Enhancing Crystallization in Hybrid Perovskite Solar Cells Using Thermally Conductive 2D Boron Nitride Nanosheet Additive
Controlling crystallization and grain growth is crucial for realizing highly efficient hybrid perovskite solar cells (PSCs). In this work, enhanced PSC photovoltaic performance and stability by accelerating perovskite crystallization and grain growth via 2D hexagonal boron nitride (hBN) nanosheet ad...
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| Veröffentlicht in: | Small (Weinheim an der Bergstrasse, Germany) Germany), 2023-04, Vol.19 (15), p.e2207092-n/a |
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| creator | Yin, Yifan Zhou, Yuchen Fu, Shi Zuo, Xianghao Lin, Yu‐Chung Wang, Likun Xue, Yuan Zhang, Yugang Tsai, Esther H. R. Hwang, Sooyeon Kissenger, Kim Li, Mingxing Cotlet, Mircea Li, Tai‐De Yager, Kevin G. Nam, Chang‐Yong Rafailovich, Miriam H. |
| description | Controlling crystallization and grain growth is crucial for realizing highly efficient hybrid perovskite solar cells (PSCs). In this work, enhanced PSC photovoltaic performance and stability by accelerating perovskite crystallization and grain growth via 2D hexagonal boron nitride (hBN) nanosheet additives incorporated into the active perovskite layer are demonstrated. In situ X‐ray scattering and infrared thermal imaging during the perovskite annealing process revealed the highly thermally conductive hBN nanosheets promoted the phase conversion and grain growth in the perovskite layer by facilitating a more rapid and spatially uniform temperature rise within the perovskite film. Complementary structural, physicochemical, and electrical characterizations further showed that the hBN nanosheets formed a physical barrier at the perovskite grain boundaries and the interfaces with charge transport layers, passivating defects, and retarding ion migration. As a result, the power conversion efficiency of the PSC is improved from 17.4% to 19.8%, along with enhanced device stability, retaining ≈90% of the initial efficiency even after 500 h ambient air storage. The results not only highlight 2D hBN as an effective additive for PSCs but also suggest enhanced thermal transport as one of the pathways for improved PSC performance by 2D material additives in general.
In situ synchrotron X‐ray scattering and real‐time thermal imaging for the first time unraveled the effects of the thermally conductive additive, hexagonal boron nitride nanosheets, on enhancing the crystallization kinetics in organic‐inorganic hybrid perovskites and the associated solar cell performance and stability. |
| doi_str_mv | 10.1002/smll.202207092 |
| format | Article |
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In situ synchrotron X‐ray scattering and real‐time thermal imaging for the first time unraveled the effects of the thermally conductive additive, hexagonal boron nitride nanosheets, on enhancing the crystallization kinetics in organic‐inorganic hybrid perovskites and the associated solar cell performance and stability.</description><identifier>ISSN: 1613-6810</identifier><identifier>EISSN: 1613-6829</identifier><identifier>DOI: 10.1002/smll.202207092</identifier><identifier>PMID: 36631283</identifier><language>eng</language><publisher>Germany: Wiley Subscription Services, Inc</publisher><subject>2D materials ; Additives ; Barriers ; Boron nitride ; Charge transport ; Crystal defects ; Crystallization ; Energy conversion efficiency ; Grain boundaries ; Grain growth ; grazing‐incidence wide‐angle X‐ray scattering (GIWAXS) ; hybrid perovskite solar cells ; Infrared imaging ; Ion migration ; NANOSCIENCE AND NANOTECHNOLOGY ; Nanosheets ; Nanotechnology ; Perovskites ; Photovoltaic cells ; Solar cells ; Stability ; Thermal imaging ; Two dimensional materials</subject><ispartof>Small (Weinheim an der Bergstrasse, Germany), 2023-04, Vol.19 (15), p.e2207092-n/a</ispartof><rights>2023 Wiley‐VCH GmbH</rights><rights>2023 Wiley-VCH GmbH.