Chirped-pulse millimeter-wave spectroscopy of Rydberg-Rydberg transitions
Transitions between Rydberg states of Ca atoms, in a pulsed, supersonic atomic beam, are directly detected by chirped-pulse millimeter-wave spectroscopy. Broadband, high-resolution spectra with accurate relative intensities are recorded instantly. Free induction decay (FID) of atoms, polarized by th...
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Veröffentlicht in: | Physical review letters 2011-09, Vol.107 (14), p.143001-143001, Article 143001 |
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container_title | Physical review letters |
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creator | Prozument, Kirill Colombo, Anthony P Zhou, Yan Park, G Barratt Petrović, Vladimir S Coy, Stephen L Field, Robert W |
description | Transitions between Rydberg states of Ca atoms, in a pulsed, supersonic atomic beam, are directly detected by chirped-pulse millimeter-wave spectroscopy. Broadband, high-resolution spectra with accurate relative intensities are recorded instantly. Free induction decay (FID) of atoms, polarized by the chirped pulse, at their Rydberg-Rydberg transition frequencies, is heterodyne detected, averaged in the time domain, and Fourier transformed into the frequency domain. Millimeter-wave transient nutations are observed, and the possibility of FID evolving to superradiance is discussed. |
doi_str_mv | 10.1103/PhysRevLett.107.143001 |
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Broadband, high-resolution spectra with accurate relative intensities are recorded instantly. Free induction decay (FID) of atoms, polarized by the chirped pulse, at their Rydberg-Rydberg transition frequencies, is heterodyne detected, averaged in the time domain, and Fourier transformed into the frequency domain. Millimeter-wave transient nutations are observed, and the possibility of FID evolving to superradiance is discussed.</description><subject>ALKALINE EARTH METALS</subject><subject>ATOMIC AND MOLECULAR PHYSICS</subject><subject>ATOMIC BEAMS</subject><subject>BEAMS</subject><subject>CALCIUM</subject><subject>CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS</subject><subject>DECAY</subject><subject>ELEMENTS</subject><subject>EMISSION</subject><subject>ENERGY LEVELS</subject><subject>ENERGY-LEVEL TRANSITIONS</subject><subject>EXCITED STATES</subject><subject>METALS</subject><subject>NUCLEAR DECAY</subject><subject>PHOTON EMISSION</subject><subject>PULSES</subject><subject>RYDBERG STATES</subject><subject>SPECTRA</subject><subject>SPECTROSCOPY</subject><subject>STIMULATED EMISSION</subject><subject>SUPERRADIANCE</subject><issn>0031-9007</issn><issn>1079-7114</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2011</creationdate><recordtype>article</recordtype><recordid>eNpNkFtLAzEQhYMotlb_QlnwwaetmewlyaMUL4WCUvQ57GZnbWRvJtlK_72RVvFpmOE7Z2YOIXOgCwCa3L5s926DuzV6vwDKF5AmlMIJmYZGxhwgPSVTShOIJaV8Qi6c-6CBYLk4JxPGAgaCT8lquTV2wCoexsZh1JqmMS16tPFXscPIDai97Z3uh33U19FmX5Vo3-NjjbwtOme86Tt3Sc7qInhcHeuMvD3cvy6f4vXz42p5t451InIfc5pVkFdAhda8rFHXSUZLzESa15JrlAxEWrCKCeS8FJmQDNMkS9O0zOqqqpMZuT749s4b5bTxqLe677pwqWKQA3DJA3VzoAbbf47ovGqN09g0RYf96JSkmcwZ4zKQ-YHU4U9nsVaDNW1h9wqo-sla_cs6zLg6ZB2E8-OKsWyx-pP9hpt8A9guffg</recordid><startdate>20110930</startdate><enddate>20110930</enddate><creator>Prozument, Kirill</creator><creator>Colombo, Anthony P</creator><creator>Zhou, Yan</creator><creator>Park, G Barratt</creator><creator>Petrović, Vladimir S</creator><creator>Coy, Stephen L</creator><creator>Field, Robert