Evaporation and Molecular Beam Scattering from a Flat Liquid Jet

An experimental setup for molecular beam scattering from flat liquid sheets has been developed, with the goal of studying reactions at gas–liquid interfaces for volatile liquids. Specifically, a crossed molecular beam instrument that can measure angular and translational energy distributions of scat...

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Veröffentlicht in:	The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory Molecules, spectroscopy, kinetics, environment, & general theory, 2022-05, Vol.126 (21)
Hauptverfasser:	Lee, Chin, Pohl, Marvin N., Ramphal, Isaac A., Yang, Walt, Winter, Bernd, Abel, Bernd, Neumark, Daniel M.
Format:	Artikel
Sprache:	eng
Schlagworte:	Collisions Energy Evaporation INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY Liquids Scattering
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container_title	The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory
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creator	Lee, Chin Pohl, Marvin N. Ramphal, Isaac A. Yang, Walt Winter, Bernd Abel, Bernd Neumark, Daniel M.
description	An experimental setup for molecular beam scattering from flat liquid sheets has been developed, with the goal of studying reactions at gas–liquid interfaces for volatile liquids. Specifically, a crossed molecular beam instrument that can measure angular and translational energy distributions of scattered products has been adapted for liquid jet scattering. A microfluidic chip is used to create a stable flat liquid sheet inside vacuum from which scattering occurs, and both evaporation and scattering from this sheet are characterized using a rotatable mass spectrometer that can measure product time-of-flight distributions. Furthermore, this article describes the instrument and reports on the first measurements of evaporation of dodecane and Ne from a Ne-doped dodecane flat jet, as well as scattering of Ne from a flat jet of pure dodecane.
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subjects	Collisions Energy Evaporation INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY Liquids Scattering
title	Evaporation and Molecular Beam Scattering from a Flat Liquid Jet
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