Ex Situ Aqueous Mineral Carbonation
The U.S. Department of Energy's National Energy Technology Laboratory (NETL) located in Albany, OR (formerly the Albany Research Center) has studied ex situ mineral carbonation as a potential option for carbon dioxide sequestration. Studies focused on the reaction of Ca−, Fe−, and Mg−silicate m...
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| Veröffentlicht in: | Environmental science & technology 2007-04, Vol.41 (7), p.2587-2593 |
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| creator | Gerdemann, Stephen J O'Connor, William K Dahlin, David C Penner, Larry R Rush, Hank |
| description | The U.S. Department of Energy's National Energy Technology Laboratory (NETL) located in Albany, OR (formerly the Albany Research Center) has studied ex situ mineral carbonation as a potential option for carbon dioxide sequestration. Studies focused on the reaction of Ca−, Fe−, and Mg−silicate minerals with gaseous CO2 to form geologically stable, naturally occurring solid carbonate minerals. The research included resource evaluation, kinetic studies, process development, and economic evaluation. An initial cost estimate of ∼$69/ton of CO2 sequestered was improved with process improvements to ∼$54/ton. The scale of ex situ mineral carbonation operations, requiring ∼55 000 tons of mineral to carbonate, the daily CO2 emissions from a 1-GW, coal-fired power plant, may make such operations impractical. |
| doi_str_mv | 10.1021/es0619253 |
| format | Article |
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Studies focused on the reaction of Ca−, Fe−, and Mg−silicate minerals with gaseous CO2 to form geologically stable, naturally occurring solid carbonate minerals. The research included resource evaluation, kinetic studies, process development, and economic evaluation. An initial cost estimate of ∼$69/ton of CO2 sequestered was improved with process improvements to ∼$54/ton. The scale of ex situ mineral carbonation operations, requiring ∼55 000 tons of mineral to carbonate, the daily CO2 emissions from a 1-GW, coal-fired power plant, may make such operations impractical.</description><identifier>ISSN: 0013-936X</identifier><identifier>EISSN: 1520-5851</identifier><identifier>DOI: 10.1021/es0619253</identifier><identifier>PMID: 17438820</identifier><identifier>CODEN: ESTHAG</identifier><language>eng</language><publisher>Washington, DC: American Chemical Society</publisher><subject>01 COAL, LIGNITE, AND PEAT ; Air Pollutants - chemistry ; Applied sciences ; Atmospheric pollution ; BENCH-SCALE EXPERIMENTS ; CALCIUM SILICATES ; CARBON DIOXIDE ; Carbon Dioxide - chemistry ; CARBON SEQUESTRATION ; CARBONATES ; Carbonates - chemical synthesis ; Chemical reactions ; Chemistry ; Climatology. Bioclimatology. Climate change ; COAL ; Coal-fired power plants ; Cost estimates ; COST ESTIMATION ; Earth, ocean, space ; ECONOMIC ANALYSIS ; ELECTRIC POWER ; Environmental Restoration and Remediation - economics ; Environmental Restoration and Remediation - instrumentation ; Environmental Restoration and Remediation - methods ; ENVIRONMENTAL SCIENCES ; Evaluation Studies as Topic ; Exact sciences and technology ; External geophysics ; FOSSIL-FUEL POWER PLANTS ; General processes of purification and dust removal ; IRON SILICATES ; KINETICS ; MAGNESIUM SILICATES ; Meteorology ; MINERALIZATION ; Minerals ; Minerals - chemistry ; Pollution ; Prevention and purification methods ; PRICES ; RESOURCE ASSESSMENT ; SILICATE MINERALS ; Silicates - chemistry ; USA</subject><ispartof>Environmental science & technology, 2007-04, Vol.41 (7), p.2587-2593</ispartof><rights>Copyright © 2007 American Chemical Society</rights><rights>2007 INIST-CNRS</rights><rights>Copyright American Chemical Society Apr 1, 2007</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a498t-a15266488f0f07c7b3952d2bb1b03178ecfa9a4d5f3d130b222957f8e3d7ca773</citedby><cites>FETCH-LOGICAL-a498t-a15266488f0f07c7b3952d2bb1b03178ecfa9a4d5f3d130b222957f8e3d7ca773</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/es0619253$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/es0619253$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>230,314,776,780,881,2752,27053,27901,27902,56713,56763</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=18664818$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/17438820$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/biblio/20885852$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Gerdemann, Stephen J</creatorcontrib><creatorcontrib>O'Connor, William K</creatorcontrib><creatorcontrib>Dahlin, David C</creatorcontrib><creatorcontrib>Penner, Larry R</creatorcontrib><creatorcontrib>Rush, Hank</creatorcontrib><title>Ex Situ Aqueous Mineral Carbonation</title><title>Environmental