The role of defect sites and oxophilicity of the support on the phenol hydrodeoxygenation reaction

[Display omitted] •Hydrodeoxygenation of phenol at gas phase over Pd/CexZr1-xO2 catalysts.•There is no correlation between oxygen vacancies amount and deoxygenation activity.•Deoxygenation is promoted by oxophilicity of the Zr4+/Zr3+ cations in the support.•The stronger interaction O - Zr4+/Zr3+ acc...

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Veröffentlicht in:	Applied catalysis. B, Environmental Environmental, 2019-07, Vol.249 (C), p.292-305
Hauptverfasser:	Teles, Camila A., de Souza, Priscilla M., Braga, Adriano Henrique, Rabelo-Neto, Raimundo C., Teran, Alejandra, Jacobs, Gary, Resasco, Daniel E., Noronha, Fabio B.
Format:	Artikel
Sprache:	eng
Schlagworte:	Benzene Bio-oil Byproducts Carbonyl groups Carbonyls Catalysis Catalysts Cations Cerium oxides Chemistry Deactivation Defect sites Density Deoxygenation Engineering Hydrocarbons Hydrodeoxygenation Oxygen vacancy Phenol Phenols Selectivity Solid solutions Stability Temperature Vapor phases Zirconium dioxide
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