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c4402-770bdb33aaba21895e9bb1e917b391adcb65cada5ade72cd6303c838b80f289d3</citedby><cites>FETCH-LOGICAL-c4402-770bdb33aaba21895e9bb1e917b391adcb65cada5ade72cd6303c838b80f289d3</cites><orcidid>0000-0002-9093-4063 ; 0000000278321475 ; 0000000290934063</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fsmll.202207092$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fsmll.202207092$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>230,314,776,780,881,1411,27901,27902,45550,45551</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/36631283$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/servlets/purl/1958563$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Yin, Yifan</creatorcontrib><creatorcontrib>Zhou, Yuchen</creatorcontrib><creatorcontrib>Fu, Shi</creatorcontrib><creatorcontrib>Zuo, Xianghao</creatorcontrib><creatorcontrib>Lin, Yu‐Chung</creatorcontrib><creatorcontrib>Wang, Likun</creatorcontrib><creatorcontrib>Xue, Yuan</creatorcontrib><creatorcontrib>Zhang, Yugang</creatorcontrib><creatorcontrib>Tsai, Esther H. R.</creatorcontrib><creatorcontrib>Hwang, Sooyeon</creatorcontrib><creatorcontrib>Kissenger, Kim</creatorcontrib><creatorcontrib>Li, Mingxing</creatorcontrib><creatorcontrib>Cotlet, Mircea</creatorcontrib><creatorcontrib>Li, Tai‐De</creatorcontrib><creatorcontrib>Yager, Kevin G.</creatorcontrib><creatorcontrib>Nam, Chang‐Yong</creatorcontrib><creatorcontrib>Rafailovich, Miriam H.</creatorcontrib><creatorcontrib>Brookhaven National Laboratory (BNL), Upton, NY (United States). National Synchrotron Light Source II (NSLS-II)</creatorcontrib><creatorcontrib>Brookhaven National Laboratory (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)</creatorcontrib><title>Enhancing Crystallization in Hybrid Perovskite Solar Cells Using Thermally Conductive 2D Boron Nitride Nanosheet Additive</title><title>Small (Weinheim an der Bergstrasse, Germany)</title><addtitle>Small</addtitle><description>Controlling crystallization and grain growth is crucial for realizing highly efficient hybrid perovskite solar cells (PSCs). In this work, enhanced PSC photovoltaic performance and stability by accelerating perovskite crystallization and grain growth via 2D hexagonal boron nitride (hBN) nanosheet additives incorporated into the active perovskite layer are demonstrated. In situ X‐ray scattering and infrared thermal imaging during the perovskite annealing process revealed the highly thermally conductive hBN nanosheets promoted the phase conversion and grain growth in the perovskite layer by facilitating a more rapid and spatially uniform temperature rise within the perovskite film. Complementary structural, physicochemical, and electrical characterizations further showed that the hBN nanosheets formed a physical barrier at the perovskite grain boundaries and the interfaces with charge transport layers, passivating defects, and retarding ion migration. As a result, the power conversion efficiency of the PSC is improved from 17.4% to 19.8%, along with enhanced device stability, retaining ≈90% of the initial efficiency even after 500 h ambient air storage. The results not only highlight 2D hBN as an effective additive for PSCs but also suggest enhanced thermal transport as one of the pathways for improved PSC performance by 2D material additives in general.
In situ synchrotron X‐ray scattering and real‐time thermal imaging for the first time unraveled the effects of the thermally conductive additive, hexagonal boron nitride nanosheets, on enhancing the crystallization kinetics in organic‐inorganic hybrid perovskites and the associated solar cell performance and stability.</description><subject>2D materials</subject><subject>Additives</subject><subject>Barriers</subject><subject>Boron nitride</subject><subject>Charge transport</subject><subject>Crystal defects</subject><subject>Crystallization</subject><subject>Energy conversion efficiency</subject><subject>Grain boundaries</subject><subject>Grain growth</subject><subject>grazing‐incidence wide‐angle X‐ray scattering (GIWAXS)</subject><subject>hybrid perovskite solar cells</subject><subject>Infrared imaging</subject><subject>Ion migration</subject><subject>NANOSCIENCE AND NANOTECHNOLOGY</subject><subject>Nanosheets</subject><subject>Nanotechnology</subject><subject>Perovskites</subject><subject>Photovoltaic cells</subject><subject>Solar cells</subject><subject>Stability</subject><subject>Thermal imaging</subject><subject>Two dimensional