Unveiling the spatial distribution of molecular coherences at conical intersections by covariance X-ray diffraction signals

Significance Monitoring the real-space motion of the electrons directly involved in ultrafast molecular dynamics is a challenging goal, hindered by the strong contributions of the remaining inactive electrons. Molecular quantum coherences can provide a direct window into elementary electronic dynami...

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Veröffentlicht in:Proceedings of the National Academy of Sciences - PNAS 2021-05, Vol.118 (22)
Hauptverfasser: Cavaletto, Stefano M., Keefer, Daniel, Rouxel, Jérémy R., Aleotti, Flavia, Segatta, Francesco, Garavelli, Marco, Mukamel, Shaul
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Sprache:eng
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