Reduced-order model for microstructure evolution prediction in the electrodes of solid oxide fuel cell with dynamic discrepancy reduced modeling
Microstructure evolution in the electrodes of solid oxide fuel cell is an important degradation mechanism which reduces active sites for redox reaction and the electric conductivity. Phase field models for microstructure evolution simulation are usually expensive for large scale simulations. In this...
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Veröffentlicht in: | Journal of power sources 2019-03, Vol.416 (C), p.37-49 |
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creator | Lei, Yinkai Cheng, Tian-Le Mebane, David S. Wen, You-Hai |
description | Microstructure evolution in the electrodes of solid oxide fuel cell is an important degradation mechanism which reduces active sites for redox reaction and the electric conductivity. Phase field models for microstructure evolution simulation are usually expensive for large scale simulations. In this work, a reduced-order coarsening model is developed using dynamic discrepancy reduced modeling, which reduces the model order by inserting Gaussian process stochastic functions into the dynamic equations of Ostwald ripening. The reduced order model has been calibrated on a dataset generated by a phase field model that has been well validated to experiments. A validating dataset has also been generated with which the model prediction show good agreement. This model is further applied to predict long term microstructure evolution in different SOFC electrodes. This work is the first attempt of building a degradation model of SOFC using data science techniques.
[Display omitted]
•A reduced order coarsening model for microstructure evolution prediction in SOFC electrode.•Dynamic discrepancy reduced modeling is used to enhance the Ostwald ripening model.•Phase field simulations used in model training and validation.•First attempt of applying data science technique in the research of SOFC degradation. |
doi_str_mv | 10.1016/j.jpowsour.2019.01.046 |
format | Article |
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[Display omitted]
•A reduced order coarsening model for microstructure evolution prediction in SOFC electrode.•Dynamic discrepancy reduced modeling is used to enhance the Ostwald ripening model.•Phase field simulations used in model training and validation.•First attempt of applying data science technique in the research of SOFC degradation.</description><identifier>ISSN: 0378-7753</identifier><identifier>EISSN: 1873-2755</identifier><identifier>DOI: 10.1016/j.jpowsour.2019.01.046</identifier><language>eng</language><publisher>United States: Elsevier B.V</publisher><subject>Bayesian calibration ; Dynamic discrepancy reduced modeling ; ENGINEERING ; INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY ; MATERIALS SCIENCE ; Microstructure evolution ; Phase-field simulation ; Reduced order model ; SOFC degradation</subject><ispartof>Journal of power sources, 2019-03, Vol.416 (C), p.37-49</ispartof><rights>2019 Elsevier B.V.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c426t-b79509d7fdacfb832d4a494483839a8a843f2a978447c2cc074f1e5e6de354e13</citedby><cites>FETCH-LOGICAL-c426t-b79509d7fdacfb832d4a494483839a8a843f2a978447c2cc074f1e5e6de354e13</cites><orcidid>0000-0002-0200-1491 ; 0000000202001491</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.jpowsour.2019.01.046$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>230,315,781,785,886,3551,27926,27927,45997</link.rule.ids><backlink>$$Uhttps://www.osti.gov/servlets/purl/1532662$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Lei, Yinkai</creatorcontrib><creatorcontrib>Cheng, Tian-Le</creatorcontrib><creatorcontrib>Mebane, David S.</creatorcontrib><creatorcontrib>Wen, You-Hai</creatorcontrib><creatorcontrib>National Energy Technology Laboratory (NETL), Pittsburgh, PA, Morgantown, WV, and Albany, OR (United States)</creatorcontrib><title>Reduced-order model for microstructure evolution prediction in the electrodes of solid oxide fuel cell with dynamic discrepancy reduced modeling</title><title>Journal of power sources</title><description>Microstructure evolution in the electrodes of solid oxide fuel cell is an important degradation mechanism which reduces active sites for redox reaction and the electric conductivity. Phase field models for microstructure evolution simulation are usually expensive for large scale simulations. In this work, a reduced-order coarsening model is developed using dynamic discrepancy reduced modeling, which reduces the model order by inserting Gaussian process stochastic functions into the dynamic equations of Ostwald ripening. The reduced order model has been calibrated on a dataset generated by a phase field model that has been well validated to experiments. A validating dataset has also been generated with which the model prediction show good agreement. This model is further applied to predict long term microstructure evolution in different SOFC electrodes. This work is the first attempt of building a degradation model of SOFC using data science techniques.
