Spin glass or random anisotropy?: The origin of magnetically glassy behavior in nanostructured GdAl{sub 2}

Initially crystalline GdAl{sub 2} was mechanically milled for long times to produce a highly chemically disordered phase with approximately 8-nm grains. Analysis of dc magnetization measurements using an Arrott plot and the approach to saturation suggest the presence of significant random anisotropy...

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Veröffentlicht in:Journal of applied physics 2005-05, Vol.97 (10)
Hauptverfasser: Shand, P.M., Stark, C.C., Williams, D., Morales, M.A., Pekarek, T.M., Leslie-Pelecky, D.L., Department of Physics and Astronomy and Center for Materials Research and Analysis, University of Nebraska-Lincoln, Lincoln, Nebraska 68588-0111, Department of Chemistry and Physics, University of North Florida, 4567 St. John's Bluff Road South, Jacksonville, Florida 32224
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container_issue 10
container_start_page
container_title Journal of applied physics
container_volume 97
creator Shand, P.M.
Stark, C.C.
Williams, D.
Morales, M.A.
Pekarek, T.M.
Leslie-Pelecky, D.L.
Department of Physics and Astronomy and Center for Materials Research and Analysis, University of Nebraska-Lincoln, Lincoln, Nebraska 68588-0111
Department of Chemistry and Physics, University of North Florida, 4567 St. John's Bluff Road South, Jacksonville, Florida 32224
Department of Physics and Astronomy and Center for Materials Research and Analysis, University of Nebraska-Lincoln, Lincoln, Nebraska 68588-0111
description Initially crystalline GdAl{sub 2} was mechanically milled for long times to produce a highly chemically disordered phase with approximately 8-nm grains. Analysis of dc magnetization measurements using an Arrott plot and the approach to saturation suggest the presence of significant random anisotropy. ac susceptibility measurements showed that the shift in the peak temperature with frequency usually seen in magnetically glassy and superparamagnetic systems was virtually undetectable in the 10-1000-Hz frequency range. Based on these results, we believe that this material represents an interacting system with random anisotropy, where the anisotropy is the result of surface and interface asymmetries.
doi_str_mv 10.1063/1.1853003
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ispartof Journal of applied physics, 2005-05, Vol.97 (10)
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language eng
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source AIP Journals Complete; AIP Digital Archive
subjects ALUMINIUM ALLOYS
ANISOTROPY
ASYMMETRY
FERROMAGNETIC MATERIALS
GADOLINIUM ALLOYS
HZ RANGE
INTERFACES
MAGNETIC SUSCEPTIBILITY
MAGNETIZATION
MATERIALS SCIENCE
METALLIC GLASSES
MILLING
NANOSTRUCTURES
RANDOMNESS
SPIN GLASS STATE
SUPERPARAMAGNETISM
title Spin glass or random anisotropy?: The origin of magnetically glassy behavior in nanostructured GdAl{sub 2}
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