Successful application of lead isotopes in source apportionment, legal proceedings, remediation and monitoring
In late 2006, the seaside community in Esperance Western Australia was alerted to thousands of native bird species dying. The source of the lead (Pb) was determined by Pb isotopes to derive from the handling of Pb carbonate concentrate through the Port, which began in July 2005. Concern was expresse...
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| Veröffentlicht in: | Environmental research 2012-01, Vol.112, p.100-110 |
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| creator | Gulson, Brian Korsch, Michael Winchester, Wayne Devenish, Matthew Hobbs, Thad Main, Cleve Smith, Gerard Rosman, Kevin Howearth, Lynette Burn-Nunes, Laurie Seow, Jimmy Oxford, Cameron Yun, Gracie Gillam, Lindsay Crisp, Michelle |
| description | In late 2006, the seaside community in Esperance Western Australia was alerted to thousands of native bird species dying. The source of the lead (Pb) was determined by Pb isotopes to derive from the handling of Pb carbonate concentrate through the Port, which began in July 2005. Concern was expressed for the impact of this on the community. Our objectives were to employ Pb isotope ratios to evaluate the source of Pb in environmental samples for use in legal proceedings, and for use in remediation and monitoring. Isotope measurements were undertaken of bird livers, plants, drinking water, soil, harbour sediments, air, bulk ceiling dust, gutter sludge, surface swabs and blood. The unique lead isotopic signature of the contaminating Pb carbonate enabled diagnostic apportionment of lead in samples. Apart from some soil and water samples, the proportion of contaminating Pb was >95% in the environmental samples. Lead isotopes were critical in resolving legal proceedings, are being used in the remediation of premises, were used in monitoring of workers involved in the decontamination of the storage facility, and monitoring transport of the concentrate through another port facility. Air samples show the continued presence of contaminant Pb, more than one year after shipping of concentrate ceased, probably arising from dust resuspension. Brief details of the comprehensive testing and cleanup of the Esperance community are provided along with the role of the Community. Lead isotopic analyses can provide significant benefits to regulatory agencies, interested parties, and the community where the signature is able to be characterised with a high degree of certainty.
▶ Lead carbonate concentrate. ▶ Successful use of Pb isotopes in identifying sources of Pb arising from transport and shipping. ▶ Use of Pb isotopes in legal proceedings and their use in cleanup of residences. ▶ Use of Pb isotopes in cleanup of a residual 9000 tonnes of Pb carbonate and in ongoing monitoring. |
| doi_str_mv | 10.1016/j.envres.2011.08.007 |
| format | Article |
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▶ Lead carbonate concentrate. ▶ Successful use of Pb isotopes in identifying sources of Pb arising from transport and shipping. ▶ Use of Pb isotopes in legal proceedings and their use in cleanup of residences. ▶ Use of Pb isotopes in cleanup of a residual 9000 tonnes of Pb carbonate and in ongoing monitoring.</description><identifier>ISSN: 0013-9351</identifier><identifier>EISSN: 1096-0953</identifier><identifier>DOI: 10.1016/j.envres.2011.08.007</identifier><identifier>PMID: 21925655</identifier><identifier>CODEN: ENVRAL</identifier><language>eng</language><publisher>Amsterdam: Elsevier Inc</publisher><subject>Air ; Air - analysis ; Animal, plant and microbial ecology ; Animals ; Applied ecology ; Biological and medical sciences ; Bird liver ; BIRDS ; Birds - blood ; Birds - metabolism ; Carbonates - analysis ; Carbonates - blood ; Carbonates - toxicity ; Child ; DRINKING WATER ; Ecotoxicology, biological effects of pollution ; Environmental Monitoring - legislation & jurisprudence ; Environmental Monitoring - methods ; Environmental Pollutants - analysis ; Environmental