLADIUM SAMPLE PREPARATION Scientific apparatus & instruments TEMPERATURE RANGE 0400-1000 K Ultrahigh vacuum |
| title | The ReactorAFM: non-contact atomic force microscope operating under high-pressure and high-temperature catalytic conditions |
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