[Display omitted]
•A reduced order coarsening model for microstructure evolution prediction in SOFC electrode.•Dynamic discrepancy reduced modeling is used to enhance the Ostwald ripening model.•Phase field simulations used in model training and validation.•First attempt of applying data science technique in the research of SOFC degradation.</description><subject>Bayesian calibration</subject><subject>Dynamic discrepancy reduced modeling</subject><subject>ENGINEERING</subject><subject>INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY</subject><subject>MATERIALS SCIENCE</subject><subject>Microstructure evolution</subject><subject>Phase-field simulation</subject><subject>Reduced order model</subject><subject>SOFC degradation</subject><issn>0378-7753</issn><issn>1873-2755</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNqFkF9LwzAUxYMoOKdfQYLvrUmTNu2bMvwHgiD6HLLkxmV0zUjazX0LP7Kp1Wef7oV7zzmcH0KXlOSU0Op6na-3fh_9EPKC0CYnNCe8OkIzWguWFaIsj9GMMFFnQpTsFJ3FuCaEUCrIDH29ghk0mMwHAwFvvIEWW582p4OPfRh0PwTAsPPt0Dvf4W0A4_TP6jrcr9KtBd2HpIzYWxx96wz2n84AtkNy09C2eO_6FTaHTiVfbFzUAbaq0wccpvwp2XUf5-jEqjbCxe-co_f7u7fFY_b88vC0uH3ONC-qPluKpiSNEdYobZc1KwxXvOG8ZjVrVK1qzmyhGlFzLnShNRHcUiihMsBKDpTN0dXkm0o6GbXrQa-077rURdKSFVVVpKdqehpZxABWboPbqHCQlMgRvlzLP_hyhC8JlQl-Et5MQkgVdg7CmABdKurCGGC8-8_iGwqelbc</recordid><startdate>20190315</startdate><enddate>20190315</enddate><creator>Lei, Yinkai</creator><creator>Cheng, Tian-Le</creator><creator>Mebane, David S.</creator><creator>Wen, You-Hai</creator><general>Elsevier B.V</general><general>Elsevier</general><scope>AAYXX</scope><scope>CITATION</scope><scope>OIOZB</scope><scope>OTOTI</scope><orcidid>https://orcid.org/0000-0002-0200-1491</orcidid><orcidid>https://orcid.org/0000000202001491</orcidid></search><sort><creationdate>20190315</creationdate><title>Reduced-order model for microstructure evolution prediction in the electrodes of solid oxide fuel cell with dynamic discrepancy reduced modeling</title><author>Lei, Yinkai ; Cheng, Tian-Le ; Mebane, David S. ; Wen, You-Hai</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c426t-b79509d7fdacfb832d4a494483839a8a843f2a978447c2cc074f1e5e6de354e13</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Bayesian calibration</topic><topic>Dynamic discrepancy reduced modeling</topic><topic>ENGINEERING</topic><topic>INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY</topic><topic>MATERIALS SCIENCE</topic><topic>Microstructure evolution</topic><topic>Phase-field simulation</topic><topic>Reduced order model</topic><topic>SOFC degradation</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Lei, Yinkai</creatorcontrib><creatorcontrib>Cheng, Tian-Le</creatorcontrib><creatorcontrib>Mebane, David S.</creatorcontrib><creatorcontrib>Wen, You-Hai</creatorcontrib><creatorcontrib>National Energy Technology Laboratory (NETL), Pittsburgh, PA, Morgantown, WV, and Albany, OR (United States)</creatorcontrib><collection>CrossRef</collection><collection>OSTI.GOV - Hybrid</collection><collection>OSTI.GOV</collection><jtitle>Journal of power sources</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lei, Yinkai</au><au>Cheng, Tian-Le</au><au>Mebane, David S.</au><au>Wen, You-Hai</au><aucorp>National Energy Technology Laboratory (NETL), Pittsburgh, PA, Morgantown, WV, and Albany, OR (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Reduced-order model for microstructure evolution prediction in the electrodes of solid oxide fuel cell with dynamic discrepancy reduced modeling</atitle><jtitle>Journal of power sources</jtitle><date>2019-03-15</date><risdate>2019</risdate><volume>416</volume><issue>C</issue><spage>37</spage><epage>49</epage><pages>37-49</pages><issn>0378-7753</issn><eissn>1873-2755</eissn><abstract>Microstructure evolution in the electrodes of solid oxide fuel cell is an important degradation mechanism which reduces active sites for redox reaction and the electric conductivity. Phase field models for microstructure evolution simulation are usually expensive for large scale simulations. In this work, a reduced-order coarsening model is developed using dynamic discrepancy reduced modeling, which reduces the model order by inserting Gaussian process stochastic functions into the dynamic equations of Ostwald ripening. The reduced order model has been calibrated on a dataset generated by a phase field model that has been well validated to experiments. A validating dataset has also been generated with which the model prediction show good agreement. This model is further applied to predict long term microstructure evolution in different SOFC electrodes. This work is the first attempt of building a degradation model of SOFC using data science techniques.
[Display omitted]
•A reduced order coarsening model for microstructure evolution prediction in SOFC electrode.•Dynamic discrepancy reduced modeling is used to enhance the Ostwald ripening model.•Phase field simulations used in model training and validation.•First attempt of applying data science technique in the research of SOFC degradation.</abstract><cop>United States</cop><pub>Elsevier B.V</pub><doi>10.1016/j.jpowsour.2019.01.046</doi><tpages>13</tpages><orcidid>https://orcid.org/0000-0002-0200-1491</orcidid><orcidid>https://orcid.org/0000000202001491</orcidid><oa>free_for_read</oa></addata></record> |
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subjects | Bayesian calibration Dynamic discrepancy reduced modeling ENGINEERING INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY MATERIALS SCIENCE Microstructure evolution Phase-field simulation Reduced order model SOFC degradation |
title | Reduced-order model for microstructure evolution prediction in the electrodes of solid oxide fuel cell with dynamic discrepancy reduced modeling |
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