Pore-Edge Tailoring of Single-Atom Iron–Nitrogen Sites on Graphene for Enhanced CO2 Reduction

Hosting atomically dispersed nitrogen-coordinated iron sites (Fe–N4) on graphene offers unique opportunities for driving electrochemical CO2 reduction reaction (CO2RR) to CO. However, the strong adsorption of *CO on the Fe–N4 site embedded in intact graphene limits current density due to slow CO des...

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Veröffentlicht in:	ACS catalysis 2020-10, Vol.10 (19), p.10803-10811
Hauptverfasser:	Pan, Fuping, Li, Boyang, Sarnello, Erik, Fei, Yuhuan, Feng, Xuhui, Gang, Yang, Xiang, Xianmei, Fang, Lingzhe, Li, Tao, Hu, Yun Hang, Wang, Guofeng, Li, Ying
Format:	Artikel
Sprache:	eng
Schlagworte:	CO adsorption CO2 reduction INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY local carbon structure pore edge single-atom catalyst
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