science & technology</title><addtitle>Environ. Sci. Technol</addtitle><description>The U.S. Department of Energy's National Energy Technology Laboratory (NETL) located in Albany, OR (formerly the Albany Research Center) has studied ex situ mineral carbonation as a potential option for carbon dioxide sequestration. Studies focused on the reaction of Ca−, Fe−, and Mg−silicate minerals with gaseous CO2 to form geologically stable, naturally occurring solid carbonate minerals. The research included resource evaluation, kinetic studies, process development, and economic evaluation. An initial cost estimate of ∼$69/ton of CO2 sequestered was improved with process improvements to ∼$54/ton. The scale of ex situ mineral carbonation operations, requiring ∼55 000 tons of mineral to carbonate, the daily CO2 emissions from a 1-GW, coal-fired power plant, may make such operations impractical.</description><subject>01 COAL, LIGNITE, AND PEAT</subject><subject>Air Pollutants - chemistry</subject><subject>Applied sciences</subject><subject>Atmospheric pollution</subject><subject>BENCH-SCALE EXPERIMENTS</subject><subject>CALCIUM SILICATES</subject><subject>CARBON DIOXIDE</subject><subject>Carbon Dioxide - chemistry</subject><subject>CARBON SEQUESTRATION</subject><subject>CARBONATES</subject><subject>Carbonates - chemical synthesis</subject><subject>Chemical reactions</subject><subject>Chemistry</subject><subject>Climatology. Bioclimatology. Climate change</subject><subject>COAL</subject><subject>Coal-fired power plants</subject><subject>Cost estimates</subject><subject>COST ESTIMATION</subject><subject>Earth, ocean, space</subject><subject>ECONOMIC ANALYSIS</subject><subject>ELECTRIC POWER</subject><subject>Environmental Restoration and Remediation - economics</subject><subject>Environmental Restoration and Remediation - instrumentation</subject><subject>Environmental Restoration and Remediation - methods</subject><subject>ENVIRONMENTAL SCIENCES</subject><subject>Evaluation Studies as Topic</subject><subject>Exact sciences and technology</subject><subject>External geophysics</subject><subject>FOSSIL-FUEL POWER PLANTS</subject><subject>General processes of purification and dust removal</subject><subject>IRON SILICATES</subject><subject>KINETICS</subject><subject>MAGNESIUM SILICATES</subject><subject>Meteorology</subject><subject>MINERALIZATION</subject><subject>Minerals</subject><subject>Minerals - chemistry</subject><subject>Pollution</subject><subject>Prevention and purification methods</subject><subject>PRICES</subject><subject>RESOURCE ASSESSMENT</subject><subject>SILICATE MINERALS</subject><subject>Silicates - chemistry</subject><subject>USA</subject><issn>0013-936X</issn><issn>1520-5851</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2007</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqF0U1LxDAQBuAgiq4fB_-ALIqCh-pM0jTpURZ1lRUFFbyFNE0x2m3XpAX992bZxQU9eMohDzPzzhCyj3CGQPHcBsgwp5ytkQFyCgmXHNfJAABZkrPsZYtsh_AGAJSB3CRbKFImJYUBObr8HD66rh9efPS27cPwzjXW63o40r5oG925ttklG5Wug91bvjvk-eryaTROJvfXN6OLSaLTXHaJjq2zLJWyggqEEQXLOS1pUWABDIW0ptK5TktesRIZFJTSnItKWlYKo4VgO-RoUbcNnVPBuM6aV9M2jTWdoiBljEWjOlmomW_jzKFTUxeMrWvdzANEyHnOIP8XYiqRMyEjPPwF39reNzGqivvClCGwiE4XyPg2BG8rNfNuqv2XQlDzK6ifK0R7sCzYF1NbruRy7REcL4EORteV141xYeXkfI84nyxZOBc6-_nzr_27ygQTXD09PKqrFMd0cjtR41VdbcIqxN8BvwFUraUQ</recordid><startdate>20070401</startdate><enddate>20070401</enddate><creator>Gerdemann, Stephen J</creator><creator>O'Connor, William K</creator><creator>Dahlin, David C</creator><creator>Penner, Larry R</creator><creator>Rush, Hank</creator><general>American Chemical Society</general><scope>BSCLL</scope><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QO</scope><scope>7ST</scope><scope>7T7</scope><scope>7U7</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>P64</scope><scope>SOI</scope><scope>7TV</scope><scope>7U6</scope><scope>OTOTI</scope></search><sort><creationdate>20070401</creationdate><title>Ex Situ Aqueous Mineral Carbonation</title><author>Gerdemann, Stephen J ; O'Connor, William K ; Dahlin, David C ; Penner, Larry R ; Rush, Hank</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a498t-a15266488f0f07c7b3952d2bb1b03178ecfa9a4d5f3d130b222957f8e3d7ca773</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2007</creationdate><topic>01 COAL, LIGNITE, AND PEAT</topic><topic>Air Pollutants - chemistry</topic><topic>Applied sciences</topic><topic>Atmospheric pollution</topic><topic>BENCH-SCALE EXPERIMENTS</topic><topic>CALCIUM SILICATES</topic><topic>CARBON DIOXIDE</topic><topic>Carbon Dioxide - chemistry</topic><topic>CARBON SEQUESTRATION</topic><topic>CARBONATES</topic><topic>Carbonates - chemical synthesis</topic><topic>Chemical reactions</topic><topic>Chemistry</topic><topic>Climatology. Bioclimatology. Climate