Stimulated Rayleigh Scattering Enhanced by a Longitudinal Plasma Mode in a Periodically Driven Dirac Semimetal Cd3As2

Using broadband (12–45 THz) multi-terahertz spectroscopy, we show that stimulated Rayleigh scattering dominates the transient optical conductivity of cadmium arsenide, a Dirac semimetal, under an optical driving field at 30 THz. Here, the characteristic dispersive line shape with net optical gain is...

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Veröffentlicht in:Physical review letters 2022-11, Vol.129 (20)
Hauptverfasser: Murotani, Yuta, Kanda, Natsuki, Ikeda, Tatsuhiko N., Matsuda, Takuya, Goyal, Manik, Yoshinobu, Jun, Kobayashi, Yohei, Stemmer, Susanne, Matsunaga, Ryusuke
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container_title Physical review letters
container_volume 129
creator Murotani, Yuta
Kanda, Natsuki
Ikeda, Tatsuhiko N.
Matsuda, Takuya
Goyal, Manik
Yoshinobu, Jun
Kobayashi, Yohei
Stemmer, Susanne
Matsunaga, Ryusuke
description Using broadband (12–45 THz) multi-terahertz spectroscopy, we show that stimulated Rayleigh scattering dominates the transient optical conductivity of cadmium arsenide, a Dirac semimetal, under an optical driving field at 30 THz. Here, the characteristic dispersive line shape with net optical gain is accounted for by optical transitions between light-induced Floquet subbands, strikingly enhanced by the longitudinal plasma mode. Stimulated Rayleigh scattering with an unprecedentedly large refractive index change may pave the way for slow light generation in conductive solids at room temperature.
doi_str_mv 10.1103/PhysRevLett.129.207402
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source American Physical Society Journals; EZB-FREE-00999 freely available EZB journals
subjects Coherent control
CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Dirac semimetal
Floquet systems
Optical & microwave phenomena
Photoexcitation
Photoinduced effect
Rayleigh scattering
Terahertz spectroscopy
title Stimulated Rayleigh Scattering Enhanced by a Longitudinal Plasma Mode in a Periodically Driven Dirac Semimetal Cd3As2
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