Pollutants - blood ; Environmental Pollutants - toxicity ; Environmental Restoration and Remediation - legislation & jurisprudence ; Environmental Restoration and Remediation - methods ; ENVIRONMENTAL SCIENCES ; Fundamental and applied biological sciences. Psychology ; Geologic Sediments - analysis ; Government Agencies ; Government Regulation ; Humans ; LEAD ; Lead - analysis ; Lead - blood ; Lead - toxicity ; Lead carbonate ; LEAD CARBONATES ; LEAD ISOTOPES ; Lead Radioisotopes - analysis ; Lead Radioisotopes - blood ; LIVER ; Liver - chemistry ; Plants ; Rain - chemistry ; Soil - analysis ; Techniques ; Water ; Western Australia</subject><ispartof>Environmental research, 2012-01, Vol.112, p.100-110</ispartof><rights>2011</rights><rights>2015 INIST-CNRS</rights><rights>Crown Copyright © 2011. Published by Elsevier Inc. All rights reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c419t-c1ddc81997486c06e943d4da62ab8a32dbe5af395c9c351437cd17926b89a1dc3</citedby><cites>FETCH-LOGICAL-c419t-c1ddc81997486c06e943d4da62ab8a32dbe5af395c9c351437cd17926b89a1dc3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0013935111002064$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>230,314,776,780,881,3536,27903,27904,65309</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=25548848$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/21925655$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/biblio/22156250$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Gulson, Brian</creatorcontrib><creatorcontrib>Korsch, Michael</creatorcontrib><creatorcontrib>Winchester, Wayne</creatorcontrib><creatorcontrib>Devenish, Matthew</creatorcontrib><creatorcontrib>Hobbs, Thad</creatorcontrib><creatorcontrib>Main, Cleve</creatorcontrib><creatorcontrib>Smith, Gerard</creatorcontrib><creatorcontrib>Rosman, Kevin</creatorcontrib><creatorcontrib>Howearth, Lynette</creatorcontrib><creatorcontrib>Burn-Nunes, Laurie</creatorcontrib><creatorcontrib>Seow, Jimmy</creatorcontrib><creatorcontrib>Oxford, Cameron</creatorcontrib><creatorcontrib>Yun, Gracie</creatorcontrib><creatorcontrib>Gillam, Lindsay</creatorcontrib><creatorcontrib>Crisp, Michelle</creatorcontrib><title>Successful application of lead isotopes in source apportionment, legal proceedings, remediation and monitoring</title><title>Environmental research</title><addtitle>Environ Res</addtitle><description>In late 2006, the seaside community in Esperance Western Australia was alerted to thousands of native bird species dying. The source of the lead (Pb) was determined by Pb isotopes to derive from the handling of Pb carbonate concentrate through the Port, which began in July 2005. Concern was expressed for the impact of this on the community. Our objectives were to employ Pb isotope ratios to evaluate the source of Pb in environmental samples for use in legal proceedings, and for use in remediation and monitoring. Isotope measurements were undertaken of bird livers, plants, drinking water, soil, harbour sediments, air, bulk ceiling dust, gutter sludge, surface swabs and blood. The unique lead isotopic signature of the contaminating Pb carbonate enabled diagnostic apportionment of lead in samples. Apart from some soil and water samples, the proportion of contaminating Pb was >95% in the environmental samples. Lead isotopes were critical in resolving legal proceedings, are being used in the remediation of premises, were used in monitoring of workers involved in the decontamination of the storage facility, and monitoring transport of the concentrate through another port facility. Air samples show the continued presence of contaminant Pb, more than one year after shipping of concentrate ceased, probably arising from dust resuspension. Brief details of the comprehensive testing and cleanup of the Esperance community are provided along with the role of the Community. Lead isotopic analyses can provide significant benefits to regulatory agencies, interested parties, and the community where the signature is able to be characterised with a high degree of certainty.
