Zero‐Valent Palladium Single‐Atoms Catalysts Confined in Black Phosphorus for Efficient Semi‐Hydrogenation

Single‐atom catalysts (SACs) represent a new frontier in heterogeneous catalysis due to their remarkable catalytic properties and maximized atomic utilization. However, single atoms often bond to the support with polarized electron density and thus exhibit a high valence state, limiting their cataly...

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Veröffentlicht in:	Advanced materials (Weinheim) 2021-09, Vol.33 (35), p.e2008471-n/a
Hauptverfasser:	Chen, Cheng, Ou, Wei, Yam, Kah‐Meng, Xi, Shibo, Zhao, Xiaoxu, Chen, Si, Li, Jing, Lyu, Pin, Ma, Lu, Du, Yonghua, Yu, Wei, Fang, Hanyan, Yao, Chuanhao, Hai, Xiao, Xu, Haomin, Koh, Ming Joo, Pennycook, Stephen J., Lu, Junling, Lin, Ming, Su, Chenliang, Zhang, Chun, Lu, Jiong
Format:	Artikel
Sprache:	eng
Schlagworte:	Atomic layer epitaxy Atomic properties black phosphorus Catalysis Chemical bonds Confined spaces Density functional theory Electron density Electronegativity Hydrogenation MATERIALS SCIENCE Nanoparticles Palladium Phosphorus reaction mechanisms Single atom catalysts single-atom catalyst Synthesis Two dimensional materials Valence zero valence
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