Tracking autoionizing-wave-packet dynamics at the 1-fs temporal scale
We present time-resolved studies and Fourier transform spectroscopy of inner-shell excited states undergoing Auger decay and doubly excited autoionizing states, utilizing coherent extreme-ultraviolet (XUV) radiation continua. Series of states spanning a range of ∼4 eV are excited simultaneously. An...
Gespeichert in:
| Veröffentlicht in: | Physical review letters 2010-07, Vol.105 (4), p.043902-043902, Article 043902 |
|---|---|
| Hauptverfasser: | , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 043902 |
|---|---|
| container_issue | 4 |
| container_start_page | 043902 |
| container_title | Physical review letters |
| container_volume | 105 |
| creator | Skantzakis, E Tzallas, P Kruse, J E Kalpouzos, C Faucher, O Tsakiris, G D Charalambidis, D |
| description | We present time-resolved studies and Fourier transform spectroscopy of inner-shell excited states undergoing Auger decay and doubly excited autoionizing states, utilizing coherent extreme-ultraviolet (XUV) radiation continua. Series of states spanning a range of ∼4 eV are excited simultaneously. An XUV probe pulse tracks the oscillatory and decaying evolution of the formed wave packet. The Fourier transform of the measured trace reproduces the spectrum of the series. The present work paves the way for ultrabroadband XUV spectroscopy and studies of ultrafast dynamics in all states of matter. |
| doi_str_mv | 10.1103/physrevlett.105.043902 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_osti_</sourceid><recordid>TN_cdi_osti_scitechconnect_21410935</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>755404819</sourcerecordid><originalsourceid>FETCH-LOGICAL-c505t-b21317fed96691c3655823c6192b790a63ae520bc375fa9a95265bd6273bc78d3</originalsourceid><addsrcrecordid>eNo9kE1rGzEQhkVoiN0kf8Es9NDTujPSSlodi0nSgqEhJGeh1c7G2-5XV7KL8-ujYrenYWaedwYexlYIa0QQX6bdMcx06CjGNYJcQyEM8Au2RNAm14jFB7YEEJgbAL1gH0P4CQDIVXnFFhxKpcuiWLK759n5X-3wmrl9HNtxaN9Sk_9xB8qntKGY1cfB9a0PmYtZ3FGGeROySP00zq7Lgncd3bDLxnWBbs_1mr3c3z1vvuXbHw_fN1-3uZcgY15xFKgbqo1SBr1QUpZceIWGV9qAU8KR5FB5oWXjjDOSK1nVimtReV3W4pp9Ot0dQ2xt8G0kv_PjMJCPlmOBYIRM1OcTNc3j7z2FaPs2eOo6N9C4D1ZLWUBRokmkOpF-HkPy2dhpbns3Hy2C_evZPibPT3TYJs9pJu3Jcwquzi_2VU_1_9g_seIdVRF7BA</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>755404819</pqid></control><display><type>article</type><title>Tracking autoionizing-wave-packet dynamics at the 1-fs temporal scale</title><source>American Physical Society Journals</source><creator>Skantzakis, E ; Tzallas, P ; Kruse, J E ; Kalpouzos, C ; Faucher, O ; Tsakiris, G D ; Charalambidis, D</creator><creatorcontrib>Skantzakis, E ; Tzallas, P ; Kruse, J E ; Kalpouzos, C ; Faucher, O ; Tsakiris, G D ; Charalambidis, D</creatorcontrib><description>We present time-resolved studies and Fourier transform spectroscopy of inner-shell excited states undergoing Auger decay and doubly excited autoionizing states, utilizing coherent extreme-ultraviolet (XUV) radiation continua. Series of states spanning a range of ∼4 eV are excited simultaneously. An XUV probe pulse tracks the oscillatory and decaying evolution of the formed wave packet. The Fourier transform of the measured trace reproduces the spectrum of the series. The present work paves the way for ultrabroadband XUV spectroscopy and studies of ultrafast dynamics in all states of matter.</description><identifier>ISSN: 0031-9007</identifier><identifier>EISSN: 1079-7114</identifier><identifier>DOI: 10.1103/physrevlett.105.043902</identifier><identifier>PMID: 20867844</identifier><language>eng</language><publisher>United States</publisher><subject>ATOMIC AND MOLECULAR PHYSICS ; ELECTROMAGNETIC RADIATION ; ENERGY LEVELS ; ENERGY RANGE ; ENERGY-LEVEL TRANSITIONS ; EV RANGE ; EXCITATION ; EXCITED STATES ; EXTREME ULTRAVIOLET RADIATION ; FOURIER TRANSFORM SPECTROMETERS ; FOURIER TRANSFORMATION ; INNER-SHELL EXCITATION ; INTEGRAL TRANSFORMATIONS ; MEASURING INSTRUMENTS ; PULSES ; RADIATIONS ; RESOLUTION ; SPECTROMETERS ; SPECTROSCOPY ; TIME RESOLUTION ; TIMING PROPERTIES ; TRANSFORMATIONS ; ULTRAVIOLET RADIATION ; WAVE PACKETS</subject><ispartof>Physical review letters, 2010-07, Vol.105 (4), p.043902-043902, Article 043902</ispartof><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c505t-b21317fed96691c3655823c6192b790a63ae520bc375fa9a95265bd6273bc78d3</citedby><cites>FETCH-LOGICAL-c505t-b21317fed96691c3655823c6192b790a63ae520bc375fa9a95265bd6273bc78d3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,780,784,885,2876,2877,27924,27925</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/20867844$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/biblio/21410935$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Skantzakis, E</creatorcontrib><creatorcontrib>Tzallas, P</creatorcontrib><creatorcontrib>Kruse, J E</creatorcontrib><creatorcontrib>Kalpouzos, C</creatorcontrib><creatorcontrib>Faucher, O</creatorcontrib><creatorcontrib>Tsakiris, G D</creatorcontrib><creatorcontrib>Charalambidis, D</creatorcontrib><title>Tracking autoionizing-wave-packet dynamics at the 1-fs temporal scale</title><title>Physical review letters</title><addtitle>Phys Rev Lett</addtitle><description>We present time-resolved studies and Fourier transform spectroscopy of inner-shell excited states undergoing Auger decay and doubly excited autoionizing states, utilizing coherent extreme-ultraviolet (XUV) radiation continua. Series of states spanning a range of ∼4 eV are excited simultaneously. An XUV probe pulse tracks the oscillatory and decaying evolution of the formed wave packet. The Fourier transform of the measured trace reproduces the spectrum of the series. The present work paves the way for ultrabroadband XUV spectroscopy and studies of ultrafast dynamics in all states of matter.</description><subject>ATOMIC AND MOLECULAR PHYSICS</subject><subject>ELECTROMAGNETIC RADIATION</subject><subject>ENERGY LEVELS</subject><subject>ENERGY RANGE</subject><subject>ENERGY-LEVEL TRANSITIONS</subject><subject>EV RANGE</subject><subject>EXCITATION</subject><subject>EXCITED STATES</subject><subject>EXTREME ULTRAVIOLET RADIATION</subject><subject>FOURIER TRANSFORM SPECTROMETERS</subject><subject>FOURIER TRANSFORMATION</subject><subject>INNER-SHELL EXCITATION</subject><subject>INTEGRAL TRANSFORMATIONS</subject><subject>MEASURING INSTRUMENTS</subject><subject>PULSES</subject><subject>RADIATIONS</subject><subject>RESOLUTION</subject><subject>SPECTROMETERS</subject><subject>SPECTROSCOPY</subject><subject>TIME RESOLUTION</subject><subject>TIMING PROPERTIES</subject><subject>TRANSFORMATIONS</subject><subject>ULTRAVIOLET RADIATION</subject><subject>WAVE PACKETS</subject><issn>0031-9007</issn><issn>1079-7114</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2010</creationdate><recordtype>article</recordtype><recordid>eNo9kE1rGzEQhkVoiN0kf8Es9NDTujPSSlodi0nSgqEhJGeh1c7G2-5XV7KL8-ujYrenYWaedwYexlYIa0QQX6bdMcx06CjGNYJcQyEM8Au2RNAm14jFB7YEEJgbAL1gH0P4CQDIVXnFFhxKpcuiWLK759n5X-3wmrl9HNtxaN9Sk_9xB8qntKGY1cfB9a0PmYtZ3FGGeROySP00zq7Lgncd3bDLxnWBbs_1mr3c3z1vvuXbHw_fN1-3uZcgY15xFKgbqo1SBr1QUpZceIWGV9qAU8KR5FB5oWXjjDOSK1nVimtReV3W4pp9Ot0dQ2xt8G0kv_PjMJCPlmOBYIRM1OcTNc3j7z2FaPs2eOo6N9C4D1ZLWUBRokmkOpF-HkPy2dhpbns3Hy2C_evZPibPT3TYJs9pJu3Jcwquzi_2VU_1_9g_seIdVRF7BA</recordid><startdate>20100723</startdate><enddate>20100723</enddate><creator>Skantzakis, E</creator><creator>Tzallas, P</creator><creator>Kruse, J E</creator><creator>Kalpouzos, C</creator><creator>Faucher, O</creator><creator>Tsakiris, G D</creator><creator>Charalambidis, D</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>OTOTI</scope></search><sort><creationdate>20100723</creationdate><title>Tracking autoionizing-wave-packet dynamics at the 1-fs temporal scale</title><author>Skantzakis, E ; Tzallas, P ; Kruse, J E ; Kalpouzos, C ; Faucher, O ; Tsakiris, G D ; Charalambidis, D</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c505t-b21317fed96691c3655823c6192b790a63ae520bc375fa9a95265bd6273bc78d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2010</creationdate><topic>ATOMIC AND MOLECULAR