▶ Lead carbonate concentrate. ▶ Successful use of Pb isotopes in identifying sources of Pb arising from transport and shipping. ▶ Use of Pb isotopes in legal proceedings and their use in cleanup of residences. ▶ Use of Pb isotopes in cleanup of a residual 9000 tonnes of Pb carbonate and in ongoing monitoring.</description><subject>Air</subject><subject>Air - analysis</subject><subject>Animal, plant and microbial ecology</subject><subject>Animals</subject><subject>Applied ecology</subject><subject>Biological and medical sciences</subject><subject>Bird liver</subject><subject>BIRDS</subject><subject>Birds - blood</subject><subject>Birds - metabolism</subject><subject>Carbonates - analysis</subject><subject>Carbonates - blood</subject><subject>Carbonates - toxicity</subject><subject>Child</subject><subject>DRINKING WATER</subject><subject>Ecotoxicology, biological effects of pollution</subject><subject>Environmental Monitoring - legislation & jurisprudence</subject><subject>Environmental Monitoring - methods</subject><subject>Environmental Pollutants - analysis</subject><subject>Environmental Pollutants - blood</subject><subject>Environmental Pollutants - toxicity</subject><subject>Environmental Restoration and Remediation - legislation & jurisprudence</subject><subject>Environmental Restoration and Remediation - methods</subject><subject>ENVIRONMENTAL SCIENCES</subject><subject>Fundamental and applied biological sciences. Psychology</subject><subject>Geologic Sediments - analysis</subject><subject>Government Agencies</subject><subject>Government Regulation</subject><subject>Humans</subject><subject>LEAD</subject><subject>Lead - analysis</subject><subject>Lead - blood</subject><subject>Lead - toxicity</subject><subject>Lead carbonate</subject><subject>LEAD CARBONATES</subject><subject>LEAD ISOTOPES</subject><subject>Lead Radioisotopes - analysis</subject><subject>Lead Radioisotopes - blood</subject><subject>LIVER</subject><subject>Liver - chemistry</subject><subject>Plants</subject><subject>Rain - chemistry</subject><subject>Soil - analysis</subject><subject>Techniques</subject><subject>Water</subject><subject>Western Australia</subject><issn>0013-9351</issn><issn>1096-0953</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2012</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNp9kU-L1TAUxYMozpvRbyBSEHEzrUnTtMlGkMFRYcCFug55N7djHm1Sk3TAb29Kn7pzlYT87p9zDiEvGG0YZf3bU4P-IWJqWspYQ2VD6fCIHBhVfU2V4I_JgVLGa8UFuyCXKZ3KkwlOn5KLlqlW9EIciP-6AmBK4zpVZlkmBya74KswVhMaW7kUclgwVc5XKawRcMNC3KAZfb4u2L2ZqiUGQLTO36frKuJcrnsj4201B-9yiOXzGXkyminh8_N5Rb7ffvh286m--_Lx8837uxo6pnINzFqQTKmhkz3QHlXHbWdN35qjNLy1RxRm5EqAgiKv4wNYNqi2P0plmAV-RV7tfUPKTidwGeEHBO8Rsm5bJvpW0EK92amy_c8VU9azS4DTZDyGNWnFpBhkR3khu52EGFKKOOolutnEX5pRvcWhT3qPQ29xaCp1iaOUvTwPWI_Fkr9Ff_wvwOszYBKYaYzGg0v_OCE6KTtZuHc7h8W0B4dx04Qeis1xk2SD-_8mvwEB26w0</recordid><startdate>20120101</startdate><enddate>20120101</enddate><creator>Gulson, Brian</creator><creator>Korsch, Michael</creator><creator>Winchester, Wayne</creator><creator>Devenish, Matthew</creator><creator>Hobbs, Thad</creator><creator>Main, Cleve</creator><creator>Smith, Gerard</creator><creator>Rosman, Kevin</creator><creator>Howearth, Lynette</creator><creator>Burn-Nunes, Laurie</creator><creator>Seow, Jimmy</creator><creator>Oxford, Cameron</creator><creator>Yun, Gracie</creator><creator>Gillam, Lindsay</creator><creator>Crisp, Michelle</creator><general>Elsevier Inc</general><general>Elsevier</general><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>OTOTI</scope></search><sort><creationdate>20120101</creationdate><title>Successful application of lead isotopes in source apportionment, legal proceedings, remediation and monitoring</title><author>Gulson, Brian ; Korsch, Michael ; Winchester, Wayne ; Devenish, Matthew ; Hobbs, Thad ; Main, Cleve ; Smith, Gerard ; Rosman, Kevin ; Howearth, Lynette ; Burn-Nunes, Laurie ; Seow, Jimmy ; Oxford, Cameron ; Yun, Gracie ; Gillam, Lindsay ; Crisp, Michelle</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c419t-c1ddc81997486c06e943d4da62ab8a32dbe5af395c9c351437cd17926b89a1dc3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2012</creationdate><topic>Air</topic><topic>Air - analysis</topic><topic>Animal, plant and microbial ecology</topic><topic>Animals</topic><topic>Applied ecology</topic><topic>Biological and medical sciences</topic><topic>Bird liver</topic><topic>BIRDS</topic><topic>Birds - blood</topic><topic>Birds - metabolism</topic><topic>Carbonates - analysis</topic><topic>Carbonates - blood</topic><topic>Carbonates - toxicity</topic><topic>Child</topic><topic>DRINKING WATER</topic><topic>Ecotoxicology, biological effects of pollution</topic><topic>Environmental Monitoring - legislation & jurisprudence</topic><topic>Environmental Monitoring - methods</topic><topic>Environmental Pollutants - analysis</topic><topic>Environmental Pollutants - blood</topic><topic>Environmental Pollutants - toxicity</topic><topic>Environmental Restoration and Remediation - legislation & jurisprudence</topic><topic>Environmental Restoration and Remediation - methods</topic><topic>ENVIRONMENTAL SCIENCES</topic><topic>Fundamental and applied biological sciences. Psychology</topic><topic>Geologic Sediments - analysis</topic><topic>Government Agencies</topic><topic>Government Regulation</topic><topic>Humans</topic><topic>LEAD</topic><topic>Lead - analysis</topic><topic>Lead - blood</topic><topic>Lead - toxicity</topic><topic>Lead carbonate</topic><topic>LEAD CARBONATES</topic><topic>LEAD ISOTOPES</topic><topic>Lead Radioisotopes - analysis</topic><topic>Lead Radioisotopes - blood</topic><topic>LIVER</topic><topic>Liver - chemistry</topic><topic>Plants</topic><topic>Rain - chemistry</topic><topic>Soil - analysis</topic><topic>Techniques</topic><topic>Water</topic><topic>Western Australia</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Gulson, Brian</creatorcontrib><creatorcontrib>Korsch, Michael</creatorcontrib><creatorcontrib>Winchester, Wayne</creatorcontrib><creatorcontrib>Devenish, Matthew</creatorcontrib><creatorcontrib>Hobbs, Thad</creatorcontrib><creatorcontrib>Main, Cleve</creatorcontrib><creatorcontrib>Smith, Gerard</creatorcontrib><creatorcontrib>Rosman, Kevin</creatorcontrib><creatorcontrib>Howearth, Lynette</creatorcontrib><creatorcontrib>Burn-Nunes, Laurie</creatorcontrib><creatorcontrib>Seow, Jimmy</creatorcontrib><creatorcontrib>Oxford, Cameron</creatorcontrib><creatorcontrib>Yun, Gracie</creatorcontrib><creatorcontrib>Gillam, Lindsay</creatorcontrib><creatorcontrib>Crisp, Michelle</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>OSTI.GOV</collection><jtitle>Environmental research</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Gulson, Brian</au><au>Korsch, Michael</au><au>Winchester, Wayne</au><au>Devenish, Matthew</au><au>Hobbs, Thad</au><au>Main, Cleve</au><au>Smith, Gerard</au><au>Rosman, Kevin</au><au>Howearth, Lynette</au><au>Burn-Nunes, Laurie</au><au>Seow, Jimmy</au><au>Oxford, Cameron</au><au>Yun, Gracie</au><au>Gillam, Lindsay</au><au>Crisp, Michelle</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Successful application of lead isotopes in source apportionment, legal proceedings, remediation and monitoring</atitle><jtitle>Environmental research</jtitle><addtitle>Environ Res</addtitle><date>2012-01-01</date><risdate>2012</risdate><volume>112</volume><spage>100</spage><epage>110</epage><pages>100-110</pages><issn>0013-9351</issn><eissn>1096-0953</eissn><coden>ENVRAL</coden><abstract>In late 2006, the seaside community in Esperance Western Australia was alerted to thousands of native bird species dying. The source of the lead (Pb) was determined by Pb isotopes to derive from the handling of Pb carbonate concentrate through the Port, which began in July 2005. Concern was expressed for the impact of this on the community. Our objectives were to employ Pb isotope ratios to evaluate the source of Pb in environmental samples for use in legal proceedings, and for use in remediation and monitoring. Isotope measurements were undertaken of bird livers, plants, drinking water, soil, harbour sediments, air, bulk ceiling dust, gutter sludge, surface swabs and blood. The unique lead isotopic signature of the contaminating Pb carbonate enabled diagnostic apportionment of lead in samples. Apart from some soil and water samples, the proportion of contaminating Pb was >95% in the environmental samples. Lead isotopes were critical in resolving legal proceedings, are being used in the remediation of premises, were used in monitoring of workers involved in the decontamination of the storage facility, and monitoring transport of the concentrate through another port facility. Air samples show the continued presence of contaminant Pb, more than one year after shipping of concentrate ceased, probably arising from dust resuspension. Brief details of the comprehensive testing and cleanup of the Esperance community are provided along with the role of the Community. Lead isotopic analyses can provide significant benefits to regulatory agencies, interested parties, and the community where the signature is able to be characterised with a high degree of certainty.
▶ Lead carbonate concentrate. ▶ Successful use of Pb isotopes in identifying sources of Pb arising from transport and shipping. ▶ Use of Pb isotopes in legal proceedings and their use in cleanup of residences. ▶ Use of Pb isotopes in cleanup of a residual 9000 tonnes of Pb carbonate and in ongoing monitoring.</abstract><cop>Amsterdam</cop><pub>Elsevier Inc</pub><pmid>21925655</pmid><doi>10.1016/j.envres.2011.08.007</doi><tpages>11</tpages></addata></record> |
| fulltext | fulltext |
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| ispartof | Environmental research, 2012-01, Vol.112, p.100-110 |
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| recordid | cdi_osti_scitechconnect_22156250 |
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| subjects | Air Air - analysis Animal, plant and microbial ecology Animals Applied ecology Biological and medical sciences Bird liver BIRDS Birds - blood Birds - metabolism Carbonates - analysis Carbonates - blood Carbonates - toxicity Child DRINKING WATER Ecotoxicology, biological effects of pollution Environmental Monitoring - legislation & jurisprudence Environmental Monitoring - methods Environmental Pollutants - analysis Environmental Pollutants - blood Environmental Pollutants - toxicity Environmental Restoration and Remediation - legislation & jurisprudence Environmental Restoration and Remediation - methods ENVIRONMENTAL SCIENCES Fundamental and applied biological sciences. Psychology Geologic Sediments - analysis Government Agencies Government Regulation Humans LEAD Lead - analysis Lead - blood Lead - toxicity Lead carbonate LEAD CARBONATES LEAD ISOTOPES Lead Radioisotopes - analysis Lead Radioisotopes - blood LIVER Liver - chemistry Plants Rain - chemistry Soil - analysis Techniques Water Western Australia |
| title | Successful application of lead isotopes in source apportionment, legal proceedings, remediation and monitoring |
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