W</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>OTOTI</scope></search><sort><creationdate>20110930</creationdate><title>Chirped-pulse millimeter-wave spectroscopy of Rydberg-Rydberg transitions</title><author>Prozument, Kirill ; Colombo, Anthony P ; Zhou, Yan ; Park, G Barratt ; Petrović, Vladimir S ; Coy, Stephen L ; Field, Robert W</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c386t-705d16d108cc7bfecf350be5846f97ce92184a2d28e77b85892e435444b5fddf3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2011</creationdate><topic>ALKALINE EARTH METALS</topic><topic>ATOMIC AND MOLECULAR PHYSICS</topic><topic>ATOMIC BEAMS</topic><topic>BEAMS</topic><topic>CALCIUM</topic><topic>CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS</topic><topic>DECAY</topic><topic>ELEMENTS</topic><topic>EMISSION</topic><topic>ENERGY LEVELS</topic><topic>ENERGY-LEVEL TRANSITIONS</topic><topic>EXCITED STATES</topic><topic>METALS</topic><topic>NUCLEAR DECAY</topic><topic>PHOTON EMISSION</topic><topic>PULSES</topic><topic>RYDBERG STATES</topic><topic>SPECTRA</topic><topic>SPECTROSCOPY</topic><topic>STIMULATED EMISSION</topic><topic>SUPERRADIANCE</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Prozument, Kirill</creatorcontrib><creatorcontrib>Colombo, Anthony P</creatorcontrib><creatorcontrib>Zhou, Yan</creatorcontrib><creatorcontrib>Park, G Barratt</creatorcontrib><creatorcontrib>Petrović, Vladimir S</creatorcontrib><creatorcontrib>Coy, Stephen L</creatorcontrib><creatorcontrib>Field, Robert W</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>OSTI.GOV</collection><jtitle>Physical review letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Prozument, Kirill</au><au>Colombo, Anthony P</au><au>Zhou, Yan</au><au>Park, G Barratt</au><au>Petrović, Vladimir S</au><au>Coy, Stephen L</au><au>Field, Robert W</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Chirped-pulse millimeter-wave spectroscopy of Rydberg-Rydberg transitions</atitle><jtitle>Physical review letters</jtitle><addtitle>Phys Rev Lett</addtitle><date>2011-09-30</date><risdate>2011</risdate><volume>107</volume><issue>14</issue><spage>143001</spage><epage>143001</epage><pages>143001-143001</pages><artnum>143001</artnum><issn>0031-9007</issn><eissn>1079-7114</eissn><abstract>Transitions between Rydberg states of Ca atoms, in a pulsed, supersonic atomic beam, are directly detected by chirped-pulse millimeter-wave spectroscopy. Broadband, high-resolution spectra with accurate relative intensities are recorded instantly. Free induction decay (FID) of atoms, polarized by the chirped pulse, at their Rydberg-Rydberg transition frequencies, is heterodyne detected, averaged in the time domain, and Fourier transformed into the frequency domain. Millimeter-wave transient nutations are observed, and the possibility of FID evolving to superradiance is discussed.</abstract><cop>United States</cop><pmid>22107187</pmid><doi>10.1103/PhysRevLett.107.143001</doi><tpages>1</tpages><oa>free_for_read</oa></addata></record> |
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subjects | ALKALINE EARTH METALS ATOMIC AND MOLECULAR PHYSICS ATOMIC BEAMS BEAMS CALCIUM CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS DECAY ELEMENTS EMISSION ENERGY LEVELS ENERGY-LEVEL TRANSITIONS EXCITED STATES METALS NUCLEAR DECAY PHOTON EMISSION PULSES RYDBERG STATES SPECTRA SPECTROSCOPY STIMULATED EMISSION SUPERRADIANCE |
title | Chirped-pulse millimeter-wave spectroscopy of Rydberg-Rydberg transitions |
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