Effects of focal volume and spatial inhomogeneity on uncertainty in single-aerosol laser-induced breakdown spectroscopy measurements
Particle location with respect to the plasma volume and the focal volume of the collection optics is identified as an important source of uncertainty in single-aerosol laser-induced breakdown spectroscopy (LIBS) measurements. Two sets of optics were used to image different regions of a LIBS plasma a...
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Veröffentlicht in: | Applied physics letters 2005-07, Vol.87 (1) |
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creator | Lithgow, G. A. Buckley, S. G. |
description | Particle location with respect to the plasma volume and the focal volume of the collection optics is identified as an important source of uncertainty in single-aerosol laser-induced breakdown spectroscopy (LIBS) measurements. Two sets of optics were used to image different regions of a LIBS plasma and simultaneously collect spectra from single particles. Strong variation and lack of correlation between the two measurement channels suggest that emission from a single particle is localized within the plasma. Measurement precision and detection efficiency were improved by imaging a larger plasma region, thus integrating the spatially distributed signal. |
doi_str_mv | 10.1063/1.1984086 |
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A.</creatorcontrib><creatorcontrib>Buckley, S. G.</creatorcontrib><title>Effects of focal volume and spatial inhomogeneity on uncertainty in single-aerosol laser-induced breakdown spectroscopy measurements</title><title>Applied physics letters</title><description>Particle location with respect to the plasma volume and the focal volume of the collection optics is identified as an important source of uncertainty in single-aerosol laser-induced breakdown spectroscopy (LIBS) measurements. Two sets of optics were used to image different regions of a LIBS plasma and simultaneously collect spectra from single particles. Strong variation and lack of correlation between the two measurement channels suggest that emission from a single particle is localized within the plasma. Measurement precision and detection efficiency were improved by imaging a larger plasma region, thus integrating the spatially distributed signal.</description><subject>70 PLASMA PHYSICS AND FUSION TECHNOLOGY</subject><subject>AEROSOLS</subject><subject>BREAKDOWN</subject><subject>CORRELATIONS</subject><subject>LASERS</subject><subject>OPTICS</subject><subject>PARTICLES</subject><subject>PLASMA</subject><subject>PLASMA DIAGNOSTICS</subject><subject>PLASMA PRODUCTION</subject><subject>SPECTROSCOPY</subject><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2005</creationdate><recordtype>article</recordtype><recordid>eNotkEtLxDAUhYMoOI4u_AcBVy465tE07VKG8QEDbnRd0vRmJtomJUmV2fvDjcysDufwce_hIHRLyYqSij_QFW3qktTVGVpQImXBKa3P0YIQwouqEfQSXcX4ma1gnC_Q78YY0Clib7DxWg342w_zCFi5HsdJJZsj6_Z-9DtwYNMBe4dnpyEkZV221uFo3W6AQkHw0Q94UBFCYV0_a-hxF0B99f4nY1P-lBHtpwMeQcU5wAguxWt0YdQQ4eakS_TxtHlfvxTbt-fX9eO20EzIVHQSaCUUyI6KitQgG60bKlnX9dxUJbC-Ak1Ib5TWHRO6Fg2XEgRTpepq2vAlujve9THZNmqbQO-1dy73ahmRhAlRZur-SOncNQYw7RTsqMKhpaT9H7ml7Wlk_ge2hHJY</recordid><startdate>20050704</startdate><enddate>20050704</enddate><creator>Lithgow, G. A.</creator><creator>Buckley, S. G.</creator><scope>AAYXX</scope><scope>CITATION</scope><scope>OTOTI</scope></search><sort><creationdate>20050704</creationdate><title>Effects of focal volume and spatial inhomogeneity on uncertainty in single-aerosol laser-induced breakdown spectroscopy measurements</title><author>Lithgow, G. A. ; Buckley, S. G.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c257t-b7e165ae7b15608e79cc9172bbd3f64e2d6ec00dfaccb25c859377e52a4ab8193</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2005</creationdate><topic>70 PLASMA PHYSICS AND FUSION TECHNOLOGY</topic><topic>AEROSOLS</topic><topic>BREAKDOWN</topic><topic>CORRELATIONS</topic><topic>LASERS</topic><topic>OPTICS</topic><topic>PARTICLES</topic><topic>PLASMA</topic><topic>PLASMA DIAGNOSTICS</topic><topic>PLASMA PRODUCTION</topic><topic>SPECTROSCOPY</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Lithgow, G. A.</creatorcontrib><creatorcontrib>Buckley, S. G.</creatorcontrib><collection>CrossRef</collection><collection>OSTI.GOV</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lithgow, G. A.</au><au>Buckley, S. G.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effects of focal volume and spatial inhomogeneity on uncertainty in single-aerosol laser-induced breakdown spectroscopy measurements</atitle><jtitle>Applied physics letters</jtitle><date>2005-07-04</date><risdate>2005</risdate><volume>87</volume><issue>1</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><abstract>Particle location with respect to the plasma volume and the focal volume of the collection optics is identified as an important source of uncertainty in single-aerosol laser-induced breakdown spectroscopy (LIBS) measurements. Two sets of optics were used to image different regions of a LIBS plasma and simultaneously collect spectra from single particles. Strong variation and lack of correlation between the two measurement channels suggest that emission from a single particle is localized within the plasma. Measurement precision and detection efficiency were improved by imaging a larger plasma region, thus integrating the spatially distributed signal.</abstract><cop>United States</cop><doi>10.1063/1.1984086</doi></addata></record> |
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source | AIP Journals Complete; AIP Digital Archive |
subjects | 70 PLASMA PHYSICS AND FUSION TECHNOLOGY AEROSOLS BREAKDOWN CORRELATIONS LASERS OPTICS PARTICLES PLASMA PLASMA DIAGNOSTICS PLASMA PRODUCTION SPECTROSCOPY |
title | Effects of focal volume and spatial inhomogeneity on uncertainty in single-aerosol laser-induced breakdown spectroscopy measurements |
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