Inline gamma-spectrometry of fission product elements after rapid high-pressure ion chromatographic separation
Analysis of irradiated material shortly after irradiation can be non-trivial due to highly radioactive activation and fission isotopes increasing dead time in gamma-ray detection systems, often requiring a “cooling-period” between receipt of a sample and the subsequent analysis. A direct separation–...
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| Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2020-05, Vol.324 (2), p.759-771 |
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| container_title | Journal of radioanalytical and nuclear chemistry |
| container_volume | 324 |
| creator | Fenske, Emilie K. Roach, Benjamin D. Hexel, Cole R. Glasgow, David C. Stewart, Ian R. Partridge, John D. Giaquinto, Joseph M. |
| description | Analysis of irradiated material shortly after irradiation can be non-trivial due to highly radioactive activation and fission isotopes increasing dead time in gamma-ray detection systems, often requiring a “cooling-period” between receipt of a sample and the subsequent analysis. A direct separation–detection method has been developed combining ion chromatography and inductively coupled mass spectrometry for rapid, low-level analysis of fission products; it cannot, however, detect certain short-lived species below the detection limit of the system. Here we report the implementation of an inline gamma-ray detector, which was added post-separation, pre-analysis, to test the quality and utility of elementally-isolated gamma-ray spectroscopy. |
| doi_str_mv | 10.1007/s10967-020-07103-x |
| format | Article |
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(ORNL), Oak Ridge, TN (United States)</creatorcontrib><title>Inline gamma-spectrometry of fission product elements after rapid high-pressure ion chromatographic separation</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><description>Analysis of irradiated material shortly after irradiation can be non-trivial due to highly radioactive activation and fission isotopes increasing dead time in gamma-ray detection systems, often requiring a “cooling-period” between receipt of a sample and the subsequent analysis. A direct separation–detection method has been developed combining ion chromatography and inductively coupled mass spectrometry for rapid, low-level analysis of fission products; it cannot, however, detect certain short-lived species below the detection limit of the system. Here we report the implementation of an inline gamma-ray detector, which was added post-separation, pre-analysis, to test the quality and utility of elementally-isolated gamma-ray spectroscopy.</description><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Chromatography</subject><subject>Detectors</subject><subject>Diagnostic Radiology</subject><subject>Fission products</subject><subject>Gamma ray detectors</subject><subject>Gamma rays</subject><subject>Gamma spectroscopy</subject><subject>Hadrons</subject><subject>Heavy Ions</subject><subject>Inductively coupled plasma mass spectrometry</subject><subject>Inline gamma-ray detection</subject><subject>Inorganic Chemistry</subject><subject>Ion chromatography</subject><subject>Irradiation</subject><subject>Mass spectrometry</subject><subject>Nuclear Chemistry</subject><subject>Nuclear fuel cycle</subject><subject>Nuclear Physics</subject><subject>Physical Chemistry</subject><subject>RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY</subject><subject>Radiation, Background</subject><subject>Rapid isotope analysis</subject><subject>Scientific imaging</subject><subject>Separation</subject><subject>Spectrum analysis</subject><issn>0236-5731</issn><issn>1588-2780</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNp9kUuLHCEUhYuQQDqT_IGsJFk7uWqXj-Uw5DEwkE2yFtu6Vjl0aUVtmPn3cVKB7IILQb9z7j2cYXjP4JoBqE-VgZGKAgcKioGgjy-GAxu1plxpeDkcgAtJRyXY6-FNrQ8AYLQWhyHdpXNMSGa3ro7WDX0recVWnkgOJMRaY05kK3m6-EbwjCumVokLDQspbosTWeK80K1grZeC5Bn3S_dwLc8dWKInFTdXXOtfb4dXwZ0rvvt7Xw0_v3z-cfuN3n__end7c0-90GOjKLUOYEboESCcJsW1VmJCh8fjKJicDA-jdGYy8shhdHo8SeMV04YJdPwkroYPu2-uLdrqY0O_-JxSz2eZBKn02KGPO9Tj_bpgbfYhX0rqe1kuTJ8DyphOXe_U7M5oYwq5Fef7mXCN3RJD7O83knOmleKyC_gu8CXXWjDYrcTVlSfLwD63Zfe2bG_L_mnLPnaR2EW1w2nG8m-X_6h-A8MgmP8</recordid><startdate>20200501</startdate><enddate>20200501</enddate><creator>Fenske, Emilie K.</creator><creator>Roach, Benjamin D.</creator><creator>Hexel, Cole R.</creator><creator>Glasgow, David C.</creator><creator>Stewart, Ian R.</creator><creator>Partridge, John D.</creator><creator>Giaquinto, Joseph M.</creator><general>Springer International Publishing</general><general>Springer</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>OIOZB</scope><scope>OTOTI</scope><orcidid>https://orcid.org/0000000181012422</orcidid><orcidid>https://orcid.org/0000000263343639</orcidid><orcidid>https://orcid.org/0000000177812013</orcidid><orcidid>https://orcid.org/0000000153085798</orcidid></search><sort><creationdate>20200501</creationdate><title>Inline gamma-spectrometry of fission product elements after rapid high-pressure ion chromatographic separation</title><author>Fenske, Emilie K. ; Roach, Benjamin D. ; Hexel, Cole R. ; Glasgow, David C. ; Stewart, Ian R. ; Partridge, John D. ; Giaquinto, Joseph M.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c385t-e688f09501580fbd728873deae445316d92f56a9d964205a85b69c718913ea2b3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Chromatography</topic><topic>Detectors</topic><topic>Diagnostic Radiology</topic><topic>Fission products</topic><topic>Gamma ray detectors</topic><topic>Gamma rays</topic><topic>Gamma spectroscopy</topic><topic>Hadrons</topic><topic>Heavy Ions</topic><topic>Inductively coupled plasma mass spectrometry</topic><topic>Inline gamma-ray detection</topic><topic>Inorganic Chemistry</topic><topic>Ion chromatography</topic><topic>Irradiation</topic><topic>Mass spectrometry</topic><topic>Nuclear Chemistry</topic><topic>Nuclear fuel cycle</topic><topic>Nuclear Physics</topic><topic>Physical Chemistry</topic><topic>RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY</topic><topic>Radiation, Background</topic><topic>Rapid isotope analysis</topic><topic>Scientific imaging</topic><topic>Separation</topic><topic>Spectrum analysis</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Fenske, Emilie K.</creatorcontrib><creatorcontrib>Roach, Benjamin D.</creatorcontrib><creatorcontrib>Hexel, Cole R.</creatorcontrib><creatorcontrib>Glasgow, David C.</creatorcontrib><creatorcontrib>Stewart, Ian R.</creatorcontrib><creatorcontrib>Partridge, John D.</creatorcontrib><creatorcontrib>Giaquinto, Joseph M.</creatorcontrib><creatorcontrib>Oak Ridge National Lab. 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| subjects | Chemistry Chemistry and Materials Science Chromatography Detectors Diagnostic Radiology Fission products Gamma ray detectors Gamma rays Gamma spectroscopy Hadrons Heavy Ions Inductively coupled plasma mass spectrometry Inline gamma-ray detection Inorganic Chemistry Ion chromatography Irradiation Mass spectrometry Nuclear Chemistry Nuclear fuel cycle Nuclear Physics Physical Chemistry RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY Radiation, Background Rapid isotope analysis Scientific imaging Separation Spectrum analysis |
| title | Inline gamma-spectrometry of fission product elements after rapid high-pressure ion chromatographic separation |
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