Electron scattering on stored mononucleotide anions
Collisions between electrons and deprotonated mononucleotides, AMP and UMP, were studied at the electrostatic storage ring ELISA where the two anions were stored with a 1/e lifetime of 13.5 s. It is found that the threshold energy for electron-induced reactions leading to production of neutral fragm...
Gespeichert in:
Veröffentlicht in: | Physical review. A, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 2004-08, Vol.70 (2), Article 020701 |
---|---|
Hauptverfasser: | , , , , , , |
Format: | Artikel |
Sprache: | eng |
Schlagworte: | |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
container_end_page | |
---|---|
container_issue | 2 |
container_start_page | |
container_title | Physical review. A, Atomic, molecular, and optical physics |
container_volume | 70 |
creator | Bluhme, H. Jensen, M. J. Nielsen, S. Brøndsted Pedersen, U. V. Seiersen, K. Svendsen, A. Andersen, L. H. |
description | Collisions between electrons and deprotonated mononucleotides, AMP and UMP, were studied at the electrostatic storage ring ELISA where the two anions were stored with a 1/e lifetime of 13.5 s. It is found that the threshold energy for electron-induced reactions leading to production of neutral fragments is as high as about 12 eV for both species. The high threshold is explained within the context of a classical reaction model, applicable for atomic anions, and a high electron-binding energy of about 5 eV for the two mononucleotides. There is no evidence in the cross sections for formation of short-lived doubly charged anions. |
doi_str_mv | 10.1103/PhysRevA.70.020701 |
format | Article |
fullrecord | <record><control><sourceid>crossref_osti_</sourceid><recordid>TN_cdi_osti_scitechconnect_20645831</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>10_1103_PhysRevA_70_020701</sourcerecordid><originalsourceid>FETCH-LOGICAL-c275t-256e61ecf94f02c581997aaacce6877b9b5db8936ac4582cf357db5c3f5593fd3</originalsourceid><addsrcrecordid>eNo1kEFLxDAQhYMouK7-AU8Fz10nSdM0x2VZXWFBET2HdJq4lW4iSRT239tSfZd5D94Mw0fILYUVpcDvXw6n9Gp_1isJK2AggZ6RBQVVlbRm7HzyAkqmKnlJrlL6hFFVoxaEbweLOQZfJDQ529j7j2JKOUTbFcfgg__GwYbcd7Ywvg8-XZMLZ4Zkb_7mkrw_bN82u3L__Pi0We9LZFLkkona1tSiU5UDhqKhSkljDKKtGylb1YqubRSvDVaiYei4kF0rkDshFHcdX5K7-W5IudcJ-2zxgMH78WPNoB63OB1bbG5hDClF6_RX7I8mnjQFPcHR_3C0BD3D4b-dWVm7</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Electron scattering on stored mononucleotide anions</title><source>American Physical Society Journals</source><creator>Bluhme, H. ; Jensen, M. J. ; Nielsen, S. Brøndsted ; Pedersen, U. V. ; Seiersen, K. ; Svendsen, A. ; Andersen, L. H.</creator><creatorcontrib>Bluhme, H. ; Jensen, M. J. ; Nielsen, S. Brøndsted ; Pedersen, U. V. ; Seiersen, K. ; Svendsen, A. ; Andersen, L. H.</creatorcontrib><description>Collisions between electrons and deprotonated mononucleotides, AMP and UMP, were studied at the electrostatic storage ring ELISA where the two anions were stored with a 1/e lifetime of 13.5 s. It is found that the threshold energy for electron-induced reactions leading to production of neutral fragments is as high as about 12 eV for both species. The high threshold is explained within the context of a classical reaction model, applicable for atomic anions, and a high electron-binding energy of about 5 eV for the two mononucleotides. There is no evidence in the cross sections for formation of short-lived doubly charged anions.