PHYSICS</topic><topic>ELECTROMAGNETIC RADIATION</topic><topic>ENERGY LEVELS</topic><topic>ENERGY RANGE</topic><topic>ENERGY-LEVEL TRANSITIONS</topic><topic>EV RANGE</topic><topic>EXCITATION</topic><topic>EXCITED STATES</topic><topic>EXTREME ULTRAVIOLET RADIATION</topic><topic>FOURIER TRANSFORM SPECTROMETERS</topic><topic>FOURIER TRANSFORMATION</topic><topic>INNER-SHELL EXCITATION</topic><topic>INTEGRAL TRANSFORMATIONS</topic><topic>MEASURING INSTRUMENTS</topic><topic>PULSES</topic><topic>RADIATIONS</topic><topic>RESOLUTION</topic><topic>SPECTROMETERS</topic><topic>SPECTROSCOPY</topic><topic>TIME RESOLUTION</topic><topic>TIMING PROPERTIES</topic><topic>TRANSFORMATIONS</topic><topic>ULTRAVIOLET RADIATION</topic><topic>WAVE PACKETS</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Skantzakis, E</creatorcontrib><creatorcontrib>Tzallas, P</creatorcontrib><creatorcontrib>Kruse, J E</creatorcontrib><creatorcontrib>Kalpouzos, C</creatorcontrib><creatorcontrib>Faucher, O</creatorcontrib><creatorcontrib>Tsakiris, G D</creatorcontrib><creatorcontrib>Charalambidis, D</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>OSTI.GOV</collection><jtitle>Physical review letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Skantzakis, E</au><au>Tzallas, P</au><au>Kruse, J E</au><au>Kalpouzos, C</au><au>Faucher, O</au><au>Tsakiris, G D</au><au>Charalambidis, D</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Tracking autoionizing-wave-packet dynamics at the 1-fs temporal scale</atitle><jtitle>Physical review letters</jtitle><addtitle>Phys Rev Lett</addtitle><date>2010-07-23</date><risdate>2010</risdate><volume>105</volume><issue>4</issue><spage>043902</spage><epage>043902</epage><pages>043902-043902</pages><artnum>043902</artnum><issn>0031-9007</issn><eissn>1079-7114</eissn><abstract>We present time-resolved studies and Fourier transform spectroscopy of inner-shell excited states undergoing Auger decay and doubly excited autoionizing states, utilizing coherent extreme-ultraviolet (XUV) radiation continua. Series of states spanning a range of ∼4 eV are excited simultaneously. An XUV probe pulse tracks the oscillatory and decaying evolution of the formed wave packet. The Fourier transform of the measured trace reproduces the spectrum of the series. The present work paves the way for ultrabroadband XUV spectroscopy and studies of ultrafast dynamics in all states of matter.</abstract><cop>United States</cop><pmid>20867844</pmid><doi>10.1103/physrevlett.105.043902</doi><tpages>1</tpages><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0031-9007 |
| ispartof | Physical review letters, 2010-07, Vol.105 (4), p.043902-043902, Article 043902 |
| issn | 0031-9007 1079-7114 |
| language | eng |
| recordid | cdi_osti_scitechconnect_21410935 |
| source | American Physical Society Journals |
| subjects | ATOMIC AND MOLECULAR PHYSICS ELECTROMAGNETIC RADIATION ENERGY LEVELS ENERGY RANGE ENERGY-LEVEL TRANSITIONS EV RANGE EXCITATION EXCITED STATES EXTREME ULTRAVIOLET RADIATION FOURIER TRANSFORM SPECTROMETERS FOURIER TRANSFORMATION INNER-SHELL EXCITATION INTEGRAL TRANSFORMATIONS MEASURING INSTRUMENTS PULSES RADIATIONS RESOLUTION SPECTROMETERS SPECTROSCOPY TIME RESOLUTION TIMING PROPERTIES TRANSFORMATIONS ULTRAVIOLET RADIATION WAVE PACKETS |
| title | Tracking autoionizing-wave-packet dynamics at the 1-fs temporal scale |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-28T02%3A30%3A52IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_osti_&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Tracking%20autoionizing-wave-packet%20dynamics%20at%20the%201-fs%20temporal%20scale&rft.jtitle=Physical%20review%20letters&rft.au=Skantzakis,%20E&rft.date=2010-07-23&rft.volume=105&rft.issue=4&rft.spage=043902&rft.epage=043902&rft.pages=043902-043902&rft.artnum=043902&rft.issn=0031-9007&rft.eissn=1079-7114&rft_id=info:doi/10.1103/physrevlett.105.043902&rft_dat=%3Cproquest_osti_%3E755404819%3C/proquest_osti_%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=755404819&rft_id=info:pmid/20867844&rfr_iscdi=true |