The Role of Subsurface Oxygen in the Silver-Catalyzed, Oxidative Coupling of Methane

The silver-catalyzed, oxidative coupling of methane to C2 hydrocarbons (OCM) is shown to be an extremely structure-sensitive reaction. Reaction-induced changes in the silver morphology lead to changes in the nature and extent of formation of various bulk and surface-terminating crystal structures. T...

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Veröffentlicht in:	Journal of catalysis 1999-11, Vol.188 (1), p.58-68
Hauptverfasser:	Nagy, Anton J., Mestl, Gerhard, Schlögl, Robert
Format:	Artikel
Sprache:	eng
Schlagworte:	03 NATURAL GAS 10 SYNTHETIC FUELS ACTIVATION ENERGY Catalysis CATALYTIC EFFECTS Catalytic reactions CHEMICAL REACTION KINETICS Chemistry diffusion electrolytic Exact sciences and technology facetting General and physical chemistry kinetics METHANE morphology OCM, oxidative coupling of methane OXIDATION recrystallization REFORMER PROCESSES SILVER sintering Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry
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