materials</subject><issn>1613-6810</issn><issn>1613-6829</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNqFkUtvEzEUhS1ERUtgyxJZsGGT4EfGM16WoaWVQkFqu7b8CnHx2K3tKZr-ehylTSU2rO5dfOeTjg4A7zBaYITI5zx4vyCIENQiTl6AI8wwnbOO8Jf7H6ND8DrnG4QoJsv2FTikjNW3o0dgOgkbGbQLv2Cfplyk9-5BFhcDdAGeTSo5A3_aFO_zb1csvIxeJthb7zO8ztvY1camocYm2MdgRl3cvYXkK_wSU5VcuFINFl7IEPPG2gKPjXFb5g04WEuf7dvHOwPXpydX_dl89ePbeX-8muvlEpF52yJlFKVSKklwxxvLlcKW41ZRjqXRijVaGtlIY1uiDaOI6o52qkNr0nFDZ-DDzhtzcSLr2kJvdAzB6iIwb7qG0Qp92kG3Kd6NNhcxuKxrSxlsHLMgLWtQSwnBFf34D3oTxxRqhUpxzmnHqnEGFjtKp5hzsmtxm9wg0yQwEtvlxHY5sV-uBt4_akc1WLPHn6aqAN8Bf5y303904vL7avUs_wu6xKYS</recordid><startdate>20230401</startdate><enddate>20230401</enddate><creator>Yin, Yifan</creator><creator>Zhou, Yuchen</creator><creator>Fu, Shi</creator><creator>Zuo, Xianghao</creator><creator>Lin, Yu‐Chung</creator><creator>Wang, Likun</creator><creator>Xue, Yuan</creator><creator>Zhang, Yugang</creator><creator>Tsai, Esther H. 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R.</au><au>Hwang, Sooyeon</au><au>Kissenger, Kim</au><au>Li, Mingxing</au><au>Cotlet, Mircea</au><au>Li, Tai‐De</au><au>Yager, Kevin G.</au><au>Nam, Chang‐Yong</au><au>Rafailovich, Miriam H.</au><aucorp>Brookhaven National Laboratory (BNL), Upton, NY (United States). National Synchrotron Light Source II (NSLS-II)</aucorp><aucorp>Brookhaven National Laboratory (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Enhancing Crystallization in Hybrid Perovskite Solar Cells Using Thermally Conductive 2D Boron Nitride Nanosheet Additive</atitle><jtitle>Small (Weinheim an der Bergstrasse, Germany)</jtitle><addtitle>Small</addtitle><date>2023-04-01</date><risdate>2023</risdate><volume>19</volume><issue>15</issue><spage>e2207092</spage><epage>n/a</epage><pages>e2207092-n/a</pages><issn>1613-6810</issn><eissn>1613-6829</eissn><abstract>Controlling crystallization and grain growth is crucial for realizing highly efficient hybrid perovskite solar cells (PSCs). In this work, enhanced PSC photovoltaic performance and stability by accelerating perovskite crystallization and grain growth via 2D hexagonal boron nitride (hBN) nanosheet additives incorporated into the active perovskite layer are demonstrated. In situ X‐ray scattering and infrared thermal imaging during the perovskite annealing process revealed the highly thermally conductive hBN nanosheets promoted the phase conversion and grain growth in the perovskite layer by facilitating a more rapid and spatially uniform temperature rise within the perovskite film. Complementary structural, physicochemical, and electrical characterizations further showed that the hBN nanosheets formed a physical barrier at the perovskite grain boundaries and the interfaces with charge transport layers, passivating defects, and retarding ion migration. As a result, the power conversion efficiency of the PSC is improved from 17.4% to 19.8%, along with enhanced device stability, retaining ≈90% of the initial efficiency even after 500 h ambient air storage. The results not only highlight 2D hBN as an effective additive for PSCs but also suggest enhanced thermal transport as one of the pathways for improved PSC performance by 2D material additives in general.
In situ synchrotron X‐ray scattering and real‐time thermal imaging for the first time unraveled the effects of the thermally conductive additive, hexagonal boron nitride nanosheets, on enhancing the crystallization kinetics in organic‐inorganic hybrid perovskites and the associated solar cell performance and stability.</abstract><cop>Germany</cop><pub>Wiley Subscription Services, Inc</pub><pmid>36631283</pmid><doi>10.1002/smll.202207092</doi><tpages>11</tpages><orcidid>https://orcid.org/0000-0002-9093-4063</orcidid><orcidid>https://orcid.org/0000000278321475</orcidid><orcidid>https://orcid.org/0000000290934063</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | 2D materials Additives Barriers Boron nitride Charge transport Crystal defects Crystallization Energy conversion efficiency Grain boundaries Grain growth grazing‐incidence wide‐angle X‐ray scattering (GIWAXS) hybrid perovskite solar cells Infrared imaging Ion migration NANOSCIENCE AND NANOTECHNOLOGY Nanosheets Nanotechnology Perovskites Photovoltaic cells Solar cells Stability Thermal imaging Two dimensional materials |
| title | Enhancing Crystallization in Hybrid Perovskite Solar Cells Using Thermally Conductive 2D Boron Nitride Nanosheet Additive |
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