</description><identifier>ISSN: 1050-2947</identifier><identifier>EISSN: 1094-1622</identifier><identifier>DOI: 10.1103/PhysRevA.70.020701</identifier><language>eng</language><publisher>United States</publisher><subject>AMP ; ANIONS ; ATOMIC AND MOLECULAR PHYSICS ; BINDING ENERGY ; BIOPHYSICS ; CHEMICAL BONDS ; CROSS SECTIONS ; DISSOCIATION ; DNA ; ELECTRON-MOLECULE COLLISIONS ; ELECTRONS ; EV RANGE ; LIFETIME ; SCATTERING ; STORAGE RINGS ; THRESHOLD ENERGY</subject><ispartof>Physical review. A, Atomic, molecular, and optical physics, 2004-08, Vol.70 (2), Article 020701</ispartof><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c275t-256e61ecf94f02c581997aaacce6877b9b5db8936ac4582cf357db5c3f5593fd3</citedby><cites>FETCH-LOGICAL-c275t-256e61ecf94f02c581997aaacce6877b9b5db8936ac4582cf357db5c3f5593fd3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,776,780,881,2863,2864,27901,27902</link.rule.ids><backlink>$$Uhttps://www.osti.gov/biblio/20645831$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Bluhme, H.</creatorcontrib><creatorcontrib>Jensen, M. J.</creatorcontrib><creatorcontrib>Nielsen, S. Brøndsted</creatorcontrib><creatorcontrib>Pedersen, U. V.</creatorcontrib><creatorcontrib>Seiersen, K.</creatorcontrib><creatorcontrib>Svendsen, A.</creatorcontrib><creatorcontrib>Andersen, L. H.</creatorcontrib><title>Electron scattering on stored mononucleotide anions</title><title>Physical review. A, Atomic, molecular, and optical physics</title><description>Collisions between electrons and deprotonated mononucleotides, AMP and UMP, were studied at the electrostatic storage ring ELISA where the two anions were stored with a 1/e lifetime of 13.5 s. It is found that the threshold energy for electron-induced reactions leading to production of neutral fragments is as high as about 12 eV for both species. The high threshold is explained within the context of a classical reaction model, applicable for atomic anions, and a high electron-binding energy of about 5 eV for the two mononucleotides. There is no evidence in the cross sections for formation of short-lived doubly charged anions.</description><subject>AMP</subject><subject>ANIONS</subject><subject>ATOMIC AND MOLECULAR PHYSICS</subject><subject>BINDING ENERGY</subject><subject>BIOPHYSICS</subject><subject>CHEMICAL BONDS</subject><subject>CROSS SECTIONS</subject><subject>DISSOCIATION</subject><subject>DNA</subject><subject>ELECTRON-MOLECULE COLLISIONS</subject><subject>ELECTRONS</subject><subject>EV RANGE</subject><subject>LIFETIME</subject><subject>SCATTERING</subject><subject>STORAGE RINGS</subject><subject>THRESHOLD ENERGY</subject><issn>1050-2947</issn><issn>1094-1622</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2004</creationdate><recordtype>article</recordtype><recordid>eNo1kEFLxDAQhYMouK7-AU8Fz10nSdM0x2VZXWFBET2HdJq4lW4iSRT239tSfZd5D94Mw0fILYUVpcDvXw6n9Gp_1isJK2AggZ6RBQVVlbRm7HzyAkqmKnlJrlL6hFFVoxaEbweLOQZfJDQ529j7j2JKOUTbFcfgg__GwYbcd7Ywvg8-XZMLZ4Zkb_7mkrw_bN82u3L__Pi0We9LZFLkkona1tSiU5UDhqKhSkljDKKtGylb1YqubRSvDVaiYei4kF0rkDshFHcdX5K7-W5IudcJ-2zxgMH78WPNoB63OB1bbG5hDClF6_RX7I8mnjQFPcHR_3C0BD3D4b-dWVm7</recordid><startdate>20040801</startdate><enddate>20040801</enddate><creator>Bluhme, H.</creator><creator>Jensen, M. J.</creator><creator>Nielsen, S. Brøndsted</creator><creator>Pedersen, U. V.</creator><creator>Seiersen, K.</creator><creator>Svendsen, A.</creator><creator>Andersen, L. H.</creator><scope>AAYXX</scope><scope>CITATION</scope><scope>OTOTI</scope></search><sort><creationdate>20040801</creationdate><title>Electron scattering on stored mononucleotide anions</title><author>Bluhme, H. ; Jensen, M. J. ; Nielsen, S. Brøndsted ; Pedersen, U. V. ; Seiersen, K. ; Svendsen, A. ; Andersen, L. H.