Hysteresis in the spontaneous emission induced by VO2 phase change
We investigate the spontaneous emission of a two-level quantum emitter in the vicinity of a vanadium dioxide (VO2) thin film. By taking advantage of effective medium techniques to describe the dielectric constant of the VO2, we demonstrate that, in the near-field regime, the spontaneous emission rat...
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Veröffentlicht in: | Journal of the Optical Society of America. B, Optical physics Optical physics, 2019-04, Vol.36 (4) |
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creator | Szilard, Daniela de Melo Kort-Kamp, Wilton Junior Rosa, F. S S Pinheiro, F. A. Farina, C. |
description | We investigate the spontaneous emission of a two-level quantum emitter in the vicinity of a vanadium dioxide (VO2) thin film. By taking advantage of effective medium techniques to describe the dielectric constant of the VO2, we demonstrate that, in the near-field regime, the spontaneous emission rate of both electric and magnetic dipole emitters can be maximized at the insulator-to-metal phase transition temperature of the film. We find that VO2’s thermal hysteresis curve produces clear fingerprints in the emitter’s decay process, offering a new degree of freedom to dynamically control light emission at the nanoscale. We also find that the spontaneous emission rate is a non-monotonic function of the emitter transition wavelength, presenting a pronounced peak at infrared frequencies. Altogether, our results reveal that VO2 phase transition is a promising mechanism to achieve on-demand tuning of an emitter’s lifetime. |
doi_str_mv | 10.1364/JOSAB.36.000C46 |
format | Article |
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S S ; Pinheiro, F. A. ; Farina, C.</creator><creatorcontrib>Szilard, Daniela ; de Melo Kort-Kamp, Wilton Junior ; Rosa, F. S S ; Pinheiro, F. A. ; Farina, C. ; Los Alamos National Lab. (LANL), Los Alamos, NM (United States)</creatorcontrib><description>We investigate the spontaneous emission of a two-level quantum emitter in the vicinity of a vanadium dioxide (VO2) thin film. By taking advantage of effective medium techniques to describe the dielectric constant of the VO2, we demonstrate that, in the near-field regime, the spontaneous emission rate of both electric and magnetic dipole emitters can be maximized at the insulator-to-metal phase transition temperature of the film. We find that VO2’s thermal hysteresis curve produces clear fingerprints in the emitter’s decay process, offering a new degree of freedom to dynamically control light emission at the nanoscale. We also find that the spontaneous emission rate is a non-monotonic function of the emitter transition wavelength, presenting a pronounced peak at infrared frequencies. Altogether, our results reveal that VO2 phase transition is a promising mechanism to achieve on-demand tuning of an emitter’s lifetime.</description><identifier>ISSN: 0740-3224</identifier><identifier>EISSN: 1520-8540</identifier><identifier>DOI: 10.1364/JOSAB.36.000C46</identifier><language>eng</language><publisher>United States: Optical Society of America (OSA)</publisher><subject>Energy Sciences ; Material Science ; MATERIALS SCIENCE</subject><ispartof>Journal of the Optical Society of America. 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(LANL), Los Alamos, NM (United States)</creatorcontrib><title>Hysteresis in the spontaneous emission induced by VO2 phase change</title><title>Journal of the Optical Society of America. B, Optical physics</title><description>We investigate the spontaneous emission of a two-level quantum emitter in the vicinity of a vanadium dioxide (VO2) thin film. By taking advantage of effective medium techniques to describe the dielectric constant of the VO2, we demonstrate that, in the near-field regime, the spontaneous emission rate of both electric and magnetic dipole emitters can be maximized at the insulator-to-metal phase transition temperature of the film. We find that VO2’s thermal hysteresis curve produces clear fingerprints in the emitter’s decay process, offering a new degree of freedom to dynamically control light emission at the nanoscale. We also find that the spontaneous emission rate is a non-monotonic function of the emitter transition wavelength, presenting a pronounced peak at infrared frequencies. Altogether, our results reveal that VO2 phase transition is a promising mechanism to achieve on-demand tuning of an emitter’s lifetime.</description><subject>Energy Sciences</subject><subject>Material Science</subject><subject>MATERIALS SCIENCE</subject><issn>0740-3224</issn><issn>1520-8540</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNotjD1PwzAUAC0EEqEws1rsCf6OPbYRtKBKGfhYK-flhQSBU_Hcof-eSjDdcKdj7FaKSmpn7p_bl-Wq0q4SQjTGnbFCWiVKb404Z4WojSi1UuaSXRF9nhojlCrYanOkjD9IE_Ep8Twip_2cckw4H4jj90Q0zenk-gNgz7sjf28V34-RkMMY0wdes4shfhHe_HPB3h4fXptNuW3XT81yW4IMIZc2ei2kjFoH0dUB9SAtBtPj4AfvHPjaeWc7r7x2AyBoE8wAHixawCCdXrC7v-9MedoRTBlhhDklhLyTVkplnP4FL1BLfA</recordid><startdate>20190401</startdate><enddate>20190401</enddate><creator>Szilard, Daniela</creator><creator>de Melo Kort-Kamp, Wilton Junior</creator><creator>Rosa, F. S S</creator><creator>Pinheiro, F. 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B, Optical physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Szilard, Daniela</au><au>de Melo Kort-Kamp, Wilton Junior</au><au>Rosa, F. S S</au><au>Pinheiro, F. A.</au><au>Farina, C.</au><aucorp>Los Alamos National Lab. (LANL), Los Alamos, NM (United States)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Hysteresis in the spontaneous emission induced by VO2 phase change</atitle><jtitle>Journal of the Optical Society of America. B, Optical physics</jtitle><date>2019-04-01</date><risdate>2019</risdate><volume>36</volume><issue>4</issue><issn>0740-3224</issn><eissn>1520-8540</eissn><abstract>We investigate the spontaneous emission of a two-level quantum emitter in the vicinity of a vanadium dioxide (VO2) thin film. By taking advantage of effective medium techniques to describe the dielectric constant of the VO2, we demonstrate that, in the near-field regime, the spontaneous emission rate of both electric and magnetic dipole emitters can be maximized at the insulator-to-metal phase transition temperature of the film. We find that VO2’s thermal hysteresis curve produces clear fingerprints in the emitter’s decay process, offering a new degree of freedom to dynamically control light emission at the nanoscale. We also find that the spontaneous emission rate is a non-monotonic function of the emitter transition wavelength, presenting a pronounced peak at infrared frequencies. Altogether, our results reveal that VO2 phase transition is a promising mechanism to achieve on-demand tuning of an emitter’s lifetime.</abstract><cop>United States</cop><pub>Optical Society of America (OSA)</pub><doi>10.1364/JOSAB.36.000C46</doi><orcidid>https://orcid.org/0000000206796690</orcidid><oa>free_for_read</oa></addata></record> |
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subjects | Energy Sciences Material Science MATERIALS SCIENCE |
title | Hysteresis in the spontaneous emission induced by VO2 phase change |
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