Photoinduced Charge Transfer with a Small Driving Force Facilitated by Exciplex-like Complex Formation in Metal–Organic Frameworks

Photoinduced charge transfer (PCT) is a key step in the light-harvesting (LH) process producing the redox equivalents for energy conversion. However, like traditional macromolecular donor–acceptor assemblies, most MOF-derived LH systems are designed with a large ΔG 0 to drive PCT. To emulate the fun...

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Veröffentlicht in:	Journal of the American Chemical Society 2021-09, Vol.143 (37), p.15286-15297
Hauptverfasser:	Li, Xinlin, Yu, Jierui, Lu, Zhiyong, Duan, Jiaxin, Fry, H. Christopher, Gosztola, David J, Maindan, Karan, Rajasree, Sreehari Surendran, Deria, Pravas
Format:	Artikel
Sprache:	eng
Online-Zugang:	Volltext
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