Unusual Phonon Heat Transport in α−RuCl3: Strong Spin-Phonon Scattering and Field-Induced Spin Gap

The honeycomb Kitaev-Heisenberg model is a source of a quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. Here we unveil the highly unusual low-temperature heat conductivity κ of α−RuCl3, a prime candidate for realizing such physics: beyond a magnetic...

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Veröffentlicht in:Physical review letters 2018-03, Vol.120 (11), p.117204
Hauptverfasser: Hentrich, Richard, Wolter, Anja U B, Zotos, Xenophon, Brenig, Wolfram, Nowak, Domenic, Isaeva, Anna, Doert, Thomas, Banerjee, Arnab, Lampen-Kelley, Paula, Mandrus, David G, Nagler, Stephen E, Sears, Jennifer, Kim, Young-June, Büchner, Bernd, Hess, Christian
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container_end_page
container_issue 11
container_start_page 117204
container_title Physical review letters
container_volume 120
creator Hentrich, Richard
Wolter, Anja U B
Zotos, Xenophon
Brenig, Wolfram
Nowak, Domenic
Isaeva, Anna
Doert, Thomas
Banerjee, Arnab
Lampen-Kelley, Paula
Mandrus, David G
Nagler, Stephen E
Sears, Jennifer
Kim, Young-June
Büchner, Bernd
Hess, Christian
description The honeycomb Kitaev-Heisenberg model is a source of a quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. Here we unveil the highly unusual low-temperature heat conductivity κ of α−RuCl3, a prime candidate for realizing such physics: beyond a magnetic field of Bc≈7.5 T, κ increases by about one order of magnitude, both for in-plane as well as out-of-plane transport. This clarifies the unusual magnetic field dependence unambiguously to be the result of severe scattering of phonons off putative Kitaev-Heisenberg excitations in combination with a drastic field-induced change of the magnetic excitation spectrum. In particular, an unexpected, large energy gap arises, which increases linearly with the magnetic field, reaching remarkable ℏω0/kB≈50 K at 18 T.
doi_str_mv 10.1103/PhysRevLett.120.117204
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source American Physical Society Journals; Elektronische Zeitschriftenbibliothek - Frei zugängliche E-Journals
subjects CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Dependence
Energy gap
Excitation spectra
Fermions
Heisenberg theory
Honeycomb construction
Magnetic fields
Phonons
Ruthenium trichloride
Scattering
Spin liquid
Statistical models
Thermal conductivity
Transport
title Unusual Phonon Heat Transport in α−RuCl3: Strong Spin-Phonon Scattering and Field-Induced Spin Gap
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