Molecular-frame angular distributions of resonant CO:C(1s) Auger electrons

The molecular-frame angular distributions of resonantly excited CO:C(1s) --> pi* Auger electrons were determined using angle-resolved electron-ion coincidence spectroscopy in combination with a novel transformation procedure. Our new methodology yields full three-dimensional electron angular dist...

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Veröffentlicht in:Physical review letters 2008-12, Vol.101 (26), p.263002-263002, Article 263002
Hauptverfasser: Rolles, D, Prümper, G, Fukuzawa, H, Liu, X J, Pesić, Z D, Fink, R F, Grum-Grzhimailo, A N, Dumitriu, I, Berrah, N, Ueda, K
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container_end_page 263002
container_issue 26
container_start_page 263002
container_title Physical review letters
container_volume 101
creator Rolles, D
Prümper, G
Fukuzawa, H
Liu, X J
Pesić, Z D
Fink, R F
Grum-Grzhimailo, A N
Dumitriu, I
Berrah, N
Ueda, K
description The molecular-frame angular distributions of resonantly excited CO:C(1s) --> pi* Auger electrons were determined using angle-resolved electron-ion coincidence spectroscopy in combination with a novel transformation procedure. Our new methodology yields full three-dimensional electron angular distributions with high energy resolution from the measurement of electrons at only two angles. The experimentally determined distributions are well reproduced by calculations performed in a simple one-center approximation, allowing an unambiguous identification of several overlapping Auger lines.
doi_str_mv 10.1103/PhysRevLett.101.263002
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source American Physical Society Journals
subjects ANGULAR DISTRIBUTION
APPROXIMATIONS
ATOMIC AND MOLECULAR PHYSICS
AUGER ELECTRON SPECTROSCOPY
ELECTRONS
ENERGY RESOLUTION
ION SPECTROSCOPY
title Molecular-frame angular distributions of resonant CO:C(1s) Auger electrons
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