change</topic><topic>COAL</topic><topic>Coal-fired power plants</topic><topic>Cost estimates</topic><topic>COST ESTIMATION</topic><topic>Earth, ocean, space</topic><topic>ECONOMIC ANALYSIS</topic><topic>ELECTRIC POWER</topic><topic>Environmental Restoration and Remediation - economics</topic><topic>Environmental Restoration and Remediation - instrumentation</topic><topic>Environmental Restoration and Remediation - methods</topic><topic>ENVIRONMENTAL SCIENCES</topic><topic>Evaluation Studies as Topic</topic><topic>Exact sciences and technology</topic><topic>External geophysics</topic><topic>FOSSIL-FUEL POWER PLANTS</topic><topic>General processes of purification and dust removal</topic><topic>IRON SILICATES</topic><topic>KINETICS</topic><topic>MAGNESIUM SILICATES</topic><topic>Meteorology</topic><topic>MINERALIZATION</topic><topic>Minerals</topic><topic>Minerals - chemistry</topic><topic>Pollution</topic><topic>Prevention and purification methods</topic><topic>PRICES</topic><topic>RESOURCE ASSESSMENT</topic><topic>SILICATE MINERALS</topic><topic>Silicates - chemistry</topic><topic>USA</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Gerdemann, Stephen J</creatorcontrib><creatorcontrib>O'Connor, William K</creatorcontrib><creatorcontrib>Dahlin, David C</creatorcontrib><creatorcontrib>Penner, Larry R</creatorcontrib><creatorcontrib>Rush, Hank</creatorcontrib><collection>Istex</collection><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Biotechnology Research Abstracts</collection><collection>Environment Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Toxicology Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Environment Abstracts</collection><collection>Pollution Abstracts</collection><collection>Sustainability Science Abstracts</collection><collection>OSTI.GOV</collection><jtitle>Environmental science & technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Gerdemann, Stephen J</au><au>O'Connor, William K</au><au>Dahlin, David C</au><au>Penner, Larry R</au><au>Rush, Hank</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Ex Situ Aqueous Mineral Carbonation</atitle><jtitle>Environmental science & technology</jtitle><addtitle>Environ. Sci. Technol</addtitle><date>2007-04-01</date><risdate>2007</risdate><volume>41</volume><issue>7</issue><spage>2587</spage><epage>2593</epage><pages>2587-2593</pages><issn>0013-936X</issn><eissn>1520-5851</eissn><coden>ESTHAG</coden><abstract>The U.S. Department of Energy's National Energy Technology Laboratory (NETL) located in Albany, OR (formerly the Albany Research Center) has studied ex situ mineral carbonation as a potential option for carbon dioxide sequestration. Studies focused on the reaction of Ca−, Fe−, and Mg−silicate minerals with gaseous CO2 to form geologically stable, naturally occurring solid carbonate minerals. The research included resource evaluation, kinetic studies, process development, and economic evaluation. An initial cost estimate of ∼$69/ton of CO2 sequestered was improved with process improvements to ∼$54/ton. The scale of ex situ mineral carbonation operations, requiring ∼55 000 tons of mineral to carbonate, the daily CO2 emissions from a 1-GW, coal-fired power plant, may make such operations impractical.</abstract><cop>Washington, DC</cop><pub>American Chemical Society</pub><pmid>17438820</pmid><doi>10.1021/es0619253</doi><tpages>7</tpages></addata></record> |
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| identifier | ISSN: 0013-936X |
| ispartof | Environmental science & technology, 2007-04, Vol.41 (7), p.2587-2593 |
| issn | 0013-936X 1520-5851 |
| language | eng |
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| source | ACS Publications; MEDLINE |
| subjects | 01 COAL, LIGNITE, AND PEAT Air Pollutants - chemistry Applied sciences Atmospheric pollution BENCH-SCALE EXPERIMENTS CALCIUM SILICATES CARBON DIOXIDE Carbon Dioxide - chemistry CARBON SEQUESTRATION CARBONATES Carbonates - chemical synthesis Chemical reactions Chemistry Climatology. Bioclimatology. Climate change COAL Coal-fired power plants Cost estimates COST ESTIMATION Earth, ocean, space ECONOMIC ANALYSIS ELECTRIC POWER Environmental Restoration and Remediation - economics Environmental Restoration and Remediation - instrumentation Environmental Restoration and Remediation - methods ENVIRONMENTAL SCIENCES Evaluation Studies as Topic Exact sciences and technology External geophysics FOSSIL-FUEL POWER PLANTS General processes of purification and dust removal IRON SILICATES KINETICS MAGNESIUM SILICATES Meteorology MINERALIZATION Minerals Minerals - chemistry Pollution Prevention and purification methods PRICES RESOURCE ASSESSMENT SILICATE MINERALS Silicates - chemistry USA |
| title | Ex Situ Aqueous Mineral Carbonation |
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