Experimental verification of a self-consistent theory of the first-, second-, and third-order (non)linear optical response

We show that a combination of linear absorption spectroscopy, hyper-Rayleigh scattering, and a theoretical analysis using sum rules to reduce the size of the parameter space leads to a prediction of the imaginary part of the second hyperpolarizability of the dye AF-455 that agrees with the experimen...

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Veröffentlicht in:	Physical review. A, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 2011-09, Vol.84 (3), Article 033837
Hauptverfasser:	Pérez-Moreno, Javier, Hung, Sheng-Ting, Kuzyk, Mark G., Zhou, Juefei, Ramini, Shiva K., Clays, Koen
Format:	Artikel
Sprache:	eng
Schlagworte:	ABSORPTION SPECTROSCOPY ATOMIC AND MOLECULAR PHYSICS EXCITED STATES NONLINEAR PROBLEMS PHOTONS PHYSICS OF ELEMENTARY PARTICLES AND FIELDS RAYLEIGH SCATTERING SUM RULES SYMMETRY VERIFICATION
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