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c275t-256e61ecf94f02c581997aaacce6877b9b5db8936ac4582cf357db5c3f5593fd3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2004</creationdate><topic>AMP</topic><topic>ANIONS</topic><topic>ATOMIC AND MOLECULAR PHYSICS</topic><topic>BINDING ENERGY</topic><topic>BIOPHYSICS</topic><topic>CHEMICAL BONDS</topic><topic>CROSS SECTIONS</topic><topic>DISSOCIATION</topic><topic>DNA</topic><topic>ELECTRON-MOLECULE COLLISIONS</topic><topic>ELECTRONS</topic><topic>EV RANGE</topic><topic>LIFETIME</topic><topic>SCATTERING</topic><topic>STORAGE RINGS</topic><topic>THRESHOLD ENERGY</topic><toplevel>online_resources</toplevel><creatorcontrib>Bluhme, H.</creatorcontrib><creatorcontrib>Jensen, M. J.</creatorcontrib><creatorcontrib>Nielsen, S. Brøndsted</creatorcontrib><creatorcontrib>Pedersen, U. V.</creatorcontrib><creatorcontrib>Seiersen, K.</creatorcontrib><creatorcontrib>Svendsen, A.</creatorcontrib><creatorcontrib>Andersen, L. H.</creatorcontrib><collection>CrossRef</collection><collection>OSTI.GOV</collection><jtitle>Physical review. A, Atomic, molecular, and optical physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Bluhme, H.</au><au>Jensen, M. J.</au><au>Nielsen, S. Brøndsted</au><au>Pedersen, U. V.</au><au>Seiersen, K.</au><au>Svendsen, A.</au><au>Andersen, L. H.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Electron scattering on stored mononucleotide anions</atitle><jtitle>Physical review. A, Atomic, molecular, and optical physics</jtitle><date>2004-08-01</date><risdate>2004</risdate><volume>70</volume><issue>2</issue><artnum>020701</artnum><issn>1050-2947</issn><eissn>1094-1622</eissn><abstract>Collisions between electrons and deprotonated mononucleotides, AMP and UMP, were studied at the electrostatic storage ring ELISA where the two anions were stored with a 1/e lifetime of 13.5 s. It is found that the threshold energy for electron-induced reactions leading to production of neutral fragments is as high as about 12 eV for both species. The high threshold is explained within the context of a classical reaction model, applicable for atomic anions, and a high electron-binding energy of about 5 eV for the two mononucleotides. There is no evidence in the cross sections for formation of short-lived doubly charged anions.</abstract><cop>United States</cop><doi>10.1103/PhysRevA.70.020701</doi></addata></record> |
fulltext | fulltext |
identifier | ISSN: 1050-2947 |
ispartof | Physical review. A, Atomic, molecular, and optical physics, 2004-08, Vol.70 (2), Article 020701 |
issn | 1050-2947 1094-1622 |
language | eng |
recordid | cdi_osti_scitechconnect_20645831 |
source | American Physical Society Journals |
subjects | AMP ANIONS ATOMIC AND MOLECULAR PHYSICS BINDING ENERGY BIOPHYSICS CHEMICAL BONDS CROSS SECTIONS DISSOCIATION DNA ELECTRON-MOLECULE COLLISIONS ELECTRONS EV RANGE LIFETIME SCATTERING STORAGE RINGS THRESHOLD ENERGY |
title | Electron scattering on stored mononucleotide anions |
url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-04T20%3A00%3A52IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-crossref_osti_&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Electron%20scattering%20on%20stored%20mononucleotide%20anions&rft.jtitle=Physical%20review.%20A,%20Atomic,%20molecular,%20and%20optical%20physics&rft.au=Bluhme,%20H.&rft.date=2004-08-01&rft.volume=70&rft.issue=2&rft.artnum=020701&rft.issn=1050-2947&rft.eissn=1094-1622&rft_id=info:doi/10.1103/PhysRevA.70.020701&rft_dat=%3Ccrossref_osti_%3E10_1103_PhysRevA_70_020701%3C/